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Frustrated Magnetism in Low-Dimensional Lattices

Mayra Tovar

Published Jan 1, 2011• 0 citations
OpenAlex

Abstract

In this dissertation we present the results of a theoretical investigation of spin models on two-dimensional and quasi one-dimensional lattices, all unified under the concept of quantum frustrated antiferromagnetism, and all discussing various aspects of the antiferromagnetic Heisenberg model on the kagomé lattice. In the Introduction (Chapter 1), we discuss at some length such concepts as frustration and superexchange, among others, which are of common relevance in the rest of the chapters. In Chapter 2, we study the effect of Dzyaloshinskii--Moriya (DM) interactions on the zero-temperature magnetic susceptibility of systems whose low energy can be described by short-range valence bond states. Our work shows that this treatment is consistent with the experimentally observed non-vanishing susceptibility -- in the specified temperature limit -- of the spin-1/2 kagomé antiferromagnetic compound ZnCu3(OH)6Cl2, also known as herbertsmithite. Although the objective of this work is explaining the aforementioned characteristic of the experimental system, our methods are more general and we apply them to the checkerboard and Shastry-Sutherland lattices as well. In Chapter 3, we discuss our findings in the study of ghost-mediated domain wall interactions in the diamondback ladder. These domain walls are the the spin excitations -- the kinks and the antikinks -- separating the ground states along one chain of the ladder. While as individual entities an antikink is energy costly and a kink energy free, our study finds that both interact via the ghosts that they produce in the opposite side of the ladder from where they are located. Through the study of these ghosts, we find that domain walls proliferate in the system above a critical value of the system's coupling constants. It is this proliferation that makes their treatment as free, non-interacting particles impossible, so we study here their interactions both quantitatively and qualitatively, in a region where the latter are yet not very strong, namely below the critical point. Based on the calculated two-body interaction potential, domain walls interact attractively (repulsively) when separated at even (odd) distances, with a strength that decays as 1/sp, where s is their separation and p<1. We also consider higher-order interactions. In the last chapter, Chapter 4, we present our study of the spin-1 kagomé Heisenberg antiferromagnet. Our approach is to first consider an SU(2)-symmetric parent Hamiltonian with known ground states on the S=1 kagomé lattice, in which nearest-neighbor Heisenberg interactions are already present. We then enhance these interactions by an additional Heisenberg term added perturbatively in order to move the system closer to a pure Heisenberg antiferromagnet. The results of this enhancement is obtaining a description of the system in terms of an effective Hamiltonian, namely a transverse field Ising AF on the triangular lattice. Based on the particular values of this effective Hamiltonian, our system is found to be in the order-by-disorder phase.

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New States of Matter in Strongly Frustrated Quantum Magnets

Max Hering

We enhance the pseudo-fermion functional-renormalisation-group (PFFRG) method for the investigation of highly frustrated quantum spin systems in two significant ways. On one hand, we generalise the method towards off-diagonal Dzyaloshinsky-Moriya (DM) interactions and single-ion anisotropies. On the other hand, we develop a self-consistent Fock-like mean-field technique which is based on vertex functions from a PFFRG analysis and calculates effective free spinon models for the considered systems at low energies. In Chap. 1, we introduce the fundamental mathematical concepts on which our studies rely. The so-called flow equations for the PFFRG are then derived in Chap. 3. The first part of our original work is presented in Chap. 4 where we, for the first time, extend the PFFRG scheme towards off-diagonal spin interactions and therefore confirm the quite general applicability of this method. There are two important results from our investigations of the spin-1/2 Heisenberg-DM model on the kagome lattice in this chapter. One is that a finite DM interaction enlarges magnetically ordered phases and thereby shrinks the paramagnetic phases which possibly house spin liquid states. The other important result is that the mineral herbertsmithite which inspired this project lies in close proximity to a quantum critical point. We obtain a phase diagram for the considered Hamiltonian and qualitatively good results in comparison to experimental data for herbertsmithite [68,69]. Our collaboration with a research group from Cologne is summarised in Chap. 5. Here, we investigate two different XXZ models with tetragonally split-up second-neighbour Heisenberg interactions and single-ion anisotropies on the diamond lattice in order to study the spin-1 A-site spinel NiRh2O4. We are able to confirm the existence of a paramagnetic phase for one of the considered models. However, such a paramagnetic behaviour cannot be verified for the Hamiltonians suggested in Refs. [29] and [30]. The second main part of this thesis is contained in Chap. 6. The developed PFFRG plus mean-field method enables us to characterise the effective low-energy spinon band structure of the spin-1/2 J1-J2 (nearest-neighbour) Heisenberg model on the square (kagome) lattice. This is achieved by comparing self-consistently determined overall amplitudes for different mean-field ansätze which are taken from corresponding PSG classifications in Refs. [182] and [111]. Our studies imply that the square lattice model realises a SU(2) spin liquid with Pi-fluxes through elementary plaquettes and that the spin-1/2 kagome antiferromagnet is most likely described by a Z2 spin liquid called Z2[0,Pi]Alpha. We argue that our analysed models have current experimental relevance and that the developed techniques show plenty of possibilities for future applications. A detailed summary and discussion of all methods and results is provided in Chap. 7.

