SU(N) chiral spin liquids and spin-1/2 plaquette phases in 2D Mott insulators
C. Boos
Abstract
In this thesis, the Hubbard model with hopping amplitude, t, and on-site interaction, U, in the Mott-insulating regime is explored for unconventional magnetic phases at T = 0 K. These phases are captured within effective low-energy descriptions, and are triggered by quantum fluctuations due to finite hopping. We aim for unconventional phases from two mechanisms, an increased symmetry SU(N) with N > 2 compared to the most common SU(2), and highly frustrated interactions. For SU(N)-symmetric fermions in artificial gauge fields, chiral spin liquid phases (CSLs) are investigated. They are determined within effective spin models, which we derive in order six in t/U for the honeycomb lattice for general values of N, and study in detail for the triangular lattice up to order five in t/U for SU(3) and SU(7) by exact diagonalisations and variational Monte Carlo simulations. On the triangular lattice, the third-order effective model is the J -K model with nearest-neighbour coupling, J ∈ R, and ring exchange, K ∈ C. For SU(3) and Im K = 0, the three-sublattice long-range ordered phase is ruled out by a spontaneously time-reversal symmetry breaking π/3-flux CSL through � nite hopping. Further, for Im K = 0, a lattice nematic, a 120◦ long-ranged ordered, and the ferromagnetically ordered phase occur. The CSL is found to be extended to Re K = 0. It is also present in the fourth- and fifth-order model in the most relevant π-flux case, where time-reversal symmetry is spontaneously broken. Together with the estimated metal-insulator transition point at larger hoppings, this CSL is therefore expected to be realised in the SU(3) Hubbard model. The analogous CSL is also predicted for SU(7)-symmetric fermions. Experimental realisations with ultra-cold atoms in optical lattices are described. SrCu2(BO3)2 is a highly frustrated quantum magnet. At ambient pressure it is captured by the spin-1/2 Shastry-Sutherland model, which yields the effective strong-coupling description of the associated SU(2) Hubbard model. To describe SrCu2(BO3)2 under higher pressure, we extend the Shastry-Sutherland model by asymmetric coupling strengths, and find that asymmetries of a few percent are sufficient to replace the empty plaquette singlet phase (EPP) of the Shastry-Sutherland model with the filled plaquette singlet phase (FPP) that is found to be identical to a quasi one-dimensional Haldane phase. These results are achieved by series expansions and infinite projected entangled-pair states. The dispersions and dynamic structure factors of both plaquette phases are derived. The EPP naturally hosts one low-lying triplon, whereas the FPP has two. Therefore, the FPP appears to be the likely candidate for SrCu2(BO3)2 under pressure. The excitations of both phases show some agreement with experimental data if the exchange amplitudes change more than expected. Further measurements are suggested. At last, an orthogonal-plaquette model of spins-1/2 is introduced and proven to host two exact valence bond crystals based on plaquette singlets with an extensive degeneracy at the phase transition. This model exhibits an extensive number of conserved quantities, which is used for further investigations of the phase diagram.