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Frontiers in Optics

Coherent and incoherent contribution of population dynamics of semiconductor exciton-polaritons

Jagannath Paul, Hendrik Rose, Jared K. Wahlstrand, T. Meier, Alan D. Bristow

Published Jan 1, 2021• 0 citations
Publisher

Abstract

Population/mixing-time-dependent two-dimensional coherent spectra are presented for exciton-polaritons in a microcavity. Theory based on dynamically-controlled truncation reveals coherent and incoherent contributions to the decay dynamics.
DOI
10.1364/fio.2021.fw5c.6

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Summary form only given. The coherence decay of optically excited electronic systems provides one of the most powerful tools to investigate interaction processes of excited states. In semiconductors, the optical coherence phenomena are usually investigated by nonlinear techniques such as four wave mixing (FWM), photon echo, or reflectivity experiments. Exciton-phonon, exciton-exciton, or exciton-free carriers scattering processes have been explored in recent years with these techniques. As demonstrated recently, a direct measurement of the optical dephasing time can be obtained through the temporal coherent control of electronic excitations. In these experiments, the emission following the excitation by an ultrashort optical pulse sequence, is detected in a non-specular direction (secondary emission). This provides an alternative approach to FWM techniques, which allows us to analyse the scattering processes either with phonons or due to mutual collisions. Using the coherent control technique monitored through the secondary emission (SE), we report on the coherent dynamics of excitons in bare quantum wells (QW) and compare it to that of exciton-polaritons in microcavity (MC) embedded quantum wells.