•Jan 1, 2019•1 citation

Theory of Quantum Spin Liquids in Quasi 1-D Systems

Amir Mohammadaghaei

Ever since the introduction of resonating valence bond states by P.\\ W.\\ Anderson in 1970s, the search for exotic many--body quantum behavior in peculiar states of matter known as quantum spin liquids has been a central challenge in the field of condensed matter physics. An important searching ground for such \\emph{quantum--ness} is the low energy physics of frustrated magnets. In a quantum system, frustration---the inability of a physical system to achieve a global state that consistently minimizes its energy locally---enables the unavoidable quantum fluctuations to hybridize an extensive number of classical states into highly entangled quantum states at low temperatures. It can be argued that this is the most practical approach to achieve genuine many--body quantum behavior at large scales. The fundamental source of frustration in many physical systems, is the existence of local non--commuting terms. In the case of antiferromagnet spin theories the simplest examples are triangles of nearest--neighboring sites. Consequently, lattices with triangles as building blocks have long been studied in hopes of discovering spin liquids physics. In particular the kagome lattice, which is composed of corner--sharing triangles, has been the center of at least four decades of spin liquid research. This is due to the underconstrained nature of system made out of corner--sharing triangles. After the first three chapters, introduction in chapter~\\ref{chap:intro}, preliminary physics in chapter~\\ref{chap:prelim}, and a brief introduction to spin--liquids in chapter~\\ref{chap:QSLs}, in chapter~\\ref{chap:kagome} I tackle a simpler version of the long-standing problem of spin--$1/2$ Heisenberg antiferromagnets by considering a quasi--1D lattice consisting entirely of corner--sharing triangles, \\emph{kagome strip}. I illustrate that the standard Heisenberg antiferromagnet Hamiltonian over kagome strip is an extended gapless quantum phase, that is well characterized by two fermionic/bosonic gapless modes and power--law decaying spin and bond--energy correlations. I also demonstrate that the correlation functions oscillate at tunably incommensurate wave vectors. It turns out that this phase can be identified by a particular marginal instability of a two-band spinon Fermi surface coupled to an emergent U(1) gauge field. This interpretation is supported by analytic Abelian bosonization and with extensive numerical large--scale density matrix renormalization group study as well as variational Monte Carlo calculations on Gutzwiller ans\\"atz wave functions. This intriguing result is the first numerical demonstration of emergent fermionic spinons in a simple SU(2) invariant nearest-neighbor Heisenberg model beyond the strictly 1D (Bethe chain) limit. The unexpected success of the fermionic spinons in describing the low energy physics of kagome antiferromagnet, reintroduces the questions about the validity of spinon physics as an effective theory of quantum spin liquids. However, numerical methods are still far behind the theoretical advances. And still even today, an accurate description of the quantum spin liquid states using tensor network methods is notoriously challenging. It is known that for large quasi-1D systems, the density matrix renormalization group and related methods usually require significant computational resources and sometimes fail to converge to a satisfactory state. On the other hand, variational wavefunctions acquired from the Gutzwiller projection of gaussian fermionic theories have long served as both a theoretical starting point for the construction of such spin liquid states and as an inspiration for numerical variational Monte Carlo (VMC) to calculate observables of interest. Noting this observation I examine a different method by exploring the possibility of constructing a matrix product state (MPS) representation for a Gutzwiller--projected state from two given MPS representations of gaussian fermionic theories in the \\ref{chap:gutz} chapter. I investigate the complexity of different approaches to achieve Gutzwiller projection for MPSs and introduce the novel algorithm which we call the Guzwiller zipper method. The performance of the algorithm is tested against two copies of a single half-filled band of spin-1/2 fermionic spinons. In a successful attempt to describe the nature of spin liquid states on quasi-1D strips of triangular and kagome-like lattices, I apply this method to two MPS of multi-band fermionic spinon theories and compare with the complexity of the traditional VMC approach. In particular, we methodically disprove the conjecture of a spinon fermi surface spin liquid for the triangular lattice. Finally, I conclude this thesis by laying out a bird's eye view of the current and future of spin liquid physics in kagome and triangular lattices and pointing out numerous possible applications of the novel Gutzwiller zipper method. In addition, I would also discuss its possible extensions to more complicated tensor networks as well as versions for higher spatial dimensions.

