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The Theoretical Study Of Multiphoton Ionization of Atom By Multiple Laser Beams

Nilam Shrestha

Published Apr 1, 2014• 0 citations
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Journal of Physics B Atomic Molecular and Optical Physics•Mar 14, 1998•4 citations
We have used interfering multiphoton ionization processes to measure changes in the relative phase between two optical laser beams. In this work, the phase variation is due to the \ensuremath{\pi} phase shift of a focused Gaussian beam as it propagates through the focal region. An array of linear collection electrodes is used to measure the multiphoton ionization rate as a function of the distance from the beam waist when two laser fields are resonant with an atomic transition, one through a linear process, the other through a three-photon process.
The narrow spectral bandwith (0.4 \AA{}) of a Nd-glass laser was tuned over a range of 40 \AA{} to populate selectively the 6f6f6f level of cesium atoms. The resulting variation of the multiphoton ionization probability was investigated as a function of the laser wavelength.
We report a strong suppression of the three-photon ionization resonant with the 2s state of atomic deuterium at 243 nm by the introduction of a second colour (486 nm) coupling the 2s and 4p states. This coupling reduces the ionization probability by several orders of magnitude. The experiment is performed using fundamental and second harmonic frequencies of the same laser, with laser intensities up to a maximum value of and an atomic target density of the order of . The production of both ions and D(2s) atoms is measured as a function of the intensity of the fundamental beam (486 nm). The experimental data are compared with a theoretical calculation using essential states and taking into account the experimental laser bandwidths.