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Optics Communications

Saturation and optical pumping effects in the fluorescence that follows the excitation of the D2 transition in atomic rubidium

G. Quiroz-Sánchez, F. Ramírez-Martínez, L M Hoyos-Campo, J. Flores-Mijangos, J. Jiménez-Mier

Published Dec 12, 2021• 2 citations
Publisher
DOI
10.1016/j.optcom.2021.127727

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The commonly quoted saturation intensity of rubidium (Rb) for D2 transitions is 16.7W.m−2\mathrm{W}.\mathrm{m}^{-2}W.m−2. This value, however, is only accurate for the cycling transition, which renders the Rb atom to resemble a two-level system. In practice, the effective saturation intensity is influenced by various factors, such as the polarization of light, optical pumping, and atom collision which can redistribute the population. As a result, it is crucial to experimentally determine the effective saturation intensity. In this context, we demonstrate a novel yet simple experimental method to measure the effective saturation intensities of Doppler-broadened transitions in atomic vapours. Our method only requires on-resonance absorbance data for various input laser intensities, which can be obtained with a tunable CW laser without the need for precise frequency locking. We applied this method to measure the effective saturation intensities of all four Doppler-broadened D2 transitions in natural rubidium (Rb) vapour (27.8%87Rb and 72.2 %85Rb{}^{\text{8}} {}^{\text{5}}Rb85Rb) atr=35∘Cr={35}^{\circ} \mathrm{C}r=35∘C. The results show that the effective saturation intensities for Rb range from 0.752 to 16.8W.m−2\mathrm{W}.\mathrm{m}^{-2}W.m−2. Notably, for certain transitions (specifically, repump transitions), the effective saturation intensities were smaller than 16.7 W.m−2\mathrm{m}^{-2}m−2(up to an order of magnitude), with potentially important implications for optical pumping in Doppler-broadened transitions.
Rubidium vapor cells play a key role in contemporary quantum optics since they have strong nonlinear interactions with a low-power incident laser light. The simplest nonlinear interaction is the Kerr effect. Although most calculations concentrate on the unsaturated Kerr effect, the saturated Kerr effect has been measured in many materials including 85Rb and 87Rb vapor. Moreover, entanglement-generating vapor cells often operate in the saturated regime. Here, the calculation of the saturated Kerr effect for rubidium vapor at the D2 line uses a density matrix formulation that includes two hyperfine-split levels and all magnetic sublevels in each of the ground and excited states to account for incomplete optical pumping: the transit time of the atoms through the beam is too short to reach a final population distribution. The calculation shows a rapid qualitative change at low optical power, in semiquantitative agreement with experimental data.