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Bulletin of the American Physical Society

A Scalable Nanophotonic Platform for Rare Earth Ions

Subhojit Dutta, Elizabeth A. Goldschmidt, Sabyasachi Barik, Uday Saha, Edo Waks A

Published Mar 5, 2020• 0 citations
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Quantum Nanophotonics with Ytterbium in Yttrium Orthovanadate

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Quantum light-matter interfaces that can reversibly map quantum information between photons and atoms are essential for building future quantum networks. Crystals doped with rare-earth ions (REIs) are an attractive solid-state platform for such light-matter interfaces due to their exceptional optical and spin coherence properties at cryogenic temperatures. Building scalable REI-based technology has proven to be challenging due to the inherently weak coupling of REIs with light. This thesis explores the integration of REIs with nanophotonic resonators to overcome this weak light-matter interaction and enable efficient, scalable quantum light-matter interfaces. Specifically, this work focuses on the development of quantum nanophotonics with ytterbium in yttrium orthovanadate. This thesis begins with an introduction to a nanophotonic platform based on photonic crystal cavities fabricated directly in rare-earth host materials and highlights the initial successes of this platform with neodymium-doped materials. This motivates an examination of the optical and spin coherence properties of 171Yb:YVO4, a REI material that was previously unexplored for quantum technology applications. This material is found to have strong optical transitions compared to other REI-doped materials, a simple energy level structure, and long optical and spin coherence lifetimes. The focus then turns to the detection and coherent manipulation of single ytterbium ions coupled to nanophotonic cavities. The Purcell-enhancement in these cavities enables efficient optical detection and spin initialization of individual ytterbium ions. We identify ions corresponding to different isotopes of ytterbium and show that the coupling of electron and nuclear spin in ytterbium-171 at zero-field gives rise to strong electron-spin-like transitions that are first-order insensitive to magnetic field fluctuations. This allows for coherent microwave control and the observation of long spin coherence lifetimes at temperatures up to 1 K. We then make use of the optical selection rules and energy structure of 171Yb:YVO4 to demonstrate high-fidelity single-shot optical readout of the spin state. These results establish nanophotonic devices in 171Yb:YVO4 as a promising platform for solid-state quantum light-matter interfaces.

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Quantum nanophotonics interfacing optical photons with coherent atomic spins have the potential to revolutionize secure communications, ultra-scale sensing, distributed quantum computing, and enhanced metrology, but currently lack scalable material and device platform necessary for building robust quantum light-matter interfaces. The trivalent rare-earth ion such as erbium (Er3+) is a promising candidate for quantum interfaces because of its narrow optical transition as well as a long spin coherence time. Here, we present an epitaxial Er3+:Y2O3 on silicon platform for scalable quantum light-matter interconnect, enabling efficient spin-photon interfaces based on individual rare-earth qubits and quantum transduction via ensembles of ions.

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Rare-Earth Doped Photonics

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Quantum light-matter interfaces that can reversibly map quantum information between photons and atoms are essential for building future quantum networks. Crystals doped with rare-earth ions (REIs) are an attractive solid-state platform for such light-matter interfaces due to their exceptional optical and spin coherence properties at cryogenic temperatures. Building scalable REI-based technology has proven to be challenging due to the inherently weak coupling of REIs with light. This thesis explores the integration of REIs with nanophotonic resonators to overcome this weak light-matter interaction and enable efficient, scalable quantum light-matter interfaces. Specifically, this work focuses on the development of quantum nanophotonics with ytterbium in yttrium orthovanadate. This thesis begins with an introduction to a nanophotonic platform based on photonic crystal cavities fabricated directly in rare-earth host materials and highlights the initial successes of this platform with neodymium-doped materials. This motivates an examination of the optical and spin coherence properties of 171Yb:YVO4, a REI material that was previously unexplored for quantum technology applications. This material is found to have strong optical transitions compared to other REI-doped materials, a simple energy level structure, and long optical and spin coherence lifetimes. The focus then turns to the detection and coherent manipulation of single ytterbium ions coupled to nanophotonic cavities. The Purcell-enhancement in these cavities enables efficient optical detection and spin initialization of individual ytterbium ions. We identify ions corresponding to different isotopes of ytterbium and show that the coupling of electron and nuclear spin in ytterbium-171 at zero-field gives rise to strong electron-spin-like transitions that are first-order insensitive to magnetic field fluctuations. This allows for coherent microwave control and the observation of long spin coherence lifetimes at temperatures up to 1 K. We then make use of the optical selection rules and energy structure of 171Yb:YVO4 to demonstrate high-fidelity single-shot optical readout of the spin state. These results establish nanophotonic devices in 171Yb:YVO4 as a promising platform for solid-state quantum light-matter interfaces.
Quantum nanophotonics interfacing optical photons with coherent atomic spins have the potential to revolutionize secure communications, ultra-scale sensing, distributed quantum computing, and enhanced metrology, but currently lack scalable material and device platform necessary for building robust quantum light-matter interfaces. The trivalent rare-earth ion such as erbium (Er3+) is a promising candidate for quantum interfaces because of its narrow optical transition as well as a long spin coherence time. Here, we present an epitaxial Er3+:Y2O3 on silicon platform for scalable quantum light-matter interconnect, enabling efficient spin-photon interfaces based on individual rare-earth qubits and quantum transduction via ensembles of ions.