•Jan 1, 2020•0 citations

Novel quantum phases in correlated electron systems

Kyusung Hwang

The quantum nature of electrons emerges in various exotic ways when they are put together with quantum many-body interactions. In Mott insulating systems with strong electron correlation, frustration and strong quantum fluctuations promote localized electron spins to form nontrivial quantum paramagnetic phases such as quantum spin liquid and valence bond solid preventing the development of conventional magnetic orders. In this thesis, we study such exotic quantum phases in various different frustrated quantum magnets. First, encouraged by the spin liquid phenomenology observed in Ba3XSb2O9 (X=Cu, Ni), we investigate Z2 spin liquids on a three dimensional triangular lattice by employing the Schwinger boson mean-field theory with projective symmetry group analysis. It is found that a nematic spin liquid is energetically favorable on this lattice structure rather than symmetric spin liquids. Next, we study various valence bond solid phases that can appear in kagome lattice antiferromagnets by generalizing the recently proposed phenomenological Z2 gauge theory for the topological Z2 spin liquid state found in the nearest-neighbor kagome lattice Heisenberg model. This work provides a bridge between the topological spin liquid and valence bond solid phases previously proposed for kagome lattice antiferromagnets via vison condensation in the gauge theory. Then, we consider optical conductivity in Mott insulators as an experimental probe to detect quantum paramagnetic phases like valence bond solid. Applying this idea to deformed kagome lattice antiferromagnet Rb2Cu3SnF12 with a 12-site valence bond solid state, we estimate the size of optical conductivity in this quantum magnet. After this, another quantum paramagnet BiCu2PO6 is carefully investigated to clarify its puzzling ground state nature and quasiparticle excitations. Utilizing recent high resolution neutron scattering data, we construct a microscopic spin model and also an effective theory for the low energy spin excitations in the compound. We find significant influences of magnetic anisotropies on the ground state and quasiparticle dynamics. Lastly, we investigate emergent quantum phases in the thin film geometries of the pyrochlore iridates, where a number of exotic quantum ground states are proposed to occur in bulk materials as a result of the interplay between electron correlation and strong spin-orbit coupling. The fate of these bulk phases, as well as the novel quantum states that may arise only in a thin film setting, are studied via a theoretical model that allows layer-dependent magnetic structures.

•Nov 1, 2016•0 citations

One-dimensional bosonization approach to higher dimensions

Vladimir A. Zyuzin

This dissertation is devoted to theoretical studies of strongly interacting one-dimensional and quasi one-dimensional electron systems. The properties of one-dimensional electron systems can be studied within the bosonization technique, which presents fermions as collective bosonic density excitations. The power of this approach is the ability to treat electron-electron interaction exactly in the low-energy limit. The approach predicts the failure of Fermi liquid and an absence of long-range order in one-dimensions. The low-energy description of one-dimensional interacting systems is called the Tomonaga-Luttinger liquid theory. For example, the edges of quantum Hall systems are one-dimensional and described by a chiral Tomonaga-Luttinger liquid. Another example is a quantum spin Hall system with helical edge states, which are also described by a Tomonaga-Luttinger liquid. In our first work, a study of magnetized edge states of quantum spin-Hall system is presented. A magnetic field dependent signature of such edges is obtained, which can be verified in a Coulomb drag experiment. The second part of the dissertation is devoted to quasi-one dimensional antiferromagnetic lattices. A spatially anisotropic lattice antiferromagnet can be viewed as an array of one dimensional spin chains coupled in a way to match the lattice symmetry. This allows to use the non-Abelian bosonization technique to describe the low-energy physics of spin chains and study the inter-chain interactions perturbatively. The work presented in the dissertation studies the effect of Dzyaloshinskii-Moriya interaction on the magnetic phase diagram of the spatially anisotropic kagome antiferromagnet. We predict a Dzyaloshinskii-Moriya interaction driven phase transition from Neel to Neel+dimer state. In the third work, a novel model of the fractional quantum Hall effect is given. Wave functions of two-dimensional electrons in strong and quantizing magnetic field are essentially one-dimensional. That invites one to use the one-dimensional phenomenological bosonization to describe the density fluctuations of the two-dimensional interacting electrons in magnetic field. Remarkably, the constructed trial bosonized fermion operator describing the electron states with a fixed Landau gauge momentum is effectively two-dimensional.

