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Chinese Physics B

Nonreciprocal two-photon transmission and statistics in a chiral waveguide QED system

Lei Wang, Zhen Yi, Lihui Sun, Wen-ju Gu

Published Dec 1, 2021• 8 citations
Publisher

Abstract

We study the nonreciprocal properties of transmitted photons in a chiral waveguide quantum electrodynamics (QED) system, including single- and two-photon transmissions and second-order correlations. For the single-photon transmission, the nonreciprocity is induced by the effects of chiral coupling and atomic dissipation in the weak coupling region. It vanishes in the strong coupling regime when the effect of atomic dissipation becomes ignorable. In the case of two-photon transmission, there exist two ways of going through the emitter: independently as plane waves and formation of bound state. Besides the nonreciprocal behavior of plane waves, the bound state that differs in two directions also alters transmission probabilities. In addition, the second-order correlation of transmitted photons depends on the interference between plane wave and bound state. The destructive interference leads to the strong antibunching in the weak coupling region, while the effective formation of bound state leads to the strong bunching in the intermediate coupling region. However, the negligible interactions for left-propagating photons hardly change the statistics of the input coherent state.

DOI
10.1088/1674-1056/ac3ecc

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We study the nonreciprocal properties of transmitted photons in a chiral waveguide quantum electrodynamics (QED) system, including single- and two-photon transmissions and second-order correlations. For the single-photon transmission, the nonreciprocity is induced by the effects of chiral coupling and atomic dissipation in the weak coupling region. It vanishes in the strong coupling regime when the effect of atomic dissipation becomes ignorable. In the case of two-photon transmission, there exist two ways of going through the emitter: independently as plane waves and formation of bound state. Besides the nonreciprocal behavior of plane waves, the bound state that differs in two directions also alters transmission probabilities. In addition, the second-order correlation of transmitted photons depends on the interference between plane wave and bound state. The destructive interference leads to the strong antibunching in the weak coupling region, while the effective formation of bound state leads to the strong bunching in the intermediate coupling region. However, the negligible interactions for left-propagating photons hardly change the statistics of the input coherent state.
We investigate the generation of nonreciprocal single photons in the chiral waveguide-cavity-emitter system. Due to the chirality of light-emitter interactions, photons in the left direction couple to a cavity which induces only linear optical effects, while photons in the right direction couple to a cavity-emitter system which can generate optical nonlinearity. In the regime of single-photon transmission, photons in the left direction are absorbed by the cavity at the resonance frequency, while photons in the right direction are transmitted due to the Rabi splitting. In the regime of two-photon transmission, optical linearity in the left direction cannot produce photon-photon interactions and does not change the statistics of photons. However, the effective repulsive interaction between photons can be produced by the optical nonlinearity in the right direction, suppressing two-photon transmission (photon blockade). Physically, the photon-photon bound state, which emerges due to the strong-photon-photon correlation mediated by the cavity-emitter system, plays a key role in generation of photon blockade at the resonance frequency. As a result, nonreciprocal single photons can be realized in the combination of single-photon transmission and photon blockade at the resonance frequency. Additionally, photon-photon interactions are sensitive to the width of the wave packet since photons should coincide at the interaction site.
We show that strongly correlated photon transport can be observed in waveguides containing optically dense ensembles of emitters. Remarkably, this occurs even for weak coupling efficiencies. Specifically, we compute the photon transport properties through a chirally coupled system of N two-level systems driven by a weak coherent field, where each emitter can also scatter photons out of the waveguide. The photon correlations arise due to an interplay of nonlinearity and coupling to a loss reservoir, which creates a strong effective interaction between transmitted photons. The highly correlated photon states are less susceptible to losses than uncorrelated photons and have a power-law decay with N. This is described using a simple universal asymptotic solution governed by a single scaling parameter which describes photon bunching and power transmission. We show numerically that, for randomly placed emitters, these results hold even in systems without chirality. The effect can be observed in existing tapered fiber setups with trapped atoms.
