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Quantum impurities in a two-dimensional Heisenberg antiferromagnet

O. P. Vajk

Published Jan 1, 2003• 1 citation
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Long-range dynamics of magnetic impurities coupled to a two-dimensional Heisenberg antiferromagnet

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We consider a two-dimensional Heisenberg antiferromagnet on a square lattice with weakly coupled impurities, i.e., additional spins interacting with the host magnet by a small dimensionless coupling constant $g⪡1$. Using linear spin-wave theory, we find that the magnetization disturbance at distance $r$ from a single impurity behaves as $\ensuremath{\delta}{S}^{z}\ensuremath{\propto}g∕r$ for $1⪡r⪡1∕g$ and as $\ensuremath{\delta}{S}^{z}\ensuremath{\propto}1∕(g{r}^{3})$ for $r⪢1∕g$. Surprisingly the magnetization disturbance is inversely proportional to the coupling constant. The interaction between two impurities separated by a distance $r$ is $\ensuremath{\delta}ϵ\ensuremath{\propto}{g}^{2}∕r$ for $1⪡r⪡1∕g$ and $\ensuremath{\delta}ϵ\ensuremath{\propto}1∕{r}^{3}$ for $r⪢1∕g$. For large distances, the interaction is therefore universal and independent of the coupling constant. We have also found that the frequency of Rabi oscillations between two impurities is logarithmically enhanced compared to the decay width ${\ensuremath{\omega}}_{\mathrm{Rabi}}\ensuremath{\propto}{g}^{2}\phantom{\rule{0.2em}{0ex}}\mathrm{ln}(1∕\mathit{gr})$ at $1⪡r⪡1∕g$. This leads to a logarithmic enhancement for NMR and EPR line broadening. All these astonishing results are due to the gapless spectrum of magnetic excitations in the quantum antiferromagnet.

arXiv:cond-mat/0408598•Physical Review B•Feb 23, 2005•16 citations
The two-dimensional quantum Heisenberg antiferromagnet at zero temperature, with locally frustrating magnetic defects, is studied. We consider two types of defects---an isolated ferromagnetic bond (FMB) and a quantum impurity spin, coupled symmetrically to the two sublattices. A technique is developed to study strong defect-environment interaction. In the case of a FMB we find that, contrary to the previous linear spin-wave result, the local magnetization stays finite even for strong frustration. For an antiferromagnetic coupling of a quantum impurity spin with its environment, we find a local change in the ground state. All our calculations are compared with numerical results from exact diagonalization.
We consider a two-dimensional Heisenberg antiferromagnet on a square lattice with weakly coupled impurities, i.e., additional spins interacting with the host magnet by a small dimensionless coupling constant g⪡1g⪡1g⪡1. Using linear spin-wave theory, we find that the magnetization disturbance at distance rrr from a single impurity behaves as $\ensuremath{\delta}{S}^{z}\ensuremath{\propto}g∕r$ for 1⪡r⪡1∕g1⪡r⪡1∕g1⪡r⪡1∕g and as $\ensuremath{\delta}{S}^{z}\ensuremath{\propto}1∕(g{r}^{3})$ for r⪢1∕gr⪢1∕gr⪢1∕g. Surprisingly the magnetization disturbance is inversely proportional to the coupling constant. The interaction between two impurities separated by a distance rrr is $\ensuremath{\delta}ϵ\ensuremath{\propto}{g}^{2}∕r$ for 1⪡r⪡1∕g1⪡r⪡1∕g1⪡r⪡1∕g and $\ensuremath{\delta}ϵ\ensuremath{\propto}1∕{r}^{3}$ for r⪢1∕gr⪢1∕gr⪢1∕g. For large distances, the interaction is therefore universal and independent of the coupling constant. We have also found that the frequency of Rabi oscillations between two impurities is logarithmically enhanced compared to the decay width ${\ensuremath{\omega}}_{\mathrm{Rabi}}\ensuremath{\propto}{g}^{2}\phantom{\rule{0.2em}{0ex}}\mathrm{ln}(1∕\mathit{gr})$ at 1⪡r⪡1∕g1⪡r⪡1∕g1⪡r⪡1∕g. This leads to a logarithmic enhancement for NMR and EPR line broadening. All these astonishing results are due to the gapless spectrum of magnetic excitations in the quantum antiferromagnet.