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arXiv:1803.02428 · Physical Review Letters

Strongly Correlated Photon Transport in Waveguide Quantum Electrodynamics with Weakly Coupled Emitters

Sahand Mahmoodian, Mantas Čepulkovskis, Sumanta Das, Peter Lodahl, Klemens Hammerer, Anders Søndberg Sørensen

Published Oct 3, 2018• 109 citations
arXivHTMLPDF

Abstract

We show that strongly correlated photon transport can be observed in waveguides containing optically dense ensembles of emitters. Remarkably, this occurs even for weak coupling efficiencies. Specifically, we compute the photon transport properties through a chirally coupled system of N two-level systems driven by a weak coherent field, where each emitter can also scatter photons out of the waveguide. The photon correlations arise due to an interplay of nonlinearity and coupling to a loss reservoir, which creates a strong effective interaction between transmitted photons. The highly correlated photon states are less susceptible to losses than uncorrelated photons and have a power-law decay with N. This is described using a simple universal asymptotic solution governed by a single scaling parameter which describes photon bunching and power transmission. We show numerically that, for randomly placed emitters, these results hold even in systems without chirality. The effect can be observed in existing tapered fiber setups with trapped atoms.

DOI
10.1103/physrevlett.121.143601

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•Jan 1, 2013•1 citation
We show that strongly correlated photon transport can be observed in waveguides containing optically dense ensembles of emitters. Remarkably, this occurs even for weak coupling efficiencies. Specifically, we compute the photon transport properties through a chirally coupled system of N two-level systems driven by a weak coherent field, where each emitter can also scatter photons out of the waveguide. The photon correlations arise due to an interplay of nonlinearity and coupling to a loss reservoir, which creates a strong effective interaction between transmitted photons. The highly correlated photon states are less susceptible to losses than uncorrelated photons and have a power-law decay with N. This is described using a simple universal asymptotic solution governed by a single scaling parameter which describes photon bunching and power transmission. We show numerically that, for randomly placed emitters, these results hold even in systems without chirality. The effect can be observed in existing tapered fiber setups with trapped atoms.
We study the nonreciprocal properties of transmitted photons in a chiral waveguide quantum electrodynamics (QED) system, including single- and two-photon transmissions and second-order correlations. For the single-photon transmission, the nonreciprocity is induced by the effects of chiral coupling and atomic dissipation in the weak coupling region. It vanishes in the strong coupling regime when the effect of atomic dissipation becomes ignorable. In the case of two-photon transmission, there exist two ways of going through the emitter: independently as plane waves and formation of bound state. Besides the nonreciprocal behavior of plane waves, the bound state that differs in two directions also alters transmission probabilities. In addition, the second-order correlation of transmitted photons depends on the interference between plane wave and bound state. The destructive interference leads to the strong antibunching in the weak coupling region, while the effective formation of bound state leads to the strong bunching in the intermediate coupling region. However, the negligible interactions for left-propagating photons hardly change the statistics of the input coherent state.
We study the correlated transport of photons through a chain of three-level emitters that are coupled chirally to a photonic mode of a waveguide. It is found that this system can transfer a weak classical input into a strongly correlated state of light in a unitary manner. Our analysis reveals two-photon scattering eigenstates, that are akin to Fano resonances or shape resonances in particle collisions and facilitate the emergence of antibunched light with long-range correlations upon crossing a critical length of the chain. By operating close to conditions of electromagnetically induced transparency of the three-level medium, a high degree of antibunching and photon transmission can be maintained in the presence of moderate losses. These features suggest a promising mechanism for single-photon generation and may open the door to exploring correlated quantum many-body states of light with repulsively interacting photons.
Waveguide QED with cold atoms provides a potent platform for the study of non-equilibrium, many-body, and open-system quantum dynamics. Even with weak coupling and strong photon loss, the collective enhancement of light-atom interactions leads to strong correlations of photons arising in transmission, as shown in recent experiments. Here we apply an improved mean-field theory based on higher-order cumulant expansions to describe the experimentally relevant, but theoretically elusive, regime of weak coupling and strong driving of large ensembles. We determine the transmitted power, squeezing spectra and the degree of second-order coherence, and systematically check the convergence of the results by comparing expansions that truncate cumulants of few-particle correlations at increasing order. This reveals the important role of many-body and long-range correlations between atoms in steady state. Our approach allows to quantify the trade-off between anti-bunching and output power in previously inaccessible parameter regimes. Calculated squeezing spectra show good agreement with measured data, as we present here.
Waveguide QED with cold atoms provides a potent platform for the study of non-equilibrium, many-body, and open-system quantum dynamics. Even with weak coupling and strong photon loss, the collective enhancement of light-atom interactions leads to strong correlations of photons arising in transmission, as shown in recent experiments. Here we apply an improved mean-field theory based on higher-order cumulant expansions to describe the experimentally relevant, but theoretically elusive, regime of weak coupling and strong driving of large ensembles. We determine the transmitted power, squeezing spectra and the degree of second-order coherence, and systematically check the convergence of the results by comparing expansions that truncate cumulants of few-particle correlations at increasing order. This reveals the important role of many-body and long-range correlations between atoms in steady state. Our approach allows to quantify the trade-off between anti-bunching and output power in previously inaccessible parameter regimes. Calculated squeezing spectra show good agreement with measured data, as we present here.
Engineering strong photon–photon interactions at the quantum level have been crucial in various areas of research, notably in quantum information processing and quantum simulation. It is often done by coupling matter strongly to light. A promising way to achieve this is via waveguide quantum electrodynamics (QED). Motivated by these advancements, we study few-photon transport in waveguide QED setups. First, we present a diagrammatic technique to systematically study multiphoton scattering based on the scattering formalism and Green’s function approach. We demonstrate our proposal through physically relevant examples involving scattering of few-photon states from two-level emitters as well as from arrays of correlated Kerr nonlinear resonators described by the Bose–Hubbard model. In the second part, we apply the diagrammatic technique that was developed to perform a comprehensive study on a Bose–Hubbard lattice with a quasi-periodic potential. This model exhibits many-body localisation. We compute the two-photon transmission probability and show that it carries signatures of the underlying localisation transition with close agreement to the participation ratio of the eigenstates. The systematic scattering approach provided in this paper provides a foundation for future works at the interface between quantum optics and condensed matter.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.