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An inhibited laser

Tiantian Shi, Duo Pan, Jingbiao Chen

Published Aug 16, 2021• 0 citations
Publisher

Abstract

Abstract Traditional lasers function using resonant cavities, in which the round-trip optical path is exactly equal to an integer multiple of the intracavity wavelengths to constructively enhance the spontaneous emission rate. By taking advantage of the resonant cavity enhancement, the narrowest sub-10-mHz-linewidth laser and a 10^-16-fractional-frequency-stability superradiant active optical clock (AOC) have been achieved. However, never has a laser with atomic spontaneous radiation being destructively inhibited in an anti-resonant cavity where the atomic resonance is exactly between two adjacent cavity resonances been proven. Herein, we present the first demonstration of the inhibited stimulated emission, which is termed an inhibited laser. Compared with traditional superradiant AOCs exhibiting superiority for the high suppression of cavity noise in lasers, the effect of cavity pulling on the inhibited laser's frequency can be further suppressed by a factor of (2F/π)^2. This study of the inhibited laser will guide further development of superradiant AOCs with better stability, and may lead to new searches in the cavity quantum electrodynamics (QED) field.

DOI
10.21203/rs.3.rs-796004/v1

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An inhibited laser

Tiantian Shi, Duo Pan, Jingbiao Chen

Traditional lasers function using resonant cavities, in which the round-trip optical path is exactly equal to an integer multiple of the intracavity wavelengths to constructively enhance the spontaneous emission rate. By taking advantage of the enhancement from the resonant cavity, the narrowest sub-10-mHz-linewidth laser and a $10^{-16}$-fractional-frequency-stability superradiant active optical clock (AOC) have been achieved. However, a laser with atomic spontaneous radiation being destructively inhibited in an anti-resonant cavity, where the atomic resonance is exactly between two adjacent cavity resonances, has not been reported. Herein, we experimentally demonstrate inhibited stimulated emission and termed it an inhibited laser. Compared with traditional superradiant AOCs, which exhibit superiority in terms of the high suppression of cavity noise, the suppression of the cavity-pulling effect of an inhibited laser can be further improved by a factor of $(2F/pi)^2$, i.e., 2.07 in this work, which was improved from 26 to 53 times. This study will guide further development of AOCs with better stability, and thus, it is significant for quantum metrology and may lead to new research in the laser physics and cavity quantum electrodynamics fields.

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Abstract Traditional lasers function using resonant cavities, in which the round-trip optical path is equal to an integer multiple of the intracavity wavelengths to constructively enhance the spontaneous emission rate. Taking advantage of the cavity enhancement effect, the narrowest sub-10-mHz-linewidth laser and a 10−16-fractional-frequency-stability superradiant active optical clock (AOC) have been achieved. However, a laser with atomic spontaneous radiation being destructively inhibited in an anti-resonant cavity, where the atomic resonance is exactly between two adjacent cavity resonances, has not been reported. Herein, we experimentally demonstrate the inhibited laser. Compared with traditional AOCs, which exhibit superiority in terms of the high suppression of cavity noise, the suppression of the cavity-pulling effect of an inhibited laser can be further improved by a factor of $${\left(2{{{{{{{\mathcal{F}}}}}}}}/\pi \right)}^{2}$$ 2F/π2 , which is improved from 26 to 53 times. This study will guide further development of AOCs with better stability, and thus, it is significant for quantum metrology and may lead to new research in the laser physics and cavity quantum electrodynamics fields.

