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Deflection of Resonant Multilevel Particles in a Standing Wave Light Field

�. Lindberg

Published Jan 1, 2004• 0 citations
OpenAlex

Abstract

We study the deflection of an atomic system with a resonant multilevel energy structure in classical and quantized wave light fields. We obtain that the shape of the momentum distribution is very sensitive to the energy level structure, whereas its moments are not. Comparison with a two-level case is made. PACS: 32.80, 33.80, 42.50 During the last two decades a remarkable development in mechanically manipulating atomary particles with resonant laser light has taken place (for a review, see for example [1, 2] and references therein). In addition to trapping and cooling of particles, the deflection of particles by a laser beam offers interesting possibilities, for example, to construct atomic interferometers or beam splitters [2-4]. This problem has been studied extensively both theoretically [2, 5, 8] and experimentally [9-12]. The fact that the momentum distribution caused by the scattering is connected to the quantum statistical properties of the scattered light has been known for some time [13]. Recently, one has also realized that the quantum statistics of the light causing the scattering can be important [14]. At low photon numbers, for example, the initial field state strongly influences the resulting momentum distribution. A related effect is that a standing wave and two counterpropagating traveling plane waves of equal emplitudes cause a different diffraction pattern when fields are treated quantum mechanically [15]. Most previous work on the deflection of particles by light fields used two-level atoms. In this paper we study how resonant multilevel systems scatter when they traverse a plane wave. In practical applications, molecules or highly excited atoms have similar energy structures as the models we use in this work. In most cases, we assume that the Raman-Nath regime is valid, i.e., the kinetic energy of the particle can be neglected. However, the field coupling is assumed to be sufficiently strong to make multiple scattering events possible. Our results show that the final momentum distribution of a multi-level system can strongly deviate from that of a two-level atom. It is of interest that the momentum distributions for resonant ladder systems are in general superpositions of few or several distributions similar to that of a two-level system. We also study the expectation values related to the momentum distribution and show that the spread in momentum is remarkably independent of the system considered. The absorption and reabsorption of photons during the scattering process causes the photon distribution to be smoothed out, and for long times a steady state is reached. The cases we studied did not show a creation of sub-Poissonian light. Our model and assumptions are described and discussed in Sect. 1. Some of the general properties of the momentum distribution are discussed in Sect. 2. In Sect. 3 we derive the generating function of the moments of momentum change in Raman-Nath regime. The main part of the paper is contained in Sects. 4 and 5, in which the momentum distribution itself is discussed for several model systems. In Sect. 4 a semiclassical field is assumed and in Sect. 5 a quantum field is used. The effects of the scattering on the field photon statistics are studied in Sect. 6. The final discussion of the results is given in Sect. 7.

