In this thesis, the Hubbard model with hopping amplitude, t, and on-site interaction, U, in the Mott-insulating regime is explored for unconventional magnetic phases at T = 0 K. These phases are captured within effective low-energy descriptions, and are triggered by quantum fluctuations due to finite hopping. We aim for unconventional phases from two mechanisms, an increased symmetry SU(N) with N > 2 compared to the most common SU(2), and highly frustrated interactions. For SU(N)-symmetric fermions in artificial gauge fields, chiral spin liquid phases (CSLs) are investigated. They are determined within effective spin models, which we derive in order six in t/U for the honeycomb lattice for general values of N, and study in detail for the triangular lattice up to order five in t/U for SU(3) and SU(7) by exact diagonalisations and variational Monte Carlo simulations. On the triangular lattice, the third-order effective model is the J -K model with nearest-neighbour coupling, J ∈ R, and ring exchange, K ∈ C. For SU(3) and Im K = 0, the three-sublattice long-range ordered phase is ruled out by a spontaneously time-reversal symmetry breaking π/3-flux CSL through � nite hopping. Further, for Im K = 0, a lattice nematic, a 120◦ long-ranged ordered, and the ferromagnetically ordered phase occur. The CSL is found to be extended to Re K = 0. It is also present in the fourth- and fifth-order model in the most relevant π-flux case, where time-reversal symmetry is spontaneously broken. Together with the estimated metal-insulator transition point at larger hoppings, this CSL is therefore expected to be realised in the SU(3) Hubbard model. The analogous CSL is also predicted for SU(7)-symmetric fermions. Experimental realisations with ultra-cold atoms in optical lattices are described. SrCu2(BO3)2 is a highly frustrated quantum magnet. At ambient pressure it is captured by the spin-1/2 Shastry-Sutherland model, which yields the effective strong-coupling description of the associated SU(2) Hubbard model. To describe SrCu2(BO3)2 under higher pressure, we extend the Shastry-Sutherland model by asymmetric coupling strengths, and find that asymmetries of a few percent are sufficient to replace the empty plaquette singlet phase (EPP) of the Shastry-Sutherland model with the filled plaquette singlet phase (FPP) that is found to be identical to a quasi one-dimensional Haldane phase. These results are achieved by series expansions and infinite projected entangled-pair states. The dispersions and dynamic structure factors of both plaquette phases are derived. The EPP naturally hosts one low-lying triplon, whereas the FPP has two. Therefore, the FPP appears to be the likely candidate for SrCu2(BO3)2 under pressure. The excitations of both phases show some agreement with experimental data if the exchange amplitudes change more than expected. Further measurements are suggested. At last, an orthogonal-plaquette model of spins-1/2 is introduced and proven to host two exact valence bond crystals based on plaquette singlets with an extensive degeneracy at the phase transition. This model exhibits an extensive number of conserved quantities, which is used for further investigations of the phase diagram.
We explore the phase diagram of the
SU(N) Hubbard models describing fermionic alkaline-earth-metal atoms in a square optical lattice with, on average, one atom per site, using a slave rotor mean-field approach. We find that the chiral spin liquid (CSL) predicted for $N\ensuremath{\ge}5$ and large interactions passes through a fractionalized state with a spinon Fermi surface as interactions are decreased before transitioning to a weakly interacting metal. We show that by adding a uniform artificial gauge field with $2\ensuremath{\pi}/N$ flux per plaquette, the CSL becomes the ground state for all $N\ensuremath{\ge}3$ at intermediate interactions, persists to weaker interactions, and exhibits a larger spin gap. For $N\ensuremath{\ge}5$ we find the CSL is the ground state everywhere the system is a Mott insulator. The gauge field stabilization of the CSL at lower interactions, and thus at weaker lattice depths, together with the increased spin gap, can relax the temperature constraints required for its experimental realization in ultracold atom systems.
We study Mott insulators of fermionic alkaline earth atoms, described by Heisenberg spin models with enhanced SU(N) symmetry. In dramatic contrast to SU(2) magnetism, more than two spins are required to form a singlet. On the square lattice, the classical ground state is highly degenerate and magnetic order is thus unlikely. In a large-N limit, we find a chiral spin liquid ground state with topological order and Abelian fractional statistics. We discuss its experimental detection. Chiral spin liquids with non-Abelian anyons may also be realizable with alkaline earth atoms.
In the physics of the fractional quantum Hall (FQH) effect, a zoo of Abelian topological phases can be obtained by varying the magnetic field. Aiming to reach the same phenomenology in spin like systems, we propose a family of
SU(N)-symmetric models in the fundamental representation, on the square lattice with short-range interactions restricted to triangular units, a natural generalization for arbitrary
N of an SU(3) model studied previously where time-reversal symmetry is broken explicitly. Guided by the recent discovery of
SU(2)1 and
SU(3)1 chiral spin liquids (CSL) on similar models we search for topological
SU(N)1 CSL in some range of the Hamiltonian parameters via a combination of complementary numerical methods such as exact diagonalizations (ED), infinite density matrix renormalization group (iDMRG) and infinite Projected Entangled Pair State (iPEPS). Extensive ED on small (periodic and open) clusters up to
N=10 and an innovative
SU(N)-symmetric version of iDMRG to compute entanglement spectra on (infinitely long) cylinders in all topological sectors provide unambiguous signatures of the
SU(N)1 character of the chiral liquids. An SU(4)-symmetric chiral PEPS, constructed in a manner similar to its SU(2) and SU(3) analogs, is shown to give a good variational ansatz of the
N=4 ground state, with chiral edge modes originating from the PEPS holographic bulk-edge correspondence. Finally, we discuss the possible observation of such Abelian CSL in ultracold atom setups where the possibility of varying
N provides a tuning parameter similar to the magnetic field in the physics of the FQH effect.
Quantum spin liquids can be faithfully represented and efficiently characterized within the framework of projected entangled pair states (PEPS). Guided by extensive exact diagonalization and density matrix renormalization group calculations, we construct an optimized symmetric PEPS for a SU(3)_{1} chiral spin liquid on the square lattice. Characteristic features are revealed by the entanglement spectrum (ES) on an infinitely long cylinder. In all three Z_{3} sectors, the level counting of the linear dispersing modes is in full agreement with SU(3)_{1} Wess-Zumino-Witten conformal field theory prediction. Special features in the ES are shown to be in correspondence with bulk anyonic correlations, indicating a fine structure in the holographic bulk-edge correspondence. Possible universal properties of topological SU(N)_{k} chiral PEPS are discussed.
We suggest a class of two-dimensional lattice spin Hamiltonians describing non-Abelian SU(2) chiral spin liquids---spin analogs of fractional non-Abelian quantum Hall states---with gapped bulk and gapless chiral edge excitations described by the SU(2)
n Wess-Zumino-Novikov-Witten conformal field theory. The models are constructed from an array of generalized spin-
n/2 ladders with multi-spin-exchange interactions which are coupled by isolated spins. Such models allow a controllable analytic treatment starting from the one-dimensional limit and are characterized by a bulk gap and non-Abelian SU(2)
n gapless edge excitations.