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Optics Letters

Integrated room temperature single-photon source for quantum key distribution

Helen Zhi Jie Zeng, Minh Anh Phan Ngyuen, Xiaoyu Ai, Adam Bennet, Alexander S. Solntsev, Arne Laucht, Ali Al-Juboori, Milos Toth, Richard P. Mildren, Robert Malaney, Igor Aharonovich

Published Feb 22, 2022• 43 citations
Publisher

Abstract

High-purity single-photon sources (SPS) that can operate at room temperature are highly desirable for a myriad of applications, including quantum photonics and quantum key distribution. In this work, we realize an ultra-bright solid-state SPS based on an atomic defect in hexagonal boron nitride (hBN) integrated with a solid immersion lens (SIL). The SIL increases the source efficiency by a factor of six, and the integrated system is capable of producing over ten million single photons per second at room temperature. Our results are promising for practical applications of SPS in quantum communication protocols.

DOI
10.1364/ol.454450

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High-purity single-photon sources (SPS) that can operate at room temperature are highly desirable for a myriad of applications, including quantum photonics and quantum key distribution. In this work, we realize an ultra-bright solid-state SPS based on an atomic defect in hexagonal boron nitride (hBN) integrated with a solid immersion lens (SIL). The SIL increases the source efficiency by a factor of six, and the integrated system is capable of producing over ten million single photons per second at room temperature. Our results are promising for practical applications of SPS in quantum communication protocols.
High-purity single photon sources (SPS) that can operate at room temperature are highly desirable for a myriad of applications, including quantum photonics and quantum key distribution. In this work, we realise an ultra-bright solid-state SPS based on an atomic defect in hexagonal boron nitride (hBN) integrated with a solid immersion lens (SIL). The SIL increases the source efficiency by a factor of six, and the integrated system is capable of producing over ten million single photons per second at room temperature. Our results are promising for practical applications of SPS in quantum communication protocols.
Single photons are the key ingredient for many photonic quantum technologies including quantum key distribution and measurement-based quantum computing. However, it remains difficult to create devices with the appropriate specifications for use in non-laboratory environments. The optical microcavity platform provides an attractive route towards a room temperature single photon source device. Our ultra-small focused ion beam (FIB) milled open-access cavities offer enhancement of the spontaneous emission rate, tunability of the emission spectrum and increased light collection. The embedment of solid-state emitters within these cavities enables us to create a robust room temperature single photon source device, with the potential for high efficiencies and single photon purities. Defects such as the nitrogen-vacancy (NV) centre in diamond have been shown to be stable room-temperature sources of single photons. There are new single emitters emerging in two-dimensional materials such as hexagonal boron nitride (hBN). Here we present developments in room-temperature coupling of single defects to open-access microcavities of a planar-hemispherical geometry with mode volumes down to λ3. We report enhancements in the spectral density of photons into a single cavity mode, combined with improved single photon purities. It will be shown that the NV-cavity system provides a ~3% single photon emission efficiency with purities of up to 94%. The hBN-cavity system provides count rates >1Mcts/s into a single cavity mode with purities up to 96%. With these high single photon purities, such devices would be robust against photon number splitting attacks making them attractive for applications in quantum cryptography.
Single photon sources based on single emitters such as 2D materials and impurities in diamond are of great interest for many application fields including quantum communication, quantum metrology and quantum sensing. In photometry and radiometry, a single photon source, having the ability to emit only one photon in a well-defined time and frequency domain, represents a promising candidate to realize a photon number-based primary standard for quantum radiometry. At the Korea Research Institute of Standards and Science (KRISS), we have realized three kinds of single photon sources based on various single emitters at room temperature: silicon vacancy in diamond, defects in gallium nitride (GaN), and vacancy in hexagonal boron nitride (hBN). We found common factors related with the relaxation times of the internal states that indirectly affect the photon number stability. We observed a high photon number stability in the GaN emitter due to faster relaxation times compared with the hBN emitter, which on the other hand produced high rates of photons per second (> 106). Moreover, we demonstrate repeatable radiant flux measurements of a bright hBN single photon emitter for a wide radiant flux range from a few tens of femtowatts to one picowatt.
Abstract Quantum key distribution (QKD) is considered the most immediate application to be widely implemented among a variety of potential quantum technologies. QKD enables sharing secret keys between distant users by using photons as information carriers. An ongoing endeavor is to implement these protocols in practice in a robust, and compact manner so as to be efficiently deployable in a range of real‐world scenarios. Single photon sources (SPS) in solid‐state materials are prime candidates in this respect. This article demonstrates a room temperature, discrete‐variable quantum key distribution system using a bright single photon source in hexagonal‐boron nitride, operating in free‐space. Employing an easily interchangeable photon source system, keys with one million bits length, and a secret key of approximately 70000 bits, at a quantum bit error rate of 6%, with ε‐security of 10 −10 are generated. This study demonstrates the first proof of concept finite‐key BB84 QKD system realized with hBN defects.
Sources of pure and indistinguishable single-photons are critical for near-future optical quantum technologies. Recently, color centers hosted by two-dimensional hexagonal boron nitride (hBN) have emerged as a promising platform for high luminosity room temperature single-photon sources. Despite the brightness of the emitters, the spectrum is rather broad and the single-photon purity is not sufficient for practical quantum information processing. Here, we report integration of such a quantum emitter hosted by hBN into a tunable optical microcavity. A small mode volume of the order of λ 3 allows us to Purcell enhance the fluorescence, with the observed excited state lifetime shortening. The cavity significantly narrows the spectrum and improves the single-photon purity by suppression of off-resonant noise. The complete device, including all optics, driving electronics, and control units, is compact and integrated in a small volume of 10 × 10 × 10 cm 3, allowing for portable usage in mobile applications.