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Physical Review Letters

Two-Photon Laser

B. Nikolaus, D. Z. Zhang, P. E. Toschek

Published Jul 20, 1981• 106 citations
Publisher

Abstract

We have demonstrated a pulsed two-photon laser at the transition $3d^{2}D\ensuremath{-}2s^{2}S$ of atomic Li (frequency ${\ensuremath{\omega}}_{31}$) by (i) generation of a coherent light beam at ${\ensuremath{\omega}}_{x}$, stimulated by light pulses at ${\ensuremath{\omega}}_{1}={\ensuremath{\omega}}_{31}\ensuremath{-}{\ensuremath{\omega}}_{x}$, and (ii) single-pass amplification of injected light at ${\ensuremath{\omega}}_{3}=\frac{{\ensuremath{\omega}}_{31}}{2}$.

DOI
10.1103/physrevlett.47.171

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We have demonstrated a pulsed two-photon laser at the transition 3d2D\ensuremath−2s2S3d^{2}D\ensuremath{-}2s^{2}S3d2D\ensuremath−2s2S of atomic Li (frequency \ensuremathω31{\ensuremath{\omega}}_{31}\ensuremathω31​) by (i) generation of a coherent light beam at \ensuremathωx{\ensuremath{\omega}}_{x}\ensuremathωx​, stimulated by light pulses at \ensuremathω1=\ensuremathω31\ensuremath−\ensuremathωx{\ensuremath{\omega}}_{1}={\ensuremath{\omega}}_{31}\ensuremath{-}{\ensuremath{\omega}}_{x}\ensuremathω1​=\ensuremathω31​\ensuremath−\ensuremathωx​, and (ii) single-pass amplification of injected light at \ensuremathω3=\ensuremathω312{\ensuremath{\omega}}_{3}=\frac{{\ensuremath{\omega}}_{31}}{2}\ensuremathω3​=2\ensuremathω31​​.
Measurements have been made of the rate at which signal photons are produced in a nonlinear crystal in the process of parametric downconversion, when a coherent light beam from a He:Ne laser is injected into the crystal in the direction of the conjugate-idler photons. The latter provides a stimulating field for the downconversion. When the phase matching condition inside the nonlinear medium is satisfied, the rate of downconversion is enhanced by the presence of the He–Ne laser beam by a factor of the form 1 + βIi, where li is the intensity of the He:Ne laser beam. The effect of defocusing either the pump beam or the He–Ne idler beam is investigated. Possible use of this phenomenon to study the photon amplifier with single-photon input will be discussed.
We demonstrate Ramsey spectroscopy with cold 87 Rb atoms via a two-photon Raman process. One laser beam has a cross-over resonant frequency on the 85 Rb transition and the other beam has a 6.8 GHz shifted frequency. These two laser beams fulfill the two-photon Raman resonance condition, which involves a single-photon detuning of −2.6 GHz. By implementing these two lasers on cold 87 Rb atoms, we demonstrate Ramsey spectroscopy with an interrogation time of the intermediate state by using π /2 Raman pulses. In our laser system, we can change the single-photon detuning to 1.2, 4.2 or −5.6 GHz by changing the 85 Rb transition line used as a locking signal and an injected sideband. The laser system that directly uses resonant light on isotope atoms will be described in this paper.
The possibility of realizing an efficient gaseous laser-beam-generating medium that utilizes $\ensuremath{\Lambda}$-type coherently phased (i.e., ``dressed'') atoms for the active laser species, but that does not inherently require the use of external laser beams for pumping, is explored. Specifically, it is investigated if multiphoton stimulated hyper-Raman scattering (SHRS) processes driven by fluorescence radiation generated in a continuous electrical discharge present within the vapor-containing cell could produce continuous-wave (cw) optical gain at the $\ensuremath{\Lambda}$-atom resonance frequencies ${\ensuremath{\omega}}_{o}$ and ${\ensuremath{\omega}}_{o}^{\ensuremath{'}}$. It is deduced that such gain could result from nnn-photon $(n\ensuremath{\geqslant}4)$ SHRS processes only if absorption of fluorescence pump light occurs in the first three transitions of the nnn-photon sequence representing the process unit step. Estimates of the amount of optical gain that could be produced in such a system indicate that it should be sufficient to allow multiwatt cw laser operation to occur on one set of $\ensuremath{\Lambda}$ transitions connecting levels in a ``double-$\ensuremath{\Lambda}$'' structure, with the pump light being discharge-produced fluorescence centered about the transitions of the other $\ensuremath{\Lambda}$ pair. However, to initiate operation of such a device would require injection into the laser optical cavity of intense ``starter'' laser pulses at both lasing frequencies. What should be an optimal experimental configuration for determining feasibility of the proposed laser device is described. In the suggested configuration, Cs-atom $6{S}_{1∕2}\text{\ensuremath{-}}6{P}_{1∕2}$ transitions form the double-$\ensuremath{\Lambda}$ structure.