Spin-squeezed state is a many-body entangled state of great interest for precision measurements. Although the absolute sensitivity at the standard quantum limit is better for a larger atom number, the greater dominance of classical noises over atom projection noise makes it harder to achieve spin squeezing. Here, we show both theoretically and experimentally that adiabatic pulse control of the pump field in state preparation is indispensable to sufficient noise suppression, which is the prerequisite for spin squeezing. This technique is generally applicable to spin-squeezing experiments involving a large ensemble and is thus of significance for quantum metrology applications.
Spin-squeezed state is a many-body entangled state of great interest for precision measurements. Although the absolute sensitivity at the standard quantum limit is better for a larger atom number, the greater dominance of classical noises over atom projection noise makes it harder to achieve spin squeezing. Here, we show both theoretically and experimentally that adiabatic pulse control of the pump field in state preparation is indispensable to sufficient noise suppression, which is the prerequisite for spin squeezing. This technique is generally applicable to spin-squeezing experiments involving a large ensemble and is thus of significance for quantum metrology applications.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.
Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is beneficial to consider macroscopic spin ensembles, such as nuclear spins in solids and liquids. Coupling a macroscopic spin ensemble to a parametrically-modulated resonant circuit can create collective spin squeezing by generating spin correlations mediated by the circuit. We analyze the squeezing dynamics in the presence of decoherence and finite spin polarization, showing that achieving 7 dB spin squeezing is feasible in several nuclear spin systems. The metrological benefit of squeezing a macroscopic spin ensemble lies in the suppression of technical noise sources in the spin detection system relative to the spin projection noise. This expands the experimental sensitivity bandwidth when searching for signals of unknown frequency and can improve the resonant signal-to-noise ratio. Squeezing macroscopic spin ensembles may prove to be a useful technique for fundamental physics experiments aimed at detecting spin interactions with oscillating background fields, such as ultralight dark matter.
Creating highly spin-squeezed states for quantum metrology surpassing the standard quantum limit is a topic of great interest. Spin squeezing has been achieved by either entangling different atoms in an ensemble, or by controlling the multilevel internal spin state of an atom. Here, we experimentally demonstrate combined internal and collective spin squeezing in a hot atomic ensemble with ∼10^{11} rubidium atoms. By synergistically combining these two types of squeezing and carefully aligning their squeezing quadratures, we have achieved a metrologically relevant spin squeezing of -6.21±0.84 dB, significantly outperforming the results obtained by utilizing either type of squeezing alone in our system. Our approach provides a new perspective on fully harnessing the degrees of freedom inherent in quantum states of an atomic ensemble.
State of the art atomic sensors operate near the standard quantum limit (SQL) of projection noise, and overcoming this limit by using atom-atom entanglement such as spin squeezing is a major goal in quantum metrology. By coupling an ensemble of approximately 1000 Yb-171 atoms to a high-finesse asymmetric micromirror cavity with single-atom cooperativity of 1.8., we produce a near-unitary spin squeezed state. The observed spin noise suppression and metrological gain are limited by the state readout to 9.4(4) dB and 6.5(4) dB, respectively, while the generated states offer a spin noise suppression of 15.9(6) dB and a metrological gain of 12.9(6) dB over the standard quantum limit, limited by the curvature of the Bloch sphere. When requiring the squeezing process to be within 30% of unitarity, we demonstrate an interferometer that improves the averaging time over the SQL by a factor of 3.7(2).
Abstract Spin-squeezed states are metrologically useful quantum states where entanglement allows for enhanced sensing with respect to the standard quantum limit. Key challenges include the efficient preparation of spin-squeezed states and the scalability of estimation precision with the number N of probes. Recently, in the context of the generation of spin-squeezed states via coupling of three-level atoms to an optical cavity, it was shown that increasing the atom-cavity coupling can be detrimental to spin squeezing generation, an effect that is not captured by the standard second-order adiabatic cavity removal approximation. We describe adiabatic elimination techniques to derive an effective Lindblad master equation up to third order for the atomic degrees of freedom. Numerical simulations show that the spin squeezing scalability loss is correctly reproduced by the reduced open system dynamics, highlighting the role of higher-order contributions. Furthermore, we conjecture an extension beyond leading order of the adiabatic elimination technique to the case of conditional dynamics under quantum non-demolition continuous measurement and fast cavity loss, whose reliability is again confirmed by numerical simulation of the dynamics and the corresponding behavior of spin squeezing as a function of N .
This paper reviews quantum spin squeezing, which characterizes the sensitivity of a state with respect to SU(2) rotations, and is significant for both entanglement detection and high-precision metrology. We first present various definitions of spin squeezing parameters, explain their origin and properties for typical states, and then discuss spin-squeezed states produced with nonlinear twisting Hamiltonians. Afterwards, we explain pairwise correlations and entanglement in spin-squeezed states, as well as the relations between spin squeezing and quantum Fisher information, where the latter plays a central role in quantum metrology. We also review the applications of spin squeezing for detecting quantum chaos and quantum phase transitions, as well as the influence of decoherence on spin squeezing. Finally, we review several experimental realizations of spin squeezing, as well as their corresponding theoretical backgrounds, including: producing spin-squeezed states via particle collisions in Bose-Einstein condensates, transferring photon squeezing to atomic ensembles, and generating spin squeezing via quantum non-demolition measurements.