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Učenye zapiski Kazanskogo gosudarstvennogo universiteta. Seriâ Fiziko-matematičeskie nauki/Učënye zapiski Kazanskogo universiteta. Seriâ Fiziko-matematičeskie nauki

On Solving the Problem of Quasi-Two-Dimensional Supercrystal Nonlinear Resonance Response

E. V. Timoshchenko, V. A. Yurevich

Published Jan 1, 2021• 2 citations
Publisher

Abstract

Taking into account the foundations of the generalized two-level scheme, an analytical solution to the problem of the evolution of superradiance in a quasi-two-dimensional supercrystal formed by quantum dots is obtained under homogeneous lasing field assumption in the resonant medium of the quasicrystal.The calculation was performed for the physical parameters of a semiconductor structure with quantum-well effects in the presence of resonant nonlinearity and intraband relaxation.We use the generalized two-level scheme, which allows us to take into account the self-modulating spectral broadening of the light field due to the absorption of radiation in quasi-resonant transitions in the quantum mechanical material equations, which are solved together with the field coupling equations.A relation is formulated that is analogous to the law of conservation of the polar angle of the Bloch vector for the more general case of interaction under consideration, in which, along with the phase nonlinearity of the response, the spread rate of active dipoles within the spectral line width is taken into account (i.e., the finiteness of the phase relaxation time of elementary emitters).The use of the Bloch vector formalism in this case makes it possible to obtain an analytical solution of the original modification of the nonlinear system of equations for the semiconductor supercrystals response variables and to calculate the shape of the superradiance pulses.The calculations predict the pronounced asymmetry of the pulses emitted by the semiconductor supercrystals.The calculated estimates of the time dynamics of the superradiance process, taking into account the nonlinearities typical for the resonant response, can be used in the development of methods for obtaining and profiling optical pulses in the sub-picosecond range of durations in modern compact nanophotonics devices.

DOI
10.26907/2541-7746.2021.1.21-30

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Taking into account the foundations of the generalized two-level scheme, an analytical solution to the problem of the evolution of superradiance in a quasi-two-dimensional supercrystal formed by quantum dots is obtained under homogeneous lasing field assumption in the resonant medium of the quasicrystal.The calculation was performed for the physical parameters of a semiconductor structure with quantum-well effects in the presence of resonant nonlinearity and intraband relaxation.We use the generalized two-level scheme, which allows us to take into account the self-modulating spectral broadening of the light field due to the absorption of radiation in quasi-resonant transitions in the quantum mechanical material equations, which are solved together with the field coupling equations.A relation is formulated that is analogous to the law of conservation of the polar angle of the Bloch vector for the more general case of interaction under consideration, in which, along with the phase nonlinearity of the response, the spread rate of active dipoles within the spectral line width is taken into account (i.e., the finiteness of the phase relaxation time of elementary emitters).The use of the Bloch vector formalism in this case makes it possible to obtain an analytical solution of the original modification of the nonlinear system of equations for the semiconductor supercrystals response variables and to calculate the shape of the superradiance pulses.The calculations predict the pronounced asymmetry of the pulses emitted by the semiconductor supercrystals.The calculated estimates of the time dynamics of the superradiance process, taking into account the nonlinearities typical for the resonant response, can be used in the development of methods for obtaining and profiling optical pulses in the sub-picosecond range of durations in modern compact nanophotonics devices.
Taking into account the ideas of the generalized two-level scheme, within the framework of the semiclassical approach to the consideration of the resonant interaction of the light field with matter, an analytical solution to the problem of the evolution of superradiance in a quasi-two-dimensional supercrystal formed by quantum dots is obtained. The calculation was carried out for the physical parameters of a semiconductor structure with quantum-well effects in the presence of resonant nonlinearity and intraband relaxation.
We conduct a theoretical study of the nonlinear optical response of a two-dimensional semiconductor quantum-dot supercrystal subjected to a quasiresonant continuous-wave excitation. A constituent quantum dot is modeled as a three-level ladderlike system (comprising the ground, the one-exciton, and the biexction states). To study the stationary response of the supercrystal, we propose an exact linear parametric method of solving the nonlinear steady-state problem, while to address the supercrystal optical dynamics qualitatively, we put forward a method to calculate the bifurcation diagram of the system. Analyzing the dynamics, we demonstrate that the supercrystal can exhibit multistability, periodic and aperiodic self-oscillations, and chaotic behavior, depending on parameters of the supercrystal and excitation conditions. The effects originate from the interplay of the intrinsic nonlinearity of quantum dots and the retarded interdot dipole-dipole interaction. The latter provides a positive feedback which results in the exotic supercrystal optical dynamics. These peculiarities of the supercrystal optical response open up a possibility for all-optical applications and devices. In particular, an all-optical switch, a tunable generator of THz pulses (in self-oscillating regime), a noise generator (in chaotic regime), and a tunable bistable mirror can be designed.
Several modifications of the Maxwell–Bloch equations are presented for analyzing the emission characteristics of pulsed lasers. The analysis is performed under the condition of coherent interaction between light and a gain medium with resonant phase nonlinearity. For the first time, the interrelated factors of instability of the phase relationship of the light field and the response of the medium, caused by the dipole-dipole interaction and the contribution of quasi-resonant polarization, are taken into account. To describe the superradiance (SR) regime, semi-analytical expressions for the response variables in the Bloch vector formalism are refined. Various approximations of the original model are represented by systems of kinetic equations for the field and response variables of the medium, as well as a nonlinear oscillatory equation for the polar angle of the Bloch vector. Modeling of the coherent SR effect in a resonator showed that the temporal structure of SR is extremely sensitive to the resonant nonlinearity of the material response. It is shown that under nonlinear conditions, the typical nutational intensity structure of synchrotron radiation is transformed into a contrasting quasi-periodic modulation of the trailing edge of the main pulse in the subpicosecond range. A computational analysis of the synchrotron radiation process in a resonator is performed for the parameters of semiconductor quantum dot systems in nanoheterostructures. Such systems are considered promising for use in compact optical electronics and photonics devices.
We investigate superradiant lasing in 1D photonic crystal taking into account both homogeneous and inhomogeneous broadening in a two-level active medium. The latter may be based on, e.g., the quantum-well heterostructures and the fibers activated by color centers where Bragg structure can be fabricated artificially by means of a periodic modulation of the cladding layers. The truncated Maxwell-Bloch equations for the counter-propagating waves, the polarization and inversion of an inhomogeneously broadened two-level medium are used to analyze numerically the interplay between the back-scattering, amplification, dispersion, and de-phasing of waves. It is found that, if the photonic band gap is less than the coherent amplification bandwidth, there is a wide range of the pumping and relaxation parameters of a two-level medium where superradiant lasing exists and results in generation of a quasi-periodic and/or chaotic series of powerful and short pulses similar to those of Dicke superfluorescence. It is the cavity mode selection due to distributed feedback caused by the resonant Bragg structure which is responsible for the existence of superradiant lasing. Typical parameters of superradiant photonic-crystal lasers, including lengths, photonic band gaps and relaxation rates, are indicated.
The paper reports the results of a theoretical study of the optical response of a two-dimensional supercrystal composed of quantum emitters with a doublet excited state (V-emitters) to a monochromatic external Gaussian pulse. The response dynamics are studied as a function of the input field’s pulse area. It is shown that the field pulses interacting with the supercrystal lead to the generation of single, double, triple, and arc pulses with durations ten times shorter than those of the exciting pulses. The generation of single ultrashort pulses is shown to be independent of the magnitude of population excitation and can be realized in the presence of phase relaxation. The properties and effects of the optical response considered in this system suggest it may prove promising for applications in nanophotonics and quantum technologies.
We study theoretically the time evolution of nonlinear optical phenomena of a probe electromagnetic field pulse in intersubband transitions of a semiconductor quantum well structure under the influence of a pump electromagnetic field. More specifically, we take into consideration the effects of electron-electron interactions and consider the interaction of a two-subband system with rectangular electromagnetic fields. The spectral form of the linear absorption, dispersion, and nonlinear optical Kerr effect is described, from the time that the external field is applied up until the dynamics of the system has reached a steady state. In order to describe the dynamics of the system, the effective nonlinear Bloch equations are used, in which renormalized terms for the transition energy and the applied field have been added, due to the effects of electron-electron interactions. These equations are properly combined, and the differential equations of the density matrix elements for the several optical phenomena up to third order are derived. These are solved numerically in the whole time range up to the steady state for a GaAs/AlGaAs quantum well structure. We show that the form of the several optical spectra studied here has a significantly altered evolution over time, according to the value of the frequency of the pump field and of electron sheet density. Even in the case in which the spectral form in the steady state case is almost identical for two different sets of parameters, their evolution can be quite different, according to the precise value of these parameters.