Single photons are naturally suited to quantum information processes as they can carry entanglement in multiple degrees of freedom and maintain coherence easily. In order to fully harness single photons for this use, it is vital to be able to mould, manipulate and measure their properties in all of these degrees of freedom. In the spirit of working towards this overarching goal, this thesis consists of two experiments that control and evaluate entangled single photon pairs. \n \nIn the first, we generate lattices of spin-orbit entangled photon states which are used in a remote state preparation protocol. The success of the protocol is confirmed by using an electron-multiplying intensified CCD camera and a pixelwise tomography technique. We propose that these hybrid lattice states be used in quantum communications, and quantum sensing and control. The pixelwise analysis may also be helpful for observing other spatially-dependent entangled states. \n \nIn the second, one partner of an energy-time entangled pair is sent through an ultrafast switch which functions by the optical Kerr effect. It is a work-in-progress with the goal of demonstrating a sub-picosecond switching speed for the further manipulation of single photons. All-optical switching is not limited by electronic speed which makes it important for applications for classical and quantum communications, and imaging and microscopy applications. In particular, we propose that this all-optical Kerr switch is used for the reconstruction of a two-photon entangled state in a third-order cross-correlation.
Single photons are naturally suited to quantum information processes as they can carry entanglement in multiple degrees of freedom and maintain coherence easily. In order to fully harness single photons for this use, it is vital to be able to mould, manipulate and measure their properties in all of these degrees of freedom. In the spirit of working towards this overarching goal, this thesis consists of two experiments that control and evaluate entangled single photon pairs. \n \nIn the first, we generate lattices of spin-orbit entangled photon states which are used in a remote state preparation protocol. The success of the protocol is confirmed by using an electron-multiplying intensified CCD camera and a pixelwise tomography technique. We propose that these hybrid lattice states be used in quantum communications, and quantum sensing and control. The pixelwise analysis may also be helpful for observing other spatially-dependent entangled states. \n \nIn the second, one partner of an energy-time entangled pair is sent through an ultrafast switch which functions by the optical Kerr effect. It is a work-in-progress with the goal of demonstrating a sub-picosecond switching speed for the further manipulation of single photons. All-optical switching is not limited by electronic speed which makes it important for applications for classical and quantum communications, and imaging and microscopy applications. In particular, we propose that this all-optical Kerr switch is used for the reconstruction of a two-photon entangled state in a third-order cross-correlation.
The thesis introduces two single-photon experiments with the lattice of spin-orbit arrays. The basic background knowledge has been introduced in Chapter 1. Chapters 2-4 describe the detailed techniques used in these two experiments. \n \nIn the first work, we implement a remote state preparation protocol on our single-photon orbital angular momentum (OAM) lattice state via hybrid-entanglement. Remote state preparation is a variant of quantum state teleportation where the sender knows the transmitted state. It is known to require fewer classical resources and exhibit a nontrivial trade-off between the entanglement and classical communication compared with quantum teleportation. Here we propose a state preparation scheme between two spatially separated photons sharing a hybrid-entangled polarization-OAM state. By sending one of the polarization-entangled photon pairs through Lattice of Optical Vortex prism pairs, we generate a two-dimensional lattice of spin-orbit coupled single-photons. We show that the measurement taken by an electron-multiplying intensified CCD camera on the transformed photons can be remotely prepared by the polarization projection of the other. Our protocol could have a significant impact on long-distance quantum communication with higher channel capacity and lead to more efficient and compatible quantum information processing techniques. \n \nThe second experiment investigates the single-photon Talbot Effect in spin-orbit arrays. The Talbot Effect is a near-field diffraction effect, that occurs with the propagation of periodically structured waves. It has enabled several unique applications in optical metrology, image processing, data transmission, and matter-wave interferometry. We observe that upon propagation, the wavefronts of the single photons manifest self-imaging whereby the OAM lattice intensity profile is recovered. Furthermore, we show that the intensity distribution at each fractional Talbot distance is indicative of the periodic helical phase structure corresponding to a lattice of OAM states. This phenomenon is a significant addition to the toolbox of orbital angular momentum and spin-orbit techniques that are becoming increasingly important in optical implementations of quantum information.
Single photons are a natural platform for quantum technologies as they support entanglement in many degrees of freedom and are inherently well protected from a detrimental type of noise called decoherence. In order to fully exploit photons for quantum technologies, it will be necessary to be able to shape, control, and measure their properties in all degrees of freedom: space, time, frequency, and polarization. \n \n The time-frequency degree of freedom of light is of particular interest for quantum information tasks as it supports various encodings, including frequency bins and time bins, and is intrinsically robust for propagation through long-distance fibre links. Applications which harness quantum correlations in this degree of freedom, referred to as energy-time entanglement, include dispersion cancellation and high-dimensional quantum key distribution. However, detection of this entanglement and observation of these effects requires time resolution beyond the capabilities of current photon detectors. Thus, for operations on ultrafast time scales, more powerful and complex methods are required. \n \n In this thesis, we use a nonlinear technique known as optical gating to surpass the limitations in current detectors and measure single photon pairs, improving the time resolution by two orders of magnitude. When a single photon enters a nonlinear medium at the same time as a strong laser pulse, it may upconvert to a higher energy photon. The strong laser pulse effectively acts as an ultrafast shutter or gate and this creates a high resolution snapshot of the photon in time. Optical gating in conjunction with single photon spectrometers then allow us to measure both the spectral and temporal features of photons on subpicosecond time scales. \n \n These high resolution measurements enable us to explore a host of quantum effects which remained previously inaccessible. First, we directly observe energy-time entanglement, analogous to Einstein-Rosen-Podolsky correlations but \\emph{in frequency and time}. Then, with full control over the dispersion of each photon, we observe nonlocal dispersion cancellation on femtosecond time scales. We also explore ultrafast interferometry in the quantum domain by temporally resolving two-photon interference from a Franson interferometer and observe a violation of the CHSH-Bell inequality. Finally, we show that, using these measurements, it is possible to reconstruct a two-photon energy-time entangled state. Such measurement capabilities will be essential to precisely control both the spectral and temporal shape of entangled photons and to develop new applications in quantum state engineering.