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Abstract Traditional lasers function using resonant cavities, in which the round-trip optical path is exactly equal to an integer multiple of the intracavity wavelengths to constructively enhance the spontaneous emission rate. By taking advantage of the resonant cavity enhancement, the narrowest sub-10-mHz-linewidth laser and a 10^-16-fractional-frequency-stability superradiant active optical clock (AOC) have been achieved. However, never has a laser with atomic spontaneous radiation being destructively inhibited in an anti-resonant cavity where the atomic resonance is exactly between two adjacent cavity resonances been proven. Herein, we present the first demonstration of the inhibited stimulated emission, which is termed an inhibited laser. Compared with traditional superradiant AOCs exhibiting superiority for the high suppression of cavity noise in lasers, the effect of cavity pulling on the inhibited laser's frequency can be further suppressed by a factor of (2F/π)^2. This study of the inhibited laser will guide further development of superradiant AOCs with better stability, and may lead to new searches in the cavity quantum electrodynamics (QED) field.
Traditional lasers function using resonant cavities, in which the round-trip optical path is exactly equal to an integer multiple of the intracavity wavelengths to constructively enhance the spontaneous emission rate. By taking advantage of the enhancement from the resonant cavity, the narrowest sub-10-mHz-linewidth laser and a 10−1610^{-16}10−16-fractional-frequency-stability superradiant active optical clock (AOC) have been achieved. However, a laser with atomic spontaneous radiation being destructively inhibited in an anti-resonant cavity, where the atomic resonance is exactly between two adjacent cavity resonances, has not been reported. Herein, we experimentally demonstrate inhibited stimulated emission and termed it an inhibited laser. Compared with traditional superradiant AOCs, which exhibit superiority in terms of the high suppression of cavity noise, the suppression of the cavity-pulling effect of an inhibited laser can be further improved by a factor of (2F/pi)2(2F/pi)^2(2F/pi)2, i.e., 2.07 in this work, which was improved from 26 to 53 times. This study will guide further development of AOCs with better stability, and thus, it is significant for quantum metrology and may lead to new research in the laser physics and cavity quantum electrodynamics fields.
Abstract Traditional lasers function using resonant cavities, in which the round-trip optical path is equal to an integer multiple of the intracavity wavelengths to constructively enhance the spontaneous emission rate. Taking advantage of the cavity enhancement effect, the narrowest sub-10-mHz-linewidth laser and a 10−16-fractional-frequency-stability superradiant active optical clock (AOC) have been achieved. However, a laser with atomic spontaneous radiation being destructively inhibited in an anti-resonant cavity, where the atomic resonance is exactly between two adjacent cavity resonances, has not been reported. Herein, we experimentally demonstrate the inhibited laser. Compared with traditional AOCs, which exhibit superiority in terms of the high suppression of cavity noise, the suppression of the cavity-pulling effect of an inhibited laser can be further improved by a factor of (2F/π)2{\left(2{{{{{{{\mathcal{F}}}}}}}}/\pi \right)}^{2}(2F/π)2 2F/π2 , which is improved from 26 to 53 times. This study will guide further development of AOCs with better stability, and thus, it is significant for quantum metrology and may lead to new research in the laser physics and cavity quantum electrodynamics fields.
We experimentally demonstrate the collective emission behavior and suppressed cavity-pulling effect of four-level active optical clock with Cesium atoms. Thermal Cesium atoms in a glass cell velocity selective pumped with a 455.5 nm laser operating at 6S1/2_{1/2}1/2​ to 7P3/2_{3/2}3/2​ transition are used as lasing medium. Population inverted Cesium atoms between 7S1/2_{1/2}1/2​ and 6P3/2_{3/2}3/2​ levels are optical weakly coupled by a pair cavity mirrors working at deep bad-cavity regime with a finesse of 4.3, and the ratio between cavity bandwidth and gain bandwidth is approximately 45. With increased 455.5 nm pumping laser intensity, the output power of cesium active optical clock at 1469.9 nm from 7S1/2_{1/2}1/2​ level to 6P3/2_{3/2}3/2​ level shows a threshold and reach a power of 13 μμμW. Active optical clock would dramatically improve the optical clock stability since the lasing frequency does not follow the cavity length variation exactly, but in a form of suppressed cavity pulling effect. In this letter the cavity pulling effect is measured using a Fabry-Perot interferometer (FPI) to be reduced by a factor of 38.2 and 41.4 as the detuning between the 1469.9 nm cavity length of the Cs active optical clock and the Cs 1469.9 nm transition is set to be 140.8 MHz and 281.6 MHz respectively. The mechanism demonstrated here is of great significance for new generation optical clocks and can be applied to improve the stability of best optical clocks by at least two orders of magnitude.
An ideal superradiant laser on an optical clock transition of noninteracting cold atoms is predicted to exhibit an extreme frequency stability and accuracy far below mHz-linewidth. In any concrete setup sufficiently many atoms have to be confined and pumped within a finite cavity mode volume. Using a magic wavelength lattice minimizes light shifts and allows for almost uniform coupling to the cavity mode. Nevertheless, the atoms are subject to dipole-dipole interaction and collective spontaneous decay which compromises the ultimate frequency stability. In the high density limit the Dicke superradiant linewidth enhancement will broaden the laser line and nearest neighbor couplings will induce shifts and fluctuations of the laser frequency. We estimate the magnitude and scaling of these effects by direct numerical simulations of few atom systems for different geometries and densities. For Strontium in a regularly filled magic wavelength configuration atomic interactions induce small laser frequency shifts only and collective spontaneous emission weakly broadens the laser. These interactions generally enhance the laser sensitivity to cavity length fluctuations but for optimally chosen operating conditions can lead to an improved synchronization of the atomic dipoles.
Abstract The atomic clocks, whether operating at optical or microwave region, can be divided into two categories according to their working mode, namely the passive clocks and active clocks. The passive clocks, whose standard frequency is locked to an ultra-narrow atomic spectral line, such as laser cooled Cs beam or lattice trapped Sr atoms, depend on the spontaneous emission line. On the contrary, the active clocks, in which the atoms are used as the gain medium, are based on the stimulated emission radiation, their spectrum can be directly used as the frequency standard. Up to now, the active hydrogen maser has been the most stable microwave atomic clocks. Also, the Sr superradiant active atomic clock is prospects for a millihertz-linewidth laser. Moreover, the optical clocks are expected to surpass the performance of microwave clocks both in stability and uncertainty, since their higher working frequency. The active optical clock has the potential to improve the stability of the best clocks by 2 orders of magnitude. In this work, we introduce the development of active optical clocks, and their types is classified according to the energy-level structure of atoms for stimulated radiation.
Abstract The concept of the active optical clock (AOC) was proposed seventeen years ago by prof. Jingbiao Chen. After early calculations and experiments that demonstrated the advantages of “cavity-pulling suppression” and “narrower linewidth”, the development of AOCs soon became an active competition involving many research groups that proposed schemes based on different atomic species, and different energy-level structures. In this paper, after a brief background introduction, we will mainly focus on the most recent experimental and theoretical progress of AOCs in Peking University. In addition, we give an outlook on AOCs based on cold atoms that can be operated continuously, and report a novel AOC scheme based on diffuse laser cooling that can be operated continuously for the first time, which is proposed and performed by Peking University. The AOC has great promise for applications in quantum metrology, as it can overcome the thermal noise of the reference cavity that limits conventional lasers, making AOC a promising candidate for future atomic optical clocks.