•May 1, 2012•0 citations

Emergent quasi-one-dimensionality in a kagome magnet: A simple route to complexity

Shou-Shu Gong, Wei Kang Zhu, Kun Yang +3 more

We study the ground-state phase diagram of the quantum $\text{spin-}1/2$ Heisenberg model on the kagome lattice with first- $({J}_{1}<0)$, second- $({J}_{2}<0)$, and third-neighbor interactions $({J}_{d}>0)$ by means of analytical low-energy field theory and numerical density-matrix renormalization group (DMRG) studies. The results offer a consistent picture of the ${J}_{d}\text{-dominant}$ regime in terms of three sets of spin chains weakly coupled by the ferromagnetic interchain interactions ${J}_{1,2}$. When either ${J}_{1}$ or ${J}_{2}$ is much stronger than the other one, the model is found to support one of two cuboctohedral phases, cuboc1, and cuboc2. These cuboc states host noncoplanar long-ranged magnetic order and possess finite scalar spin chirality. However, in the compensated regime ${J}_{1}\ensuremath{\simeq}{J}_{2}$, a valence bond crystal phase emerges between the two cuboc phases. We find excellent agreement between an analytical theory based on coupled spin chains and unbiased DMRG calculations, including at a very detailed level of comparison of the structure of the valence bond crystal state. To our knowledge, this is the first such comprehensive understanding of a highly frustrated two-dimensional quantum antiferromagnet. We find no evidence of either the one-dimensional gapless spin liquid or the chiral spin liquids, which were previously suggested by parton mean-field theories.

arXiv:1604.01459•Physical review. B./Physical review. B•Jul 27, 2016•27 citations

Chern-Simons theory of magnetization plateaus on the kagome lattice

Ponnuraj Krishnakumar

Frustrated spin systems on Kagome lattices have long been considered to be a promising candidate for realizing exotic spin liquid phases. Recently, there has been a lot of renewed interest in these systems with the discovery of experimental materials such as Volborthite and Herbertsmithite that have Kagome like structures. In this thesis I will focus on studying frustrated spin systems on the Kagome lattice using a spin-1/2 antiferromagnetic XXZ Heisenberg model in the presence of an external magnetic field as well as other perturbations. Such a system is expected to give rise to magnetization platueaus which can exhibit topological characteristics in certain regimes. We will first develop a flux-attachment transformation that maps the Heisenberg spins (hard-core bosons) onto a problem of fermions coupled to a Chern-Simons gauge field. This mapping relies on being able to define a consistent Chern-Simons term on the lattice. Using this newly developed mapping we analyse the phases/magnetization plateaus that arise at the mean-field level and also consider the effects of adding fluctuations to various mean-fi eld states. Along the way, we show how to discretize an abelian Chern-Simons gauge theory on generic 2D planar lattices that satisfy certain conditions. We find that as long as there exists a one-to-one correspondence between the vertices and plaquettes defined on the graph, one can write down a discretized lattice version of the abelian Chern-Simons gauge theory. Using the newly developed flux attachment transformation, we show the existence of chiral spin liquid states for various magnetization plateaus for certain range of parameters in the XXZ Heisenberg model in the presence of an external magnetic field. Speci cally, in the regime of XY anisotropy the ground states at the 1/3 and 2/3 plateau are equivalent to a bosonic fractional quantum Hall Laughlin state with filling fraction 1/2 and that the 5/9 plateau is equivalent to the first bosonic Jain daughter state at filling fraction 2/3. Next, we also consider the effects of several perturbations: a) a chirality term, b) a Dzyaloshinskii-Moriya term, and c) a ring-exchange type term on the bowties of the kagome lattice, and inquire if they can also support chiral spin liquids as ground states. We find that the chirality term leads to a chiral spin liquid even in the absence of an uniform magnetic field, with an effective spin Hall conductance of 1/2 in the regime of XY anisotropy. The Dzyaloshinkii-Moriya term also leads a similar chiral spin liquid but only when this term is not too strong. An external magnetic field when combined with some of the above perturbations also has the possibility of giving rise to additional plateaus which also behave like chiral spin liquids in the XY regime. Under the in influence of a ring-exchange term we find that provided its coupling constant is large enough, it may trigger a phase transition into a chiral spin liquid by the spontaneous breaking of time-reversal invariance. Finally, we also present some numerical results based on some exact diagonalization studies. Here, we specifically focus on the 2/3-magnetization plateau which we previously argued should be a chiral spin liquid with a spin hall conductance of 1/2 . Such a topological state has a non-trivial ground state degeneracy and it excitations are described by semionic quasiparticles. In the numerical analysis, we analyse the ground state degeneracy structure on various Kagome clusters of different sizes. We compute modular matrices from the resultant minimally entangled states as well as the Chern numbers of various eigenstates all of which provide strong evidence that the 2/3-magnetization plateau very closely resembles a chiral spin liquid state with the expected characteristics.

