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Wuli

Slowing molecular beams using electrostatic Stark deceleration, magnetostatic Zeeman deceleration and optical Stark deceleration

Hou Shun-Yong, Yaling Yin, Yin Jianping

Published Jan 1, 2017• 0 citations
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We propose a promising scheme to repeatedly decelerate a pulsed molecular beam using a red-detuned quasi-cw semi-Gaussian laser beam (SGB) and an electrostatic storage ring. Using the Monte-Carlo simulation method, we demonstrate that this promising optical Stark decelerator can be used to efficiently slow a pulsed ND 3 molecular beam extracted from a Stark decelerator or a cryogenic reservoir by using a single SGB. The deceleration effect of this scheme on the intensity of the SGB is discussed in detail.

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Abstract We demonstrate the production of cold, slow NH3 molecules from a supersonic NH3 molecular beam using our electrostatic Stark decelerator consisting of 179 slowing stages. By using this long Stark decelerator, a supersonic NH3 molecular beam can be easily decelerated to trappable velocities. Here we present two modes for operating the Stark decelerator to slow the supersonic NH3 molecules. The first is the normal mode, where all 179 stages are used to decelerate molecules, and it allows decelerating the NH3 molecular beam from 333 m/s to 18 m/s, with a final temperature of 29.2 mK. The second is the deceleration-bunch mode, which allows us to decelerate the supersonic NH3 beam from 333 m/s to 24 m/s, with a final temperature of 2.9 mK. It is clear that the second mode promises to produce colder (high-energy-resolution) molecular samples than the normal mode. Three-dimensional Monte Carlo simulations are also performed for the experiments and they show a good agreement with the observed results. The deceleration-bunch operation mode presented here can find applications in the fields of cold collisions, high-resolution spectroscopy, and precision measurements.

Chinese Physics B•May 1, 2019•1 citation
We propose a promising scheme to repeatedly decelerate a pulsed molecular beam using a red-detuned quasi-cw semi-Gaussian laser beam (SGB) and an electrostatic storage ring. Using the Monte-Carlo simulation method, we demonstrate that this promising optical Stark decelerator can be used to efficiently slow a pulsed ND 3 molecular beam extracted from a Stark decelerator or a cryogenic reservoir by using a single SGB. The deceleration effect of this scheme on the intensity of the SGB is discussed in detail.
Abstract We demonstrate the production of cold, slow NH3 molecules from a supersonic NH3 molecular beam using our electrostatic Stark decelerator consisting of 179 slowing stages. By using this long Stark decelerator, a supersonic NH3 molecular beam can be easily decelerated to trappable velocities. Here we present two modes for operating the Stark decelerator to slow the supersonic NH3 molecules. The first is the normal mode, where all 179 stages are used to decelerate molecules, and it allows decelerating the NH3 molecular beam from 333 m/s to 18 m/s, with a final temperature of 29.2 mK. The second is the deceleration-bunch mode, which allows us to decelerate the supersonic NH3 beam from 333 m/s to 24 m/s, with a final temperature of 2.9 mK. It is clear that the second mode promises to produce colder (high-energy-resolution) molecular samples than the normal mode. Three-dimensional Monte Carlo simulations are also performed for the experiments and they show a good agreement with the observed results. The deceleration-bunch operation mode presented here can find applications in the fields of cold collisions, high-resolution spectroscopy, and precision measurements.