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Physical Review A

Determination of the mean tunneling flight time in the Büttiker-Landauer oscillating-barrier model as the reflected phase time

Reuven Ianconescu, Eli Pollak

Published Apr 20, 2021• 8 citations
Publisher

Abstract

The oscillating-barrier model was used by B\"uttiker and Landauer to determine a ``traversal time for tunneling.'' The model sets a timescale but is not the physically measured flight time of a wave packet scattered on the oscillating-barrier potential. In this paper we show that the flight time in the limit of a narrow-in-momentum wave packet is given by the reflected phase time associated with the various branches of the scattered particle. This is but another example which establishes that tunneling flight times are a reflection of the Wigner phase times. As such, the oscillating-barrier model does not add any new information about tunneling flight times which has not been elucidated previously using static barrier models.

DOI
10.1103/physreva.103.042215

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The oscillating-barrier model was used by B"uttiker and Landauer to determine a ``traversal time for tunneling.'' The model sets a timescale but is not the physically measured flight time of a wave packet scattered on the oscillating-barrier potential. In this paper we show that the flight time in the limit of a narrow-in-momentum wave packet is given by the reflected phase time associated with the various branches of the scattered particle. This is but another example which establishes that tunneling flight times are a reflection of the Wigner phase times. As such, the oscillating-barrier model does not add any new information about tunneling flight times which has not been elucidated previously using static barrier models.
Using the time parameter in the time-dependent Schr\"odinger equation, we study the time of flight for a particle tunneling through a square barrier potential. Comparing the mean and variance of the energy and the flight time for transmitted and reflected particles, using both density and flux distributions, we find that, when accounting for momentum filtering, the suitably normalized transmitted and reflected distributions are identical in both the density and flux cases. In contrast to previous studies, we demonstrate that these results do not imply a vanishing tunneling time, but rather that the time it takes to tunnel through a square barrier is precisely given by the reflected phase time. For wide barriers, this becomes independent of the barrier width, as predicted independently by MacColl and Hartman. We show that these conclusions can be reached using a variety of arguments, including purely quantum mechanical ones. Analysis of the shapes of the distributions under consideration reveals that wave-packet reshaping is not an explanation for the MacColl-Hartman effect. The results presented here have direct implications for understanding recent experimental results in the study of the barrier crossing of rubidium atoms. The finite width of an incident wave packet significantly ``masks'' the tunneling time, and induces substantial asymmetry between the flight times of transmitted and reflected atoms.
Abstract Different approaches for considering barrier crossing times are analyzed, with special emphasis on recent experiments which attempt to measure what is commonly referred to as the Larmor tunneling time. We show that that these experiments cannot reveal the Larmor time, due to the finite energy width of the incident particles. The Larmor time, which measures changes in spin polarization, is classified together with other measurements such as the Buttiker–Landauer oscillating barrier time as indirect measurements of interaction times of scattered particles. In contrast, we present a direct quantum mechanical measure of a barrier crossing time taken to be the difference between the mean flight time for a particle transmitted through a potential barrier incident on a screen and the time it would take to reach the same screen without the barrier. These metrics are asymptotic, in the sense that they infer a time from a measurement after the scattering event is over, whereas other measures like the dwell time are local. Some time measures are well-defined only for incident states which are monochromatic in energy, others are well-defined also for incident wavepackets whose incident energy width is finite. In this paper we compare the different approaches to conclude that only the flight time can be used to answer the provocative (but ultimately ill-posed) question: how much time does it take to tunnel through a barrier?
Asymptotic time evolution of a wave packet describing a non-relativistic particle incident on a potential barrier is considered, using the Wigner phase-space distribution. The distortion of the trasmitted wave packet is determined by two time-like parameters, given by the energy derivative of the complex transmission amplitude. The result is consistent with various definitions of the tunneling time (e.g. the Büttiker-Landauer time, the complex time and Wigner's phase time). The speed-up effect and the negative dispersion are discussed, and new experimental implications are considered.
The authors analyse tunnelling through time-modulated barriers. The numerical results for the transmitted sideband intensities, obtained with wave-packet simulations, are in quantitative agreement with the analytical results of Buttiker and Landauer (1982, 1985). For opaque barriers the asymmetry of the sideband intensities can be characterized with a single frequency whose inverse Buttiker and Landauer interpret as the traversal time. This simple behaviour does not hold in general, and the authors discuss some of the difficulties one meets in an attempt to generalise the one-parameter description to arbitrary barriers. Furthermore, they examine analytically the transmitted wavefunction in the adiabatic limit, and show that the related density and current involve both the dwell time and the Buttiker time, defined in the context of a Larmor clock. This suggests the possibility that experiments probing different aspects of the transmitted wavefunction may yield different, but complementary, information about the tunnelling process.
How much time does it take for a particle to tunnel through a barrier? This question continues to baffle up to this very day, one of the reasons being the non-existence of an energy–time commutator analogous to the position–momentum commutation relation. Instead of worrying about the definition of an operator one may consider time as a parameter in the time-dependent Schrödinger equation and study the time evolution of a wavepacket appropriately scattered on a potential barrier. Using this approach, one may formally define a tunnelling flight time that may be measured in a time-of-flight experiment. The resulting tunnelling flight time either vanishes or is very small. The implications of this observation with respect to recent hydrogen and helium atom attosecond photoionization experiments are discussed. The vanishing or small flight time does not contradict the finite time measured in Larmor clock experiments, where the tunnelling particle affects an external degree of freedom whose dynamics induced by the tunnelling may be interpreted in terms of a time scale. Flight times are also relevant to quantum reflection where coherences due to resonance scattering are not well accounted for by Wigner's phase time delay.
The tunneling time of a particle through a given barrier is commonly defined in terms of “internal clocks” that effectively measure the interaction time with internal degrees of freedom of the barrier. It is known that this definition of the time scale for tunneling is not unique in the sense that it depends on the clock used to define it. For the case of resonance tunneling, a particular choice that in the limit of a high/broad square barrier yields the original result of Büttiker and Landauer ( Phys. Rev. Lett. 1982, 49, 1739) is correlated to the lifetime of the resonance state. This is illustrated for analytically solvable one-dimensional double barrier models and for a realistic model of electron tunneling through a static water barrier. The latter calculation constitutes a novel application of this concept to a 3-dimensional model, and the observed structure in the energy dependence of the computed traversal time reflects the existence of transient tunneling resonances associated with instantaneous water structures. These models, characterized by the existence of shape resonances in the barrier, make it possible to examine different internal clocks that were proposed for measuring tunneling times in situations where a “clock independent” intrinsic time scale (the resonance lifetime) for the tunneling time exists. It is argued that this time may be used in order to estimate the relative importance of dynamical barrier processes that affect the tunneling probability.