•Nov 29, 2016•0 citations
In this dissertation we present the results of a theoretical investigation of spin models on two-dimensional and quasi one-dimensional lattices, all unified under the concept of quantum frustrated antiferromagnetism, and all discussing various aspects of the antiferromagnetic Heisenberg model on the kagomé lattice. In the Introduction (Chapter 1), we discuss at some length such concepts as frustration and superexchange, among others, which are of common relevance in the rest of the chapters. In Chapter 2, we study the effect of Dzyaloshinskii--Moriya (DM) interactions on the zero-temperature magnetic susceptibility of systems whose low energy can be described by short-range valence bond states. Our work shows that this treatment is consistent with the experimentally observed non-vanishing susceptibility -- in the specified temperature limit -- of the spin-1/2 kagomé antiferromagnetic compound ZnCu3(OH)6Cl2, also known as herbertsmithite. Although the objective of this work is explaining the aforementioned characteristic of the experimental system, our methods are more general and we apply them to the checkerboard and Shastry-Sutherland lattices as well. In Chapter 3, we discuss our findings in the study of ghost-mediated domain wall interactions in the diamondback ladder. These domain walls are the the spin excitations -- the kinks and the antikinks -- separating the ground states along one chain of the ladder. While as individual entities an antikink is energy costly and a kink energy free, our study finds that both interact via the ghosts that they produce in the opposite side of the ladder from where they are located. Through the study of these ghosts, we find that domain walls proliferate in the system above a critical value of the system's coupling constants. It is this proliferation that makes their treatment as free, non-interacting particles impossible, so we study here their interactions both quantitatively and qualitatively, in a region where the latter are yet not very strong, namely below the critical point. Based on the calculated two-body interaction potential, domain walls interact attractively (repulsively) when separated at even (odd) distances, with a strength that decays as 1/sp, where s is their separation and p<1. We also consider higher-order interactions. In the last chapter, Chapter 4, we present our study of the spin-1 kagomé Heisenberg antiferromagnet. Our approach is to first consider an SU(2)-symmetric parent Hamiltonian with known ground states on the S=1 kagomé lattice, in which nearest-neighbor Heisenberg interactions are already present. We then enhance these interactions by an additional Heisenberg term added perturbatively in order to move the system closer to a pure Heisenberg antiferromagnet. The results of this enhancement is obtaining a description of the system in terms of an effective Hamiltonian, namely a transverse field Ising AF on the triangular lattice. Based on the particular values of this effective Hamiltonian, our system is found to be in the order-by-disorder phase.
We enhance the pseudo-fermion functional-renormalisation-group (PFFRG) method for the investigation of highly frustrated quantum spin systems in two significant ways. On one hand, we generalise the method towards off-diagonal Dzyaloshinsky-Moriya (DM) interactions and single-ion anisotropies. On the other hand, we develop a self-consistent Fock-like mean-field technique which is based on vertex functions from a PFFRG analysis and calculates effective free spinon models for the considered systems at low energies. In Chap. 1, we introduce the fundamental mathematical concepts on which our studies rely. The so-called flow equations for the PFFRG are then derived in Chap. 3. The first part of our original work is presented in Chap. 4 where we, for the first time, extend the PFFRG scheme towards off-diagonal spin interactions and therefore confirm the quite general applicability of this method. There are two important results from our investigations of the spin-1/2 Heisenberg-DM model on the kagome lattice in this chapter. One is that a finite DM interaction enlarges magnetically ordered phases and thereby shrinks the paramagnetic phases which possibly house spin liquid states. The other important result is that the mineral herbertsmithite which inspired this project lies in close proximity to a quantum critical point. We obtain a phase diagram for the considered Hamiltonian and qualitatively good results in comparison to experimental data for herbertsmithite [68,69]. Our collaboration with a research group from Cologne is summarised in Chap. 5. Here, we investigate two different XXZ models with tetragonally split-up second-neighbour Heisenberg interactions and single-ion anisotropies on the diamond lattice in order to study the spin-1 A-site spinel NiRh2O4. We are able to confirm the existence of a paramagnetic phase for one of the considered models. However, such a paramagnetic behaviour cannot be verified for the Hamiltonians suggested in Refs. [29] and [30]. The second main part of this thesis is contained in Chap. 6. The developed PFFRG plus mean-field method enables us to characterise the effective low-energy spinon band structure of the spin-1/2 J1-J2 (nearest-neighbour) Heisenberg model on the square (kagome) lattice. This is achieved by comparing self-consistently determined overall amplitudes for different mean-field ansätze which are taken from corresponding PSG classifications in Refs. [182] and [111]. Our studies imply that the square lattice model realises a SU(2) spin liquid with Pi-fluxes through elementary plaquettes and that the spin-1/2 kagome antiferromagnet is most likely described by a Z2 spin liquid called Z2[0,Pi]Alpha. We argue that our analysed models have current experimental relevance and that the developed techniques show plenty of possibilities for future applications. A detailed summary and discussion of all methods and results is provided in Chap. 7.
