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NASA STI/Recon Technical Report N

Coherence in laser excitation

BERNARD SHORE

Published Feb 1, 1981• 0 citations
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We study the statistical properties of a three-level laser where cascade coherent excitation as a two-step process is used as a coherent pump and a laser field is generated on the upper transition. It is shown that the laser intensity fluctuations are suppressed up to 50% below the shot noise limit and that the laser linewidth is reduced below the Schawlow-Townes formula by more than one order of magnitude of the laser intensity. By transforming to the picture dressed by the coherent field on the upper transition, we identify a transfer of the lower coherent excitation to be responsible for the quantum noise reduction. Cascade coherent excitation turns out to be a new way in which one can create a pathway for recycling of active electrons and regularization of laser excitation process. The conditions for the physical realization of the Raman scheme (Ritsch et al 1992 Europhys. Lett. 19 7) as a limiting case is discussed.
In coherent Raman beat experiments a laser field coherently scatters off a material excitation that evolves under the internal Hamiltonian of the system. The Raman signal, which is observed as a beat signal between the test laser and the scattered Raman field, provides information on energy-level splittings and dephasing rates. We propose a modification of this technique, which allows, in contrast to the conventional method, the excitation of coherent Raman beats also in systems with large sublevel splittings and small oscillator strengths. For this purpose, we use a bichromatic laser field to excite the coherent superposition in the medium. We calculate the evolution of the coherence during the laser excitation analytically and discuss its dependence on various experimental parameters. We compare the theoretical results with experimental data from Pr3+{\mathrm{Pr}}^{3+}Pr3+:YAlO3{\mathrm{YAlO}}_{3}YAlO3​.