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Chinese Physics B

Widely tunable single-photon source with high spectral-purity from telecom wavelength to mid-infrared wavelength based on MgO:PPLN*

Changwei Sun, Yu Sun, Jia-Chen Duan, Guang-Tai Xue, Yichen Liu, Liangliang Lu, Qun-Yong Zhang, Yan-Xiao Gong, Ping Xu, Shining N. Zhu

Published Aug 25, 2021• 5 citations
Publisher

Abstract

By utilizing the extended phase-matching (EPM) method, we investigate the generation of single photons with high spectral-purity in a magnesium-doped periodically-poled lithium niobate (MgO:PPLN) crystal via the spontaneous parametric down-conversion (SPDC) process. By adjusting the temperature and pump wavelength, the wavelength of the single photons can be tuned from telecom to mid-infrared (MIR) wavelengths, for which the spectral-purity can be above 0.95 with high transmission filters. In experiments, we engineer a MgO:PPLN with poling period of 20.35 μm which emits the EPM photon pair centered at 1496.6 nm and 1644.0 nm and carry out the joint spectral intensity (JSI) and Glauber’s second-order self-correlation measurements to characterize the spectral purity. The results are in good agreement with the numerical simulations. Our work may provide a valuable approach for the generation of spectrally pure single photons at a wide range of wavelengths which is competent for various photonic quantum technologies.

DOI
10.1088/1674-1056/ac20cb

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By utilizing the extended phase-matching (EPM) method, we investigate the generation of single photons with high spectral-purity in a magnesium-doped periodically-poled lithium niobate (MgO:PPLN) crystal via the spontaneous parametric down-conversion (SPDC) process. By adjusting the temperature and pump wavelength, the wavelength of the single photons can be tuned from telecom to mid-infrared (MIR) wavelengths, for which the spectral-purity can be above 0.95 with high transmission filters. In experiments, we engineer a MgO:PPLN with poling period of 20.35 μm which emits the EPM photon pair centered at 1496.6 nm and 1644.0 nm and carry out the joint spectral intensity (JSI) and Glauber’s second-order self-correlation measurements to characterize the spectral purity. The results are in good agreement with the numerical simulations. Our work may provide a valuable approach for the generation of spectrally pure single photons at a wide range of wavelengths which is competent for various photonic quantum technologies.
The single-photon source in mid-infrared (MIR) band is very important for the next generation of quantum sensing, quantum communication and quantum imaging. At present, the commonly used method of generating MIR single-photon source is based on the spontaneous parametric down conversion (SPDC) process in the periodically poled lithium niobate (PPLN) crystal. However, the spectral purity of single-photon source based on the ordinary PPLN is not high, specifically, its maximum value is only about 0.82, which affects the fidelity of quantum information processing scheme. In this paper, 4000 polarized domains in a 30-mm-long LN crystal are customized by using the domain design theory. The sidelobes in the phase matching function are eliminated, and the Gaussian distribution is obtained. The calculated spectral purity of the single-photon source can reach 0.99, and its tunable range is 2.7–3.3 μm. The customized poled lithium niobate (CPLN) is expected to provide a single-photon source with excellent performance for the study of quantum information in the MIR band.
We study the spectral correlation of photon pairs generated via type-II spontaneous parametric down conversion in periodically poled lithium niobate crystals. By performing Schmidt decomposition on the two-photon wavefunction, we calculate the spectral purity of the two-photon state under various pump laser characteristics and doping concentrations of MgO in lithium niobate crystals. Our results show that periodically poled 5% MgO doped lithium niobate is a good candidate to generate photon-pairs with high spectral purity at telecom wavelength.
We theoretically and experimentally investigate the spectral tunability and purity of photon pairs generated from spontaneous parametric down conversion in periodically poled KTiOPO(4) crystal with group-velocity matching condition. The numerical simulation predicts that the spectral purity can be kept higher than 0.81 when the wavelength is tuned from 1460 nm to 1675 nm, which covers the S-, C-, L-, and U-band in telecommunication wavelengths. We also experimentally measured the joint spectral intensity at 1565 nm, 1584 nm and 1565 nm, yielding Schmidt numbers of 1.01, 1.02 and 1.04, respectively. Such a photon source is useful for quantum information and communication systems.
Recent advances of high-quality lithium niobate (LN) on insulator technology have revitalized the progress of novel chip-integrated LN-based photonic devices and accelerated application research. One of the promising technologies of interest is the generation of entangled photon pairs based on spontaneous parametric down-conversion (SPDC) in LNs. In this paper, we investigated, theoretically and numerically, Type II SPDC in two kinds of LNs—undoped and 5-mol% MgO doped LNs. In each case, both non-poled and periodically poled crystals were considered. The technique is based on the SPDC under Type II extended phase matching, where the phase matching and the group velocity matching are simultaneously achieved between interacting photons. The proposed approach has not yet been reported for LNs. We discussed all factors required to generate photon pairs in LNs, in terms of the beam propagation direction, the spectral position of photons, and the corresponding effective nonlinearities and walk-offs. We showed that the spectral positions of the generated photon pairs fall into the mid-infrared region with high potential for free-space quantum communication, spectroscopy, and high-sensitivity metrology. The joint spectral analyses showed that photon pairs can be generated with high purities of 0.995–0.999 with proper pump filtering.
We theoretically investigate the preparation of mid-infrared (MIR) spectrally-uncorrelated biphotons from a spontaneous parametric down-conversion process using doped LN crystals, including MgO doped LN, ZnO doped LN, and In2O3 doped ZnLN with doping ratio from 0 to 7 mol%. The tilt angle of the phase-matching function and the corresponding poling period are calculated under type-II, type-I, and type-0 phase-matching conditions. We also calculate the thermal properties of the doped LN crystals and their performance in Hong-Ou-Mandel interference. It is found that the doping ratio has a substantial impact on the group-velocity-matching (GVM) wavelengths. Especially, the GVM2 wavelength of co-doped InZnLN crystal has a tunable range of 678.7 nm, which is much broader than the tunable range of less than 100 nm achieved by the conventional method of adjusting the temperature. It can be concluded that the doping ratio can be utilized as a degree of freedom to manipulate the biphoton state. The spectrally uncorrelated biphotons can be used to prepare pure single-photon source and entangled photon source, which may have promising applications for quantum-enhanced sensing, imaging, and communications at the MIR range.
We demonstrate a spectrally correlated photon-pair source at telecom wavelengths (spanning across the S-, C-, and L-bands), based on type-0 spontaneous parametric downconversion (SPDC) in a fiber-coupled Zn-indiffused MgO doped periodically poled lithium niobate (PPLN) ridge waveguide. Modal analysis of the waveguide performed through numerical finite element method (FEM) simulation indicates that device temperature can be used to dramatically vary and control the emission spectrum. Efficient photon-pair generation is measured over a broad wavelength range from ∼1520 − 1580 nm [full width at half maximum (FWHM) > 45 nm] with a coincidence-to-accidental ratio (CAR) as high as ∼668 and spectral brightness ∼2.5 × 10 7 pairs/s/mW/nm. Such sources can be employed in wavelength division multiplexed (WDM) quantum key distribution (QKD) over existing fiber-optic networks.