Ever since the introduction of resonating valence bond states by P.\\ W.\\ Anderson in 1970s, the search for exotic many--body quantum behavior in peculiar states of matter known as quantum spin liquids has been a central challenge in the field of condensed matter physics. An important searching ground for such \\emph{quantum--ness} is the low energy physics of frustrated magnets. In a quantum system, frustration---the inability of a physical system to achieve a global state that consistently minimizes its energy locally---enables the unavoidable quantum fluctuations to hybridize an extensive number of classical states into highly entangled quantum states at low temperatures. It can be argued that this is the most practical approach to achieve genuine many--body quantum behavior at large scales. The fundamental source of frustration in many physical systems, is the existence of local non--commuting terms. In the case of antiferromagnet spin theories the simplest examples are triangles of nearest--neighboring sites. Consequently, lattices with triangles as building blocks have long been studied in hopes of discovering spin liquids physics. In particular the kagome lattice, which is composed of corner--sharing triangles, has been the center of at least four decades of spin liquid research. This is due to the underconstrained nature of system made out of corner--sharing triangles. After the first three chapters, introduction in chapter~\\ref{chap:intro}, preliminary physics in chapter~\\ref{chap:prelim}, and a brief introduction to spin--liquids in chapter~\\ref{chap:QSLs}, in chapter~\\ref{chap:kagome} I tackle a simpler version of the long-standing problem of spin--1/21/21/2 Heisenberg antiferromagnets by considering a quasi--1D lattice consisting entirely of corner--sharing triangles, \\emph{kagome strip}. I illustrate that the standard Heisenberg antiferromagnet Hamiltonian over kagome strip is an extended gapless quantum phase, that is well characterized by two fermionic/bosonic gapless modes and power--law decaying spin and bond--energy correlations. I also demonstrate that the correlation functions oscillate at tunably incommensurate wave vectors. It turns out that this phase can be identified by a particular marginal instability of a two-band spinon Fermi surface coupled to an emergent U(1) gauge field. This interpretation is supported by analytic Abelian bosonization and with extensive numerical large--scale density matrix renormalization group study as well as variational Monte Carlo calculations on Gutzwiller ans\\"atz wave functions. This intriguing result is the first numerical demonstration of emergent fermionic spinons in a simple SU(2) invariant nearest-neighbor Heisenberg model beyond the strictly 1D (Bethe chain) limit. The unexpected success of the fermionic spinons in describing the low energy physics of kagome antiferromagnet, reintroduces the questions about the validity of spinon physics as an effective theory of quantum spin liquids. However, numerical methods are still far behind the theoretical advances. And still even today, an accurate description of the quantum spin liquid states using tensor network methods is notoriously challenging. It is known that for large quasi-1D systems, the density matrix renormalization group and related methods usually require significant computational resources and sometimes fail to converge to a satisfactory state. On the other hand, variational wavefunctions acquired from the Gutzwiller projection of gaussian fermionic theories have long served as both a theoretical starting point for the construction of such spin liquid states and as an inspiration for numerical variational Monte Carlo (VMC) to calculate observables of interest. Noting this observation I examine a different method by exploring the possibility of constructing a matrix product state (MPS) representation for a Gutzwiller--projected state from two given MPS representations of gaussian fermionic theories in the \\ref{chap:gutz} chapter. I investigate the complexity of different approaches to achieve Gutzwiller projection for MPSs and introduce the novel algorithm which we call the Guzwiller zipper method. The performance of the algorithm is tested against two copies of a single half-filled band of spin-1/2 fermionic spinons. In a successful attempt to describe the nature of spin liquid states on quasi-1D strips of triangular and kagome-like lattices, I apply this method to two MPS of multi-band fermionic spinon theories and compare with the complexity of the traditional VMC approach. In particular, we methodically disprove the conjecture of a spinon fermi surface spin liquid for the triangular lattice. Finally, I conclude this thesis by laying out a bird's eye view of the current and future of spin liquid physics in kagome and triangular lattices and pointing out numerous possible applications of the novel Gutzwiller zipper method. In addition, I would also discuss its possible extensions to more complicated tensor networks as well as versions for higher spatial dimensions.