Chiral interactions enable directional control of quantum light, providing new routes for nonreciprocal photon dynamics. While previous studies focused on single photon regimes, this work explores the non-Markovian multiphoton regime in a giant nonlinear system nonlocally coupled to a one-dimensional waveguide, with a tunable phase difference breaking parity symmetry. We show that single-photon transport remains reciprocal, but multiphoton dynamics become chiral, generating direction-dependent higher-order correlations and enabling deterministic creation of multiphoton states with nontrivial statistics from a single input direction, even under strong dissipation. The non-Markovian nature allows tuning of transmitted photon statistics via the coupling-point separation. At a specific phase, internal dynamics become Markovian while output photons retain non-Markovian features. Under strong coherent driving, we uncover nonreciprocal dissipative phase transitions and demonstrate how non-Markovianity shapes the critical response. This framework offers a general strategy for controlling chiral multiphoton dynamics in nonlocally coupled waveguide QED systems. Chiral light-matter interactions offer directional control of quantum states. This work demonstrates that a giant quantum emitter with tunable nonlocal coupling to a waveguide enables direction-dependent multiphoton correlations and dissipative phase transitions, providing a route to engineer non-Markovian chiral dynamics.
We examine quantum statistical properties of transmission and reflection from a chiral waveguide coupled to qubits for arbitrary input powers. We report on several remarkable features of output fields such as transparency, quantum nonreciprocity, and the second-order correlation function g ( 2 ) ( 0 ) values less than unity. In particular, for two qubits detuned antisymmetrically with respect to the central waveguide frequency, we find transparency in forward transmission and in photon numbers for arbitrary values of the input powers provided the phase separation between qubits is an integer multiple of π . Values of g ( 2 ) ( 0 ) less than unity can be reached even for nonzero value of the intrinsic damping by using phase separation different from integer multiple of π , marking the transition from classical to quantum light. We also uncover a different type of critical coupling regime for qubits that enables complete suppression of forward-propagating amplitude transmission at specific driving powers, giving rise to enhanced nonreciprocal effects in both transmission and quantum fluctuations in amplitudes. Forward propagation amplifies the quantum fluctuations in amplitudes, while backward propagation significantly suppresses them. These findings open pathways for controlling light-matter interactions in chiral quantum electrodynamics, with potential applications in quantum information and nonreciprocal quantum devices.
We study chiral and nonreciprocal single-photon scattering in a chiral-giant-molecule waveguide-QED system. Here, the giant molecule consists of two coupled giant atoms, which interact with two linear waveguides, forming a four-port quantum device. We obtain the exact analytical expressions of the four scattering amplitudes using a real-space method. Under the Markovian limit, we find that the single-photon scattering behavior is determined by the coupling strength between the giant atoms and the waveguides, the coupling strength between the two giant atoms, and the nondipole effect caused by the phase accumulation of photons traveling between the coupling points. It is also found that chiral and nonreciprocal single-photon scattering can be realized by introducing the chiral coupling to break the symmetry in the coupling configuration between the giant molecule and the waveguides. In addition, an ideal chiral emitter-waveguide coupling enables a directional single-photon routing. In the non-Markovian regime, the scattering spectra are characterized by more abundant structures with multiple peaks and dips. In particular, we demonstrate that the non-Markovian retarded effect can induce the nonreciprocal single-photon scattering. Our results have potential applications in the design of optical quantum devices involving giant atoms, which can provide an efficient platform for studying chiral quantum optics.
In recent years, chiral quantum optics has emerged as an active research area due to the promising applications in quantum information processing as well as nonlinear optics. We present results on the properties of the incoherent component of the transmitted light after transmons chirally coupled to a waveguide. The well-known resonance fluorescence of one chiral transmon resembles nonlinear quantum optics as it can convert the coherent light, with photons having spatially extensive coherence and Poisson distribution, into a field with spatially localized coherence and bunching photon statistics. However, another chiral transmon can undo the effect of the first transmon regardless of the Rabi frequency under the idealization involved in this work. A full wavefunction calculation shows that, in the weak driving limit, this incoherent light mainly comes from two-photon processes - one chiral transmon converts two independent photons into a photon pair with opposite momentum shift. In addition to the driving through the waveguide, a local driving with independently tunable amplitude and phase can address each transmon individually. The interplay between the waveguide driving and local driving modulates the contribution of the incoherent transmission and hence enables the engineering of the quantum statistics of the transmitted field, with tunable g(2)(0)g^{(2)}(0)g(2)(0) spanning anti-bunched, coherent, and strongly bunched regimes.