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We study the deflection of an atomic system with a resonant multilevel energy structure in classical and quantized wave light fields. We obtain that the shape of the momentum distribution is very sensitive to the energy level structure, whereas its moments are not. Comparison with a two-level case is made. PACS: 32.80, 33.80, 42.50 During the last two decades a remarkable development in mechanically manipulating atomary particles with resonant laser light has taken place (for a review, see for example [1, 2] and references therein). In addition to trapping and cooling of particles, the deflection of particles by a laser beam offers interesting possibilities, for example, to construct atomic interferometers or beam splitters [2-4]. This problem has been studied extensively both theoretically [2, 5, 8] and experimentally [9-12]. The fact that the momentum distribution caused by the scattering is connected to the quantum statistical properties of the scattered light has been known for some time [13]. Recently, one has also realized that the quantum statistics of the light causing the scattering can be important [14]. At low photon numbers, for example, the initial field state strongly influences the resulting momentum distribution. A related effect is that a standing wave and two counterpropagating traveling plane waves of equal emplitudes cause a different diffraction pattern when fields are treated quantum mechanically [15]. Most previous work on the deflection of particles by light fields used two-level atoms. In this paper we study how resonant multilevel systems scatter when they traverse a plane wave. In practical applications, molecules or highly excited atoms have similar energy structures as the models we use in this work. In most cases, we assume that the Raman-Nath regime is valid, i.e., the kinetic energy of the particle can be neglected. However, the field coupling is assumed to be sufficiently strong to make multiple scattering events possible. Our results show that the final momentum distribution of a multi-level system can strongly deviate from that of a two-level atom. It is of interest that the momentum distributions for resonant ladder systems are in general superpositions of few or several distributions similar to that of a two-level system. We also study the expectation values related to the momentum distribution and show that the spread in momentum is remarkably independent of the system considered. The absorption and reabsorption of photons during the scattering process causes the photon distribution to be smoothed out, and for long times a steady state is reached. The cases we studied did not show a creation of sub-Poissonian light. Our model and assumptions are described and discussed in Sect. 1. Some of the general properties of the momentum distribution are discussed in Sect. 2. In Sect. 3 we derive the generating function of the moments of momentum change in Raman-Nath regime. The main part of the paper is contained in Sects. 4 and 5, in which the momentum distribution itself is discussed for several model systems. In Sect. 4 a semiclassical field is assumed and in Sect. 5 a quantum field is used. The effects of the scattering on the field photon statistics are studied in Sect. 6. The final discussion of the results is given in Sect. 7.
We investigate to which extent the quantum nature of light modifies laser-induced atomic beam deflection in a plane standing wave. Our model considers a single two-level atom interacting with a single quantized standing wave mode of the electromagnetic field. We neglect spontaneous emission into other field modes, an approximation valid for short enough times. We find that there is an essential qualitative difference between the cases of a coherent field and a thermal field. For a coherent field, the atomic momentum distribution after interaction has two symmetric peaks on the wings and resembles the semiclassical result of Arimondo et al. [Phys. Rev. A 24, 898 (1981)]. For a thermal field, this distribution has its maximum at p = 0. It is characterized by a constant contribution at p = 0, some sharp interference features, and near-Gaussian wings. The only feature common to both cases is that in the Raman-Nath regime of scattering, the range on transverse momenta grows linearly with time at a rate proportional to 〈 n 〉 , where 〈 n 〉 is the mean number of photons in the field.
We investigate the diffraction of a three-level atom from a "walking" light wave composed of counterpropagating traveling waves of different frequencies. The coupling of the two nondegenerate internal ground states by means of an off-resonant Raman transition resonantly couples the initial external momentum state to only one other momentum state. This happens even in the Raman-Nath regime, where the interaction time is short enough that momentum transfer is not constrained by phase-matching conditions. The final momentum state depends on the initial internal state of the atom and the relative directions of the two traveling waves. By using multiple diffraction regions, this process can be used to coherently split a beam of atoms into two beams that are widely separated in momentum space. This type of beam splitter would be useful in the building an atom interferometer.
We extend the previous theoretical treatment of standing-wave deflection of two-level atoms to include nonresonant excitation, nonorthogonal laser and atomic beams, and excitation duration upper bounded only by atomic relaxation times. Numerically solving equations analogous to those of abruptly initiated multilevel atomic excitation, we find bounds on the maximum deflection fixed by balancing acquired kinetic energy against interaction energy. We find that frequency detuning or nonorthogonal orientation of laser and atomic beams can enhance the deflection and, given sufficiently long interaction time, one can observe deflections at larger discrete angles. We comment on the connection between these Bragg scatterings and multiphoton resonances.
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Atomic beam deflection in a quantum field is studied theoretically for the case of an atom passing through the mode of a resonant optical cavity. Deflection probability is calculated for a coupling rate g of order g/2{pi}=1 MHz, which is experimentally feasible in a short optical cavity. Atomic velocities are taken in the range of 1-10 m/s, which can be reached with current cooling and trapping techniques. We calculate deflection for a coherent state with mean photon number , and for a number state. For the parameters studied, the predicted scattering is in an intermediate regime between Raman-Nath and Bragg, but is closer to the former. We find significant deflection probability even for =1, indicating potential for a high level of sensitivity. We report on our progress in the experimental realization of this system with laser cooled sodium atoms as the atomic medium, and directions for future work are indicated.