The quantum nature of electrons emerges in various exotic ways when they are put together with quantum many-body interactions. In Mott insulating systems with strong electron correlation, frustration and strong quantum fluctuations promote localized electron spins to form nontrivial quantum paramagnetic phases such as quantum spin liquid and valence bond solid preventing the development of conventional magnetic orders. In this thesis, we study such exotic quantum phases in various different frustrated quantum magnets. First, encouraged by the spin liquid phenomenology observed in Ba3XSb2O9 (X=Cu, Ni), we investigate Z2 spin liquids on a three dimensional triangular lattice by employing the Schwinger boson mean-field theory with projective symmetry group analysis. It is found that a nematic spin liquid is energetically favorable on this lattice structure rather than symmetric spin liquids. Next, we study various valence bond solid phases that can appear in kagome lattice antiferromagnets by generalizing the recently proposed phenomenological Z2 gauge theory for the topological Z2 spin liquid state found in the nearest-neighbor kagome lattice Heisenberg model. This work provides a bridge between the topological spin liquid and valence bond solid phases previously proposed for kagome lattice antiferromagnets via vison condensation in the gauge theory. Then, we consider optical conductivity in Mott insulators as an experimental probe to detect quantum paramagnetic phases like valence bond solid. Applying this idea to deformed kagome lattice antiferromagnet Rb2Cu3SnF12 with a 12-site valence bond solid state, we estimate the size of optical conductivity in this quantum magnet. After this, another quantum paramagnet BiCu2PO6 is carefully investigated to clarify its puzzling ground state nature and quasiparticle excitations. Utilizing recent high resolution neutron scattering data, we construct a microscopic spin model and also an effective theory for the low energy spin excitations in the compound. We find significant influences of magnetic anisotropies on the ground state and quasiparticle dynamics. Lastly, we investigate emergent quantum phases in the thin film geometries of the pyrochlore iridates, where a number of exotic quantum ground states are proposed to occur in bulk materials as a result of the interplay between electron correlation and strong spin-orbit coupling. The fate of these bulk phases, as well as the novel quantum states that may arise only in a thin film setting, are studied via a theoretical model that allows layer-dependent magnetic structures.
This dissertation is devoted to theoretical studies of strongly interacting one-dimensional and quasi one-dimensional electron systems. The properties of one-dimensional electron systems can be studied within the bosonization technique, which presents fermions as collective bosonic density excitations. The power of this approach is the ability to treat electron-electron interaction exactly in the low-energy limit. The approach predicts the failure of Fermi liquid and an absence of long-range order in one-dimensions. The low-energy description of one-dimensional interacting systems is called the Tomonaga-Luttinger liquid theory. For example, the edges of quantum Hall systems are one-dimensional and described by a chiral Tomonaga-Luttinger liquid. Another example is a quantum spin Hall system with helical edge states, which are also described by a Tomonaga-Luttinger liquid. In our first work, a study of magnetized edge states of quantum spin-Hall system is presented. A magnetic field dependent signature of such edges is obtained, which can be verified in a Coulomb drag experiment. The second part of the dissertation is devoted to quasi-one dimensional antiferromagnetic lattices. A spatially anisotropic lattice antiferromagnet can be viewed as an array of one dimensional spin chains coupled in a way to match the lattice symmetry. This allows to use the non-Abelian bosonization technique to describe the low-energy physics of spin chains and study the inter-chain interactions perturbatively. The work presented in the dissertation studies the effect of Dzyaloshinskii-Moriya interaction on the magnetic phase diagram of the spatially anisotropic kagome antiferromagnet. We predict a Dzyaloshinskii-Moriya interaction driven phase transition from Neel to Neel+dimer state. In the third work, a novel model of the fractional quantum Hall effect is given. Wave functions of two-dimensional electrons in strong and quantizing magnetic field are essentially one-dimensional. That invites one to use the one-dimensional phenomenological bosonization to describe the density fluctuations of the two-dimensional interacting electrons in magnetic field. Remarkably, the constructed trial bosonized fermion operator describing the electron states with a fixed Landau gauge momentum is effectively two-dimensional.
We study the ground-state phase diagram of the quantum spin-1/2\text{spin-}1/2spin-1/2 Heisenberg model on the kagome lattice with first- (J1<0)({J}_{1}<0)(J1​<0), second- (J2<0)({J}_{2}<0)(J2​<0), and third-neighbor interactions (Jd>0)({J}_{d}>0)(Jd​>0) by means of analytical low-energy field theory and numerical density-matrix renormalization group (DMRG) studies. The results offer a consistent picture of the Jd-dominant{J}_{d}\text{-dominant}Jd​-dominant regime in terms of three sets of spin chains weakly coupled by the ferromagnetic interchain interactions J1,2{J}_{1,2}J1,2​. When either J1{J}_{1}J1​ or J2{J}_{2}J2​ is much stronger than the other one, the model is found to support one of two cuboctohedral phases, cuboc1, and cuboc2. These cuboc states host noncoplanar long-ranged magnetic order and possess finite scalar spin chirality. However, in the compensated regime ${J}_{1}\ensuremath{\simeq}{J}_{2}$, a valence bond crystal phase emerges between the two cuboc phases. We find excellent agreement between an analytical theory based on coupled spin chains and unbiased DMRG calculations, including at a very detailed level of comparison of the structure of the valence bond crystal state. To our knowledge, this is the first such comprehensive understanding of a highly frustrated two-dimensional quantum antiferromagnet. We find no evidence of either the one-dimensional gapless spin liquid or the chiral spin liquids, which were previously suggested by parton mean-field theories.
Frustrated spin systems on Kagome lattices have long been considered to be a promising candidate for realizing exotic spin liquid phases. Recently, there has been a lot of renewed interest in these systems with the discovery of experimental materials such as Volborthite and Herbertsmithite that have Kagome like structures. In this thesis I will focus on studying frustrated spin systems on the Kagome lattice using a spin-1/2 antiferromagnetic XXZ Heisenberg model in the presence of an external magnetic field as well as other perturbations. Such a system is expected to give rise to magnetization platueaus which can exhibit topological characteristics in certain regimes. We will first develop a flux-attachment transformation that maps the Heisenberg spins (hard-core bosons) onto a problem of fermions coupled to a Chern-Simons gauge field. This mapping relies on being able to define a consistent Chern-Simons term on the lattice. Using this newly developed mapping we analyse the phases/magnetization plateaus that arise at the mean-field level and also consider the effects of adding fluctuations to various mean-fi eld states. Along the way, we show how to discretize an abelian Chern-Simons gauge theory on generic 2D planar lattices that satisfy certain conditions. We find that as long as there exists a one-to-one correspondence between the vertices and plaquettes defined on the graph, one can write down a discretized lattice version of the abelian Chern-Simons gauge theory. Using the newly developed flux attachment transformation, we show the existence of chiral spin liquid states for various magnetization plateaus for certain range of parameters in the XXZ Heisenberg model in the presence of an external magnetic field. Speci cally, in the regime of XY anisotropy the ground states at the 1/3 and 2/3 plateau are equivalent to a bosonic fractional quantum Hall Laughlin state with filling fraction 1/2 and that the 5/9 plateau is equivalent to the first bosonic Jain daughter state at filling fraction 2/3. Next, we also consider the effects of several perturbations: a) a chirality term, b) a Dzyaloshinskii-Moriya term, and c) a ring-exchange type term on the bowties of the kagome lattice, and inquire if they can also support chiral spin liquids as ground states. We find that the chirality term leads to a chiral spin liquid even in the absence of an uniform magnetic field, with an effective spin Hall conductance of 1/2 in the regime of XY anisotropy. The Dzyaloshinkii-Moriya term also leads a similar chiral spin liquid but only when this term is not too strong. An external magnetic field when combined with some of the above perturbations also has the possibility of giving rise to additional plateaus which also behave like chiral spin liquids in the XY regime. Under the in influence of a ring-exchange term we find that provided its coupling constant is large enough, it may trigger a phase transition into a chiral spin liquid by the spontaneous breaking of time-reversal invariance. Finally, we also present some numerical results based on some exact diagonalization studies. Here, we specifically focus on the 2/3-magnetization plateau which we previously argued should be a chiral spin liquid with a spin hall conductance of 1/2 . Such a topological state has a non-trivial ground state degeneracy and it excitations are described by semionic quasiparticles. In the numerical analysis, we analyse the ground state degeneracy structure on various Kagome clusters of different sizes. We compute modular matrices from the resultant minimally entangled states as well as the Chern numbers of various eigenstates all of which provide strong evidence that the 2/3-magnetization plateau very closely resembles a chiral spin liquid state with the expected characteristics.