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Journal of Experimental and Theoretical Physics Letters

Correlation Properties of an Optical–Terahertz Biphoton Field

Pavel A. Prudkovskii

Published Aug 1, 2021• 7 citations
Publisher

Abstract

The effect of the structure of angular modes of an optical–terahertz biphoton field appearing in strongly nondegenerate parametric down-conversion on the possibility of measuring nonclassical correlation properties of this field has been studied theoretically. It has been shown that the nonlinear interaction operator describing parametric down-conversion can be diagonalized in the space of azimuth angles if idler radiation has a terahertz frequency. This feature makes it possible to determine azimuthal eigenmodes and the scattering matrix at arbitrary coefficients of the parametric gain. The determined scattering matrix has been used to find the dependences of the normalized correlation function and the noise reduction factor of the optical–terahertz biphoton field on the angular apertures of detectors recording the signal and idler radiation.

DOI
10.1134/s0021364021160098

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The effect of the structure of angular modes of an optical–terahertz biphoton field appearing in strongly nondegenerate parametric down-conversion on the possibility of measuring nonclassical correlation properties of this field has been studied theoretically. It has been shown that the nonlinear interaction operator describing parametric down-conversion can be diagonalized in the space of azimuth angles if idler radiation has a terahertz frequency. This feature makes it possible to determine azimuthal eigenmodes and the scattering matrix at arbitrary coefficients of the parametric gain. The determined scattering matrix has been used to find the dependences of the normalized correlation function and the noise reduction factor of the optical–terahertz biphoton field on the angular apertures of detectors recording the signal and idler radiation.
The angular structure of an optical-terahertz biphoton field generated by strongly non-degenerate parametric down-conversion is studied theoretically. Azimuthal eigenmodes of scattered radiation are found, in the basis of which the nonlinear interaction operator has a diagonal form. The solution of the evolution equations for these eigenmodes allows us to find a scattering matrix describing the intensity and correlation properties of nonclassical optical-terahertz scattered radiation at arbitrary parametric gain and at different frequencies of the idler terahertz wave.
We study conditions for the generation of strongly correlated photons of two extremely different frequency ranges, optical and terahertz, via the spontaneous parametric down-conversion effect in a nonlinear medium. Analytical expressions for the correlation function are derived using equations of the generalized Kirchhoff law for the second-order field moments with account of both classical thermal and quantum vacuum field fluctuations, possible inherent absorption of the medium at terahertz frequencies, and angular divergences of signal and idler radiation caused by a transverse limited spatial profile of the Gaussian pump beam. Associated with the current absence of terahertz photon counting detectors and coincidence schemes, the possible experimental limitations in measuring the second-order optical-terahertz field correlations are studied. Numerical calculations of noncollinear eee-geometry parametric down-conversion in a Mg:LiNbO3\mathrm{Mg}:\mathrm{LiNb}{\mathrm{O}}_{3}Mg:LiNbO3​ crystal demonstrate angular characteristics, particular features of the temperature and spectral behavior of the second-order quantum correlation function of optical-terahertz biphotons.
The possibility to manage and control spectral and spatial properties of optical-terahertz nonclassical fields generated in strongly nondegenerate parametric down-conversion is demonstrated experimentally using Mach-Zehnder nonlinear interferometer and analyzed theoretically in terms of Schmidt modes. The interferometer can be used for measuring the dispersion properties of different materials in the terahertz frequency range. The key point is that the information about these properties is extracted from the measurements in the optical channel due to strong frequency-angular correlations between optical and terahertz photons. The developed theoretical approach is used to predict properties of the optical-terahertz fields and photon correlations in different regimes of nondegenerate parametric down-conversion. The considered interferometer is shown to be a promising source of terahertz fields with new features and frequency-filtered terahertz Schmidt modes.
Frequency-angular characteristics of signal and idler photons generated under spontaneous parametric down-conversion are studied in a strongly frequency nondegenerate regime, without paraxial approximation, accounting for possible inherent absorption of idler waves in a nonlinear crystal, classical thermal field fluctuations, and the multimode character of parametric interaction induced by transverse spatial limitation of the pump beam. Spatial limitation is shown to lead to a huge increase in angular divergence of the idler photons generated at terahertz frequencies. General expressions are obtained for the frequency-angular sensitivity function of the nonlinear-optical terahertz wave detector and for power densities of the signal and idler photon fluxes. The absorption-induced difference in the parametric conversion coefficients for the noise and externally incident radiation of the idler frequency is shown to be described by approximately the same loss factor for all active spatial idler modes. Two different parametric contributions of the internal thermal noise to the number of output idler photons were revealed with different dependence on the idler-wave absorption. Expressions for the loss factors, which describe absorption-induced effects in signal and idler channels, are obtained and shown to be turning into one another by changing the sign of the absorption coefficient. Relative contribution of thermal and quantum field fluctuations into the intrinsic radiation of a nonlinear crystal at signal and idler frequencies is analyzed accounting for the crystal absorption properties.
We examine the features of parametric down-conversion for generating non-classical optical-terahertz biphoton fields. The calculations were performed for a second-order correlation function and noise reduction factor (NRF), which were selected as measures of non-classicality of the field states. NRF measurement schemes were found to be less advantageous. Overall system temperature at which non-classical effects are still observable has been estimated as about 10 K. The priority of the main complicating factors for the quantum-optical measurements in the terahertz range has been determined. Thus, the most important parameter is the temperature of the system, after that come the absorption losses at terahertz frequencies, and the parametric conversion efficiency has the lowest impact. Increasing the pump radiation power has been found to be inefficient for "noise" suppression in this case. The calculations performed were based on lithium niobate dispersion properties due to its outstanding nonlinear optical properties and because it is frequently used for optical-to-terahertz frequency conversion.