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Liouvillian spectral collapse in Scully-Lamb lasing: Non-equilibrium second-order phase transition with or without $U(1)$ symmetry breaking

Fabrizio Minganti, Ievgen I. Arkhipov, Adam Miranowicz, Franco Nori

Published Mar 9, 2021• 2 citations
OpenAlex

Abstract

The paradigm of second-order phase transition and symmetry breaking for thermal and quantum systems is a pillar of modern physics that has been fruitfully applied to out-of-equilibrium open quantum systems. Despite the non-equilibrium nature of lasing, the laser threshold was compared with thermal phase transitions systems more than forty years ago. For instance, the Landau theory -- based on thermodynamical consideration -- has been used to characterize the Scully-Lamb laser model (SLLM), describing a single-mode laser without saturable absorbers. Accordingly, the laser threshold is a second-order phase transition, associated with a spontaneous symmetry breaking (SSB) of the $U(1)$ symmetry of the model. To capture a genuine non-equilibrium, quantum, and dissipative phase transition of the SLLM, here we employ a Liouvillian superoperator formalism derived from a Lindblad master equation. Our results confirm that the $U(1)$ SSB can occur at the lasing threshold but, in contrast to the Landau theory and semiclassical approximation, they signal that the SLLM fundamental transition is a different phenomenon, which we call Liouvillian spectral collapse; that is, the emergence of diabolic points of infinite degeneracy. By considering a generalized SLLM with additional dephasing, we witness a second-order phase transition, with a Liouvillian spectral collapse, but in the absence of symmetry breaking. This demonstrates the difference between the Liouvillian spectral collapse and a standard second-order phase transition with symmetry breaking. We characterize the new phenomena associated with the spectral collapse, such as the onset of a rather unusual multistability enabled (and not suppressed) by the very presence of fluctuations. This multistability, characterizing the dissipative and quantum origin of lasing, can be experimentally revealed by the presence of a dynamical hysteresis.

