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Chapman & Hall/CRC eBooks

More Tools for Quantum Control

Domenico D’Alessandro

Published Jul 13, 2021• 0 citations
Publisher

Abstract

This chapter discusses some more tools for the control of quantum systems. A common technique in the control of quantum systems is to transfer population between two energy levels using a field whose frequency is tuned at the energy difference between the selected levels. This idea is at the foundation of quantum optics and the theory of absorption and emission of radiation by atoms. The study of Magnus expansion is more complicated than the study of the Dyson series. In adiabatic quantum computation, the solution of a computational problem is encoded in an eigenstate of a Hamiltonian. A population transfer between two levels which are not directly coupled can be obtained with a technique called STImulated Raman scattering involving Adiabatic Passage, which combines control via frequency tuned pulses with adiabatic control.

DOI
10.1201/9781003051268-8

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This chapter discusses some more tools for the control of quantum systems. A common technique in the control of quantum systems is to transfer population between two energy levels using a field whose frequency is tuned at the energy difference between the selected levels. This idea is at the foundation of quantum optics and the theory of absorption and emission of radiation by atoms. The study of Magnus expansion is more complicated than the study of the Dyson series. In adiabatic quantum computation, the solution of a computational problem is encoded in an eigenstate of a Hamiltonian. A population transfer between two levels which are not directly coupled can be obtained with a technique called STImulated Raman scattering involving Adiabatic Passage, which combines control via frequency tuned pulses with adiabatic control.
This thesis is based upon the work published in the following two articles entitled: Robust Operation of a Universal Set of Logic Gates for Quantum Computation using Adiabatic Population Transfer between Molecular Levels [37], and Piecewise Adiabatic Passage with a Series of Femtosecond Pulses [54]. Both papers involve using the concept of a quantum control phenomenon, known as adiabatic passage in different manners, in order to achieve particular goals. In the first paper we present a robust construction of a set of logic gates operating on a system of qubits encoded in the ro-vibrational eigenstates of an Na₂ molecule using the optical Adiabatic Population Transfer (APT) method. We demonstrate the operation of a complete universal gate-set for quantum computation on a two-qubit system with gate fidelities approaching 99.99%. Like other APT-based processes, the method is robust against substantial fluctuations in the intensity of the laser pulse. Our construction is easily scalable to dealing with a larger number of qubits. The second line of research developed from the desire to merge the robustness of an adiabatic process, as presented in the previous paper, with the speed and additional level of control available by using pulse shaping techniques of broadband pulses. Therein we develop a method of executing complete population transfers between quantum states in a piecewise manner using a series of femtosecond laser pulses. The method can be applied to a large class of problems as it benefits from the high peak powers and large spectral bandwidths afforded by femtosecond pulses. The degree of population transfer is found to be robust to a wide variation in the absolute and relative intensities, durations, and time ordering of the pulses. The method is studied in detail for atomic sodium where piecewise adiabatic population transfer, as well as the induction of Ramsey-type interferences, is demonstrated.
The manipulation of population transfer and the creation of an arbitrary superposition between two atomic states in the framework of a closed inverse Y-type four-level system driven by a series of pulse pairs and an external control field is reported. It is shown that when the laser fields are tuned to resonance with respective transitions, the non-adiabatic coupling between two degenerate adiabatic states can be reduced tremendously and complete population transfer from the initial state to the target state can be achieved in a piecewise manner. Moreover, an arbitrary superposition between the initial state and target state can be created by suitably tuning the Rabi frequency of the control laser field, inter-pair time delay, pulse number or intra-pair time delay between the pump and Stokes pulses. This scheme combines stimulated Raman adiabatic passage and temporal coherent control, and may be useful for quantum information processing and control of chemical reactions.
Shortcuts to adiabaticity in various quantum systems have attracted much attention with their wide applications in quantum information processing and quantum control. In this paper, we concentrate on a stimulated Raman shortcut-to-adiabatic passage in quantum three-level systems. To implement counterdiabatic driving but without additional coupling, we first reduce the quantum three-level systems to effective two-level problems at large intermediate-level detuning, or on resonance, apply counterdiabatic driving along with the unitary transformation and eventually modify the pump and Stokes pulses for achieving fast and high-fidelity population transfer. The required laser intensity and stability against parameter variation are further discussed, to demonstrate the advantage of shortcuts to adiabaticity.
The main goal of this PhD work is an experimental study of coherent excitation of atomic and molecular wavepackets, i.e. superpositions of many quantum eigenstates, by shaped femtosecond pulses. Approaches allowing nearly complete population transfer between quantum eigenstates were well studied in the past within the two level approximation. In this work we focus on adiabatic and non-adiabatic methods of population transfer beyond the two-level approximation. Excitation of multi-level target states is possible due to broad spectrum of an ultrashort pulse which contains frequencies needed for multiple transitions to different states in the final superposition. At the same time, the spectrum of an ultrashort pulse can be modified, or ``shaped'', in order to affect the excitation process and control the amplitudes in the final superposition. Both non-adiabatic and quasi-adiabatic methods were first implemented and studied in electronic wavepackets in alkali atoms. The non-adiabatic approach revealed features linked to the strong-field perturbations of the energy level structure of the quantum system. An adiabatic method was implemented for the first time on a femtosecond time scale, and was thoroughly characterized. The control over complex amplitudes in the target superposition was demonstrated as well as completeness of the population transfer. In the second part of this work, we focused on coherent control of rotational wavepackets in diatomic molecules. Rotational excitation by a periodic train of femtosecond pulses was investigated in the context of ``delta-kicked'' rotor - a paradigm system for studying quantum chaos, and the effect of quantum resonance was demonstrated for the first time in a system of true quantum rotors. Control of uni-directional molecular rotation was proposed and demonstrated with a novel ``chiral pulse train'' - a sequence of femtosecond pulses with polarization rotating from pulse to pulse by a predefined angle. All the developed techniques offer new tools in coherent control of atomic and molecular wavepackets on an ultrashort time scale.