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CRC Press eBooks

Atomic and Molecular Beams

Cyril Bernard Lucas

Published Nov 27, 2013• 23 citations
Publisher

Abstract

Atomic and molecular beams are employed in physics and chemistry experiments and, to a lesser extent, in the biological sciences. These beams enable atoms to be studied under collision-free conditions and allow the study of their interaction with other atoms, charged particles, radiation, and surfaces. Atomic and Molecular Beams: Production and Col

DOI
10.1201/b16345

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The field of cold molecules has become an important source of new insight in fundamental chemistry and molecular physics. High-resolution spectroscopy benefits from translationally and internally cold molecules by increased interaction times and reduced spectral congestion. Completely new effects in scattering dynamics become accessible with cold and controlled molecules. Many of these experiments use molecular beams as a starting point for the generation of molecular samples. This review gives an overview of methods to produce beams of cold molecules, starting from supersonic expansions or effusive sources, and provides examples of applications in spectroscopy and molecular dynamics studies.

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We describe the state of the art in preparing, manipulating and detecting coherent molecular matter. We focus on experimental methods for handling the quantum motion of compound systems from diatomic molecules to clusters or biomolecules.Molecular quantum optics offers many challenges and innovative prospects: already the combination of two atoms into one molecule takes several well-established methods from atomic physics, such as for instance laser cooling, to their limits. The enormous internal complexity that arises when hundreds or thousands of atoms are bound in a single organic molecule, cluster or nanocrystal provides a richness that can only be tackled by combining methods from atomic physics, chemistry, cluster physics, nanotechnology and the life sciences.We review various molecular beam sources and their suitability for matter-wave experiments. We discuss numerous molecular detection schemes and give an overview over diffraction and interference experiments that have already been performed with molecules or clusters.Applications of de Broglie studies with composite systems range from fundamental tests of physics up to quantum-enhanced metrology in physical chemistry, biophysics and the surface sciences.Nanoparticle quantum optics is a growing field, which will intrigue researchers still for many years to come. This review can, therefore, only be a snapshot of a very dynamical process.

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The design and construction of a molecular-beam apparatus for the production of atomic and molecular beams in the 1 to 10 ev energy range are discussed. A shock tube is used as the source of high-temperature, high-pressure gas, and a hypersonic expansion is used to obtain a high-energy, nearly mono- energetic beam. Use of a two-center potential for the treatment of atom-molecule collisions is discussed. (auth)

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Manipulating atoms with photons

Claude N. Cohen-Tannoudji, Jean Dalibard

Introduction Electromagnetic interactions play a central role in low-energy physics, chemistry, and biology. They are responsible for the cohesion of atoms and molecules and are at the origin of the emission and absorption of light by such systems. They can be described in terms of absorptions and emissions of photons by charged particles or by systems of charged particles like atoms and molecules. Photons are the energy quanta associated with a light beam. Since the discoveries of Planck and Einstein at the beginning of the last century, we know that a plane light wave with frequency ν , propagating along a direction defined by the unit vector u , can also be considered as a beam of photons with energy E = hν and linear momentum p = ( h ν/ c ) u . We shall see later on that these photons also have an angular momentum along u depending on the polarization of the associated light wave. Conservation laws are very useful for understanding the consequences of atom–photon interactions. They express that the total energy, the total linear momentum, and the total angular momentum are conserved when the atom emits or absorbs a photon. Consider for example the conservation of the total energy. Quantum mechanics tells us that the energy of an atom cannot take any value. It is quantized, the possible values of the energy forming a discrete set E a , E b , E c , . . . In an emission process, the atom goes from an upper energy level E b to a lower one E a and emits a photon with energy h ν. Conservation of the total energy requires The energy lost by the atom on going from E b to E a is carried away by the photon.

Cambridge University Press eBooks•Feb 13, 2006•2 citations

Molecular beams

Otto Robert Frisch

Summary Molecular beams are beams of molecules (which may be single atoms) travelling through vacuum at thermal velocities. They have been used to explore many properties of atoms and molecules, chiefly through their deflection in magnetic and electric inhomogeneous fields. Atomic beams first clearly established the phenomenon of space quantization, which means that the magnetic (or electric) energy of an atomic system in a given field can have only certain discrete values, and is not a continuum as classical physics supposed. Transitions between those energy states can be induced by radio-frequency fields; sharp resonances are observed and can be used to get accurate values of atomic and nuclear constants or to provide accurate frequency standards ('atomic clocks'). Molecular beams have also been used to test de Broglie's surmise that beams of particles should show wave properties (diffraction), to study collisions between molecules, and to supply spectroscopic sources in which the line broadening by Doppler effect is greatly reduced.

Contemporary Physics•Oct 1, 1959•3 citations
Atomic and molecular beams are employed in physics and chemistry experiments and, to a lesser extent, in the biological sciences. These beams enable atoms to be studied under collision-free conditions and allow the study of their interaction with other atoms, charged particles, radiation, and surfaces. Atomic and Molecular Beams: Production and Col
The field of cold molecules has become an important source of new insight in fundamental chemistry and molecular physics. High-resolution spectroscopy benefits from translationally and internally cold molecules by increased interaction times and reduced spectral congestion. Completely new effects in scattering dynamics become accessible with cold and controlled molecules. Many of these experiments use molecular beams as a starting point for the generation of molecular samples. This review gives an overview of methods to produce beams of cold molecules, starting from supersonic expansions or effusive sources, and provides examples of applications in spectroscopy and molecular dynamics studies.
We describe the state of the art in preparing, manipulating and detecting coherent molecular matter. We focus on experimental methods for handling the quantum motion of compound systems from diatomic molecules to clusters or biomolecules.Molecular quantum optics offers many challenges and innovative prospects: already the combination of two atoms into one molecule takes several well-established methods from atomic physics, such as for instance laser cooling, to their limits. The enormous internal complexity that arises when hundreds or thousands of atoms are bound in a single organic molecule, cluster or nanocrystal provides a richness that can only be tackled by combining methods from atomic physics, chemistry, cluster physics, nanotechnology and the life sciences.We review various molecular beam sources and their suitability for matter-wave experiments. We discuss numerous molecular detection schemes and give an overview over diffraction and interference experiments that have already been performed with molecules or clusters.Applications of de Broglie studies with composite systems range from fundamental tests of physics up to quantum-enhanced metrology in physical chemistry, biophysics and the surface sciences.Nanoparticle quantum optics is a growing field, which will intrigue researchers still for many years to come. This review can, therefore, only be a snapshot of a very dynamical process.
Recent years have seen tremendous progress in research on cold and controlled molecular collisions, both in theory and in experiment. The advent of techniques to prepare cold and ultracold molecules and ions, to store them in optical lattices or in charged quasicristalline structures, and to use them in crossed or merged beam experiments have opened many new possibilities to study the most fundamental aspects of molecular interactions. At the same time, theoretical work has made progress in tackling these problems and accurately describing quantum effects in complex systems, and in proposing viable options to control chemical reactions at ultralow energies. Through tutorials on both the theoretical and experimental aspects of research in cold and ultracold molecular collisions, this book provides advanced undergraduate students, graduate students and researchers with the foundations needed to understand this exciting field.
Introduction Electromagnetic interactions play a central role in low-energy physics, chemistry, and biology. They are responsible for the cohesion of atoms and molecules and are at the origin of the emission and absorption of light by such systems. They can be described in terms of absorptions and emissions of photons by charged particles or by systems of charged particles like atoms and molecules. Photons are the energy quanta associated with a light beam. Since the discoveries of Planck and Einstein at the beginning of the last century, we know that a plane light wave with frequency ν , propagating along a direction defined by the unit vector u , can also be considered as a beam of photons with energy E = hν and linear momentum p = ( h ν/ c ) u . We shall see later on that these photons also have an angular momentum along u depending on the polarization of the associated light wave. Conservation laws are very useful for understanding the consequences of atom–photon interactions. They express that the total energy, the total linear momentum, and the total angular momentum are conserved when the atom emits or absorbs a photon. Consider for example the conservation of the total energy. Quantum mechanics tells us that the energy of an atom cannot take any value. It is quantized, the possible values of the energy forming a discrete set E a , E b , E c , . . . In an emission process, the atom goes from an upper energy level E b to a lower one E a and emits a photon with energy h ν. Conservation of the total energy requires The energy lost by the atom on going from E b to E a is carried away by the photon.
Summary Molecular beams are beams of molecules (which may be single atoms) travelling through vacuum at thermal velocities. They have been used to explore many properties of atoms and molecules, chiefly through their deflection in magnetic and electric inhomogeneous fields. Atomic beams first clearly established the phenomenon of space quantization, which means that the magnetic (or electric) energy of an atomic system in a given field can have only certain discrete values, and is not a continuum as classical physics supposed. Transitions between those energy states can be induced by radio-frequency fields; sharp resonances are observed and can be used to get accurate values of atomic and nuclear constants or to provide accurate frequency standards ('atomic clocks'). Molecular beams have also been used to test de Broglie's surmise that beams of particles should show wave properties (diffraction), to study collisions between molecules, and to supply spectroscopic sources in which the line broadening by Doppler effect is greatly reduced.