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Liouvillian spectral collapse in Scully-Lamb lasing: Non-equilibrium second-order phase transition with or without U(1)U(1)U(1) symmetry breaking
The paradigm of second-order phase transition and symmetry breaking for thermal and quantum systems is a pillar of modern physics that has been fruitfully applied to out-of-equilibrium open quantum systems. Despite the non-equilibrium nature of lasing, the laser threshold was compared with thermal phase transitions systems more than forty years ago. For instance, the Landau theory -- based on thermodynamical consideration -- has been used to characterize the Scully-Lamb laser model (SLLM), describing a single-mode laser without saturable absorbers. Accordingly, the laser threshold is a second-order phase transition, associated with a spontaneous symmetry breaking (SSB) of the U(1)U(1)U(1) symmetry of the model. To capture a genuine non-equilibrium, quantum, and dissipative phase transition of the SLLM, here we employ a Liouvillian superoperator formalism derived from a Lindblad master equation. Our results confirm that the U(1)U(1)U(1) SSB can occur at the lasing threshold but, in contrast to the Landau theory and semiclassical approximation, they signal that the SLLM fundamental transition is a different phenomenon, which we call Liouvillian spectral collapse; that is, the emergence of diabolic points of infinite degeneracy. By considering a generalized SLLM with additional dephasing, we witness a second-order phase transition, with a Liouvillian spectral collapse, but in the absence of symmetry breaking. This demonstrates the difference between the Liouvillian spectral collapse and a standard second-order phase transition with symmetry breaking. We characterize the new phenomena associated with the spectral collapse, such as the onset of a rather unusual multistability enabled (and not suppressed) by the very presence of fluctuations. This multistability, characterizing the dissipative and quantum origin of lasing, can be experimentally revealed by the presence of a dynamical hysteresis.
Phase transitions of thermal systems and the laser threshold were first connected more than forty years ago. Despite the nonequilibrium nature of the laser, the Landau theory of thermal phase transitions, applied directly to the Scully-Lamb laser model (SLLM), indicates that the laser threshold is a second-order phase transition, associated with a U(1) spontaneous symmetry breaking (SSB). To capture the genuine nonequilibrium phase transition of the SLLM (i.e., a single-mode laser without a saturable absorber), here we employ a quantum theory of dissipative phase transitions. Our results confirm that the U(1) SSB can occur at the lasing threshold but, in contrast to the Landau theory and semiclassical approximation, they signal that the SLLM ``fundamental'' transition is a different phenomenon, which we call Liouvillian spectral collapse; that is, the emergence of diabolic points of infinite degeneracy. By considering a generalized SLLM with additional dephasing, we witness a second-order phase transition, with a Liouvillian spectral collapse, but in the absence of symmetry breaking. Most surprisingly, the phase transition corresponds to the emergence of dynamical multistability even without SSB. Normally, bistability is suppressed by quantum fluctuations, while in this case, the very presence of quantum fluctuations enables bistability. This rather anomalous bistability, characterizing the truly dissipative and quantum origin of lasing, can be an experimental signature of our predictions, and we show that it is associated with an emergent dynamical hysteresis.
A state of an open quantum system is described by a density matrix, whose dynamics is governed by a Liouvillian superoperator. Within a general framework, we explore fundamental properties of both first-order dissipative phase transitions and second-order dissipative phase transitions associated with a symmetry breaking. In the critical region, we determine the general form of the steady-state density matrix and of the Liouvillian eigenmatrix whose eigenvalue defines the Liouvillian spectral gap. We illustrate our exact results by studying some paradigmatic quantum optical models exhibiting critical behavior.
Nanocavity lasers are commonly characterized by the spontaneous coupling coefficient β that represents the fraction of photons emitted into the lasing mode. While β is conventionally discussed in semiconductor lasers where the photon lifetime is much shorter than the carrier lifetime (class-B lasers), little is known about β in atomic lasers where the photon lifetime is much longer than the other lifetimes and only the photon degree of freedom exists (class-A lasers). We investigate the impact of the spontaneous coupling coefficient β on lasing properties in the class-A limit by extending the well-known Scully–Lamb master equation. We demonstrate that in the class-A limit all the photon statistics are uniquely characterized by β and that the laser phase transition-like analogy becomes transparent. In fact, β perfectly represents the “system size” in phase transition. Finally, we investigate the laser-phase transition analogy from the standpoint of a quantum dissipative system. Calculating a Liouvillian gap, we clarify the relation between β and the continuous phase symmetry breaking.
Usually, when investigating exceptional points (EPs) of an open Markovian bosonic system, one deals with spectral degeneracies of a non-Hermitian Hamiltonian (NHH), which can correctly describe the system dynamics only in the semiclassical regime. A recently proposed quantum Liouvillian framework [Minganti et al., Phys. Rev. A 100, 062131 (2019)] enables the complete determination of the dynamical properties of such systems and their EPs (referred to as Liouvillian EPs, or LEPs) in the quantum regime by taking into account the effects of quantum jumps, which are ignored in the NHH formalism. Moreover, the symmetry and eigenfrequency spectrum of the NHH become a part of much larger Liouvillian eigenspace. As such, the EPs of an NHH form a subspace of the LEPs. Here we show that once an NHH of a dissipative linear bosonic system exhibits an EP of a certain finite order nnn, it immediately implies that the corresponding LEP can become of any higher order $m\ensuremath{\ge}n$ defined in the infinite Hilbert space. These higher-order LEPs can be identified by the coherence and spectral functions at the steady state. The coherence functions can offer a convenient tool to probe extreme system sensitivity to external perturbations in the vicinity of higher-order LEPs. As an example, we study a linear bosonic system of a bimodal cavity with incoherent mode coupling to reveal its higher-order LEPs; particularly, of second and third order via first- and second-order coherence functions, respectively. Accordingly, these LEPs can be additionally revealed by squared and cubic Lorentzian spectral lineshapes in the power and intensity-fluctuation spectra. Moreover, we demonstrate that these EPs can also be associated with spontaneous parity-time (PT\mathcal{PT}PT) and anti-PT\mathcal{PT}PT-symmetry breaking in the system studied. These symmetries can be switched in the output fields (the so-called supermodes) of an additional linear coupler with a properly chosen coupling strength. Thus, we show that the initial loss-loss dynamics for the supermodes can be equivalent to the balanced gain-loss evolution.
After reviewing the interpretation of laser operation as a nonequilibrium Bose-Einstein condensation phase transition, we illustrate the novel features arising from the nonequilibrium nature of photon and polariton Bose-Einstein condensates recently observed in experiments. We then propose a quantitative criterion to experimentally assess the equilibrium versus nonequilibrium nature of a specific condensation process, based on fluctuation-dissipation relations. The