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Optics Express

Distinction of electromagnetically induced transparency and Autler-Towners splitting in a Rydberg-involved ladder-type cold atom system

Zhonghua Ji, Yuechun Jiao, Yongmei Xue, Liping Hao, Jianming Zhao, Suotang Jia

Published Mar 22, 2021• 13 citations
Publisher

Abstract

Electromagnetically induced transparency (EIT) and Autler-Townes splitting (ATS) are two similar quantum coherent phenomena but have different mechanisms and applications. Akaike information criteria (AIC), an objective method to discriminate EIT and ATS from an experimental viewpoint, has been employed in a variety of systems. Here we use AIC method to quantitively discriminate a series of spectra of cold atoms in a Rydberg-involved upper-driving ladder-type. The derived weights of EIT and ATS reflect that our spectra change from EIT-ATS intermediate region to ATS-dominated region along Rabi frequency of coupling field increases. We find that there are two factors affecting EIT-ATS weights in a Rydberg-involved three-level system: dephasing rate, induced by the interactions among Rydberg atoms, makes the EIT-ATS crossover move to the direction of low Rabi frequency of coupling field and the experimental noise makes the difference between EIT and ATS weights reduce at elsewhere. Our investigation could provide a meaningful reference for the observations and applications of Rydberg-involved quantum coherent spectroscopy.

DOI
10.1364/oe.417529

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Electromagnetically induced transparency (EIT) and Autler-Townes splitting (ATS) are two similar quantum coherent phenomena but have different mechanisms and applications. Akaike information criteria (AIC), an objective method to discriminate EIT and ATS from an experimental viewpoint, has been employed in a variety of systems. Here we use AIC method to quantitively discriminate a series of spectra of cold atoms in a Rydberg-involved upper-driving ladder-type. The derived weights of EIT and ATS reflect that our spectra change from EIT-ATS intermediate region to ATS-dominated region along Rabi frequency of coupling field increases. We find that there are two factors affecting EIT-ATS weights in a Rydberg-involved three-level system: dephasing rate, induced by the interactions among Rydberg atoms, makes the EIT-ATS crossover move to the direction of low Rabi frequency of coupling field and the experimental noise makes the difference between EIT and ATS weights reduce at elsewhere. Our investigation could provide a meaningful reference for the observations and applications of Rydberg-involved quantum coherent spectroscopy.
Electromagnetically induced transparency (EIT) and Autler–Townes splitting (ATS) are two similar yet distinct phenomena that modify the transmission of a weak probe field through an absorption medium in the presence of a coupling field, featured in a variety of three-level atomic systems. In many applications it is important to distinguish EIT from ATS splitting. We present EIT and ATS spectra in a three-level cascade system, involving cold cesium atoms in the Rydberg state. The EIT linewidth, γ EIT , defined as the full width at half maximum of the transparency window, and the ATS splitting, γ ATS , defined as the peak-to-peak distance between AT absorption peaks, are used to delineate the EIT and ATS regimes and to characterize the transition between the regimes. In the cold-atom medium, in the weak-coupler (EIT) regime γ EIT ≈ A + B ( + , where Ω c and Ω p are the coupler and probe Rabi frequencies, Γ eg is the spontaneous decay rate of the intermediate 6P 3/2 level, and parameters A and B that depend on the laser linewidth. We explore the transition into the strong-coupler (ATS) regime, which is characterized by the relation γ ATS ≈ Ω c . The experiments are in agreement with numerical solutions of the Master equation. Our analysis accounts for non-ideal conditions that exist in typical realizations of Rydberg-EIT, including laser-frequency jitter, Doppler mismatch of the utilized two-color Rydberg EIT system, and strong probe fields. The obtained criteria to distinguish cold-atom EIT from ATS are readily accessible and applicable in practical implementations.
Autler-Townes splitting (ATS) and electromagnetically induced transparency (EIT) both yield transparency in an absorption profile, but only EIT yields strong transparency for a weak pump field due to Fano interference. Empirically discriminating EIT from ATS is important but so far has been subjective. We introduce an objective method, based on Akaike's information criterion, to test ATS vs EIT from experimental data for three-level atomic systems and determine which pertains. We apply our method to a recently reported induced-transparency experiment in superconducting-circuit quantum electrodynamics.
Summary form only given. If in general the transparency of an initially absorbing medium for a probe field is increased by the presence of a control field on an adjacent transition, two very different processes can be invoked to explain it. One of them is a quantum Fano interference between two paths in the three-level system, which occurs even at low control intensity and gives rise to electromagnetically-induced transparency (EIT), the other one is the appearance of two dressed states in the excited level at higher control intensity, corresponding to the Autler-Townes splitting (ATS). This distinction is particularly critical for instance for the implementation of slow light or optical quantum memories. In a recent paper, P. M. Anisimov, J. P. Dowling and B. C. Sanders proposed a quantitative test to objectively discerning ATS from EIT. We experimentally investigated this test with cold atoms and demonstrated that it is very sensitive to the specific properties of the medium. In this study, we use an ensemble of cold Cesium atoms trapped in a MOT, interacting with light via a Λ-type scheme on the D2 line. Absorption profiles are obtained for various values of the control Rabi frequency Ω between 0.1Γ and 4Γ, where Γ is the natural linewidth.
Electromagnetically induced transparency is a quantum interference (QI) effect in a coherent system, in which the similar but distinct effect of Autler–Townes splitting (ATS) without QI also happens concurrently. The Akaike information criterion (AIC) has been proven to be an efficient and objective method to discern them by evaluating their relative AIC weights for different Rabi frequencies of the coupling field. Here, we investigate in detail the influence of the dephasing effect on the AIC weights of QI and ATS, and present the transition among destructive QI, constructive QI, and ATS without QI by controlling the dephasing rates. By comparing the effects of different dephasing rates on the QI and ATS weights, we show that the field-phase-diffusion dephasing provides more feasibility than the atom-collision dephasing in control of QI and ATS. Therefore, precise and selective dephasing engineering can be realized by manipulating the linewidths and phase correlation of the fields. This indicates that various collision-related effects (e.g., collision-dephasing-induced coherences) can be experimentally studied using more controllable field-phase-diffusion dephasing instead of buffer-gas-controlling collision dephasing.
We propose a general theoretical scheme to investigate the crossover from electromagnetically induced transparency (EIT) to Autler–Townes splitting (ATS) in open ladder-type atomic and molecular systems with Doppler broadening. We show that when the wavenumber ratio kc/kp≈−1, EIT, ATS, and EIT-ATS crossover exist for both ladder-I and ladder-II systems, where kc (kp) is the wavenumber of control (probe) field. Furthermore, when kc/kp is far from −1, EIT can occur, but ATS is destroyed if the upper state of the ladder-I system is a Rydberg state. In addition, ATS exists but EIT is not possible if the control field used to couple the two lower states of the ladder-II system is a microwave field. The theoretical scheme developed here can be applied to atoms, molecules, and other systems (including Na2 molecules, and Rydberg atoms), and the results obtained may have practical applications in optical information processing and transformation.