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Journal of Physics B Atomic Molecular and Optical Physics

Photoionization of a quantum grating formed by a single atom

S F Zhang, Bennaceur Najjari, X. Ma

Published Aug 4, 2021• 2 citations
Publisher

Abstract

Abstract When an atom passes through a macroscopic diffraction grating its wave function acquires a regular space structure and its collision by another particle can be thought of as scattering, of the latter, on a grating composed of a single atom (hereafter termed as ‘quantum-grating’). Photoionization of such a ‘quantum grating’ unveils interference features and in particular a striking difference in the photoelectron and recoil ion spectra which no longer ‘mirroring’ each other as in the case of photoionization of atoms or molecules. We show that complete information about the macroscopic diffraction grating is directly contained in the recoil ion spectra while only partly exhibited in the spectra of the electron.

DOI
10.1088/1361-6455/ac1c37

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Abstract When an atom passes through a macroscopic diffraction grating its wave function acquires a regular space structure and its collision by another particle can be thought of as scattering, of the latter, on a grating composed of a single atom (hereafter termed as ‘quantum-grating’). Photoionization of such a ‘quantum grating’ unveils interference features and in particular a striking difference in the photoelectron and recoil ion spectra which no longer ‘mirroring’ each other as in the case of photoionization of atoms or molecules. We show that complete information about the macroscopic diffraction grating is directly contained in the recoil ion spectra while only partly exhibited in the spectra of the electron.
We consider photo ionization of an atom which, due to passing through a diffraction grating, is prepared in a multi-site state possessing a periodic space structure with alternating maxima and minima. It has been found that this process qualitatively differs from photo ionization of a 'normal' atom. In particular, the spectra of emitted electrons and recoil ions in this process display clear one- and two-particle interference effects. Moreover, there are also striking differences between the momentum distributions of these particles, which no longer mirror each other. The origin of all these features is discussed in detail. It is also shown that the information about the diffraction grating, which is encoded in the multi-site state of the atom, can be fully decoded by exploring the spectra of recoil ions whereas the photo-electron spectra contain this information only partially.
The wave function of an atom passed through a diffraction grating acquires a regular space structure and the interaction of another particle with this atom can be thought of as scattering on a 'quantum grating' composed of a single atom. Probing this 'grating' by collisions with charged projectiles reveals interference effects due to coherent contributions of its 'slits' to the transition amplitude. In particular, the spectra of electrons emitted from the atom in collisions with swift ions exhibit a pronounced interference pattern whose shape can be extremely sensitive to the collision velocity.
The wave function of an atom, which passed through a diffraction grating, is characterized by a regular space structure. Correspondingly, the interaction of another particle with this atom can be viewed as scattering on an ‘atomic quantum grating’ made of just a single atom. Probing this ‘grating’ by collisions with a charged projectile reveals few-body interference phenomena caused by the coherent contributions of its ‘slits’ to the transition amplitude (the superposition principle) and quantum entanglement of the particles involved. In particular, the spectra of electrons emitted from the atom in collisions with swift ions exhibit a pronounced interference pattern whose shape can be extremely sensitive to the collision velocity.
Photoionization of atoms immersed in an environment such as an ultracold gas is investigated. We show that the interference of two ionization pathways, one passing directly to the continuum and one accounting for scattering processes between the photoelectron and a neighboring atom, produces a fine structure in the photoionization cross-section over an energy range less than 1 eV above threshold. This fine structure includes all the details of the corresponding three-body system, e.g. the interatomic distance or the scattering information of the electron-atom subsystem; therefore, photoelectrons produced in a multi-particle environment can be utilized as structural probes. As an illustration, for experimentally relevant parameters, we propose a scheme based on the photoionization of a Rydberg molecule where the low-energy electron-atom phase shifts are extracted from the fine structure spectra using neural networks.
Since de Broglie's work on the wave nature of particles, various optical phenomena have been observed with matter waves of atoms and molecules. However, the analogy between classical and atom/molecule optics is not exact because of different dispersion relations. In addition, according to de Broglie's formula, different combinations of particle mass and velocity can give the same de Broglie wavelength. As a result, even for identical wavelengths, different molecular properties such as electric polarizabilities, Casimir-Polder forces, and dissociation energies modify (and potentially suppress) the resulting matter-wave optical phenomena such as diffraction intensities or interference effects. We report on the universal behavior observed in matter-wave diffraction of He atoms and He2 and D2 molecules from a ruled grating. Clear evidence for emerging beam resonances is observed in the diffraction patterns, which are quantitatively the same for all three particles and only depend on the de Broglie wavelength. A model, combining secondary scattering and quantum reflection, permits us to trace the observed universal behavior back to the peculiar principles of quantum reflection.
The narrowing of electron and ion wave packets in the process of photoionization is investigated, with the electron-ion recoil taken fully into account. Packet localization of this type is directly related to entanglement in the joint quantum state of the electron and ion, and to Einstein-Podolsky-Rosen localization. Experimental observation of such packet-narrowing effects is suggested via coincidence registration by two detectors, with a fixed position of one and varying position of the other. A similar effect, typically with an enhanced degree of entanglement, is shown to occur in the case of photodissociation of molecules.