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Chinese Journal of Physics

Statistical Properties of Light Interacting with Two-Level Atoms

T. H. Cheung

Published Dec 1, 1988• 0 citations
OpenAlex

Abstract

The quantum-statistical properties of light interacting with a collection of two-level atoms are investigated without making the rotating-wave approximation. Corrections to the steady-state mean photon number, the second-order coherence properties of light and behavior of the average light field are obtained.

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Two-photon absorption and emission for a collection of two level atoms from a single mode beam of light are considered and the statistical proper- ties of the field after the interaction are investigated without placing any restriction of the population of the atomic levels . The dynamical behaviour of the field is described by assuming the atomic levels maintained with a nearly fixed popula- tion distribution . By applying iteration methods the time development for the density operator of the field is written and an expression for the coherent component is obtained . This component appears to be present only when there is a coherent component in the field before the interaction . The statistical properties of the field after the interaction, when the mean photon number is large initially, are then discussed and explicit calculations are carried out for some special cases of initial fields . Finally, it is shown that two-photon spontaneous emission field can be expressed as a superposition of chaotic fields .
The effects of two-photon absorption from a single beam of light on the statistical properties of the beam are considered. Simple expressions are obtained for the initial rates of change and limiting steady-state values of the mean photon number and degree of second-order coherence of the beam. The general time dependences of these properties of the light and of the complete photon probability distribution are evaluated for several initial types of beam. The physical significance of the results is described, and their relationship to calculations which use a classical representation of the light is discussed.
The authors consider a system comprised of a collection of identical two-level atoms interacting with the electromagnetic field in the dipole approximation and with an externally applied steady-state coherent driving field. The atoms are considered to interact with each other only via the electromagnetic field and are assumed to be contained within a volume much smaller than a resonance wavelength. The system is treated as a quantum-statistical ensemble in the rotating frame, rotating at the carrier frequency of the externally applied coherent field. The Hamiltonian in this frame is explicitly time independent and the exact analog of a spin temperature is defined. The thermodynamic-Green's-function method is used to determine the thermodynamic equilibrium properties of the system in the rotating frame. This results in a nonlinear relation between the applied field and the field in the volume containing the atoms. The expression is a nonlinear function of the effective or "spin" temperature as well, and has the form of a first-order phase transition with the macroscopic atomic polarization as order parameter. In the low-"spin"-temperature limit, and for perfect tuning, the expression reduces to the exact form of the nonlinear relation for optical bistability derived by Bonifacio and Lugiato and relating the incident and transmitted fields for atoms in a ring cavity in the mean-field approximation. The results contain absorptive as well as dispersive contributions. These results predict essentially different behavior as a function of off tuning compared with behavior predicted by others using statistical steady-state models far from thermodynamic equilibrium. In the limit of zero value for the applied field amplitude, the results reduce to the conditions for the well-known second-order superradiant" phase transition. The condition for the existence of the second-order phase transition is shown to depend on the cavity tuning and the photon escape rate. The authors also show why, in light of the experiments in optical bistability, this second-order phase is difficult to observe.