Single photons provide a natural platform for quantum communication and quantum networking, as they can be entangled in many degrees of freedom and maintain coherence over long-distance links. However, while their minimal interactions with the environment isolate them from detrimental noise, it can make them difficult to measure and manipulate. In particular, manipulation on the ultrafast timescale is necessary to fully exploit the energy-time (or spectral) photonic degree of freedom. Full control over the spectral properties of single photons is key to many quantum technologies and opens the door to natural high-dimensional quantum encodings. \n \nIn this thesis, we theoretically and experimentally examine the use of nonlinear optical processes mediated by strong laser pulses as a method to control the spectral properties of ultrafast single photons. By mixing single-photon pulses with strong escort pulses that have been shaped through dispersion in a nonlinear crystal, the shape of the escort is imprinted on the photon, resulting in a custom-tailored upconverted pulse. We theoretically examine this process for quadratic spectral phases and show that it has the potential to be simultaneously effective and efficient for the customization of single-photon spectral waveforms, and can be performed in an entanglement-conserving manner. \n \nWe then experimentally demonstrate the range of this technique through three applications. First, we show that sum-frequency generation with shaped pulses can be used to coherently measure time-bin encoded photons with bin separations on the order of picoseconds, well below the timing resolution of our detectors. Secondly, we show that this technique can be adapted to convert a train of pulses to a frequency comb, which can be read out in a straightforward manner using diffraction-based spectrometry. We also show here that this process can be performed in a polarization-maintaining fashion, and demonstrate that entanglement with a partner photon is conserved with high fidelity. Finally, we show that this process can be viewed as a time lens, which modulates a temporal waveform in an analogous fashion to a lens focusing a beam of light. We apply the time lens to a photon from an energy-time entangled pair, and show negative magnification of the joint spectrum through a reversal of the spectral correlations. Such processes could find application in quantum state engineering and high-speed single-photon measurement.
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
Energy-time entangled photons are critical in many quantum optical phenomena and have emerged as important elements in quantum information protocols. Entanglement in this degree of freedom often manifests itself on ultrafast time scales, making it very difficult to detect, whether one employs direct or interferometric techniques, as photon-counting detectors have insufficient time resolution. Here, we implement ultrafast photon counters based on nonlinear interactions and strong femtosecond laser pulses to probe energy-time entanglement in this important regime. Using this technique and single-photon spectrometers, we characterize all the spectral and temporal correlations of two entangled photons with femtosecond resolution. This enables the witnessing of energy-time entanglement using uncertainty relations and the direct observation of nonlocal dispersion cancellation on ultrafast time scales. These techniques are essential to understand and control the energy-time degree of freedom of light for ultrafast quantum optics.
InAs quantum dots (QDs) can be used as optically coupled quantum storage devices for quantum information applications. The QD can be charged with a single electron, where the spin state (up or down) provides a long lived quantum bit (qubit). The QD's optically excited states are used to initialize, manipulate, and read out the electron spin state with laser pulses. However, most practical quantum information applications require many interacting qubits, forming a quantum network. Since QDs are based on semiconductor technology, and are compatible with standard nano-fabrication processing, there is promise that they can provide a solid state platform where a scalable quantum information architecture is realizable. We focus on scaling the QD system to multiple qubits using intermediate spin-photon entangled states. In this work, experimental and theoretical techniques are developed to study the QD-light matter interaction at the single photon level. Resonance fluorescence from a single QD is experimentally realized, and the single photon nature of the scattered radiation is verified through intensity correlation experiments. Transient fluorescence measurements on resonantly excited QDs are performed using time correlated single photon counting techniques to measure the excited state lifetime. High speed electro-optic modulators are used to time gate narrow bandwidth lasers, so that a QD can be driven under step-wise excitation, allowing for the direct observation of time-dependent optical Rabi oscillations. From these measurements, we are able to extract a decoherence rate which is consistent with the lifetime limit, indicating that pure dephasing is negligible in this system. These techniques are applied to the QD spin system to demonstrate a spin-photon entangled state, by performing correlation measurements on the spin and photon state in two bases. A lower bound on the entanglement fidelity of 0.59(4) is achieved, which exceeds the classical limit of 0.5 by more than two standard deviations. The entanglement fidelity is limited primarily by the finite timing resolution of available single photon detectors. Taking this into account, we achieve 84% of the apparatus limited fidelity. These spin-entangled photons can be used to mediate entanglement between distant QD spins, providing the basis of an optically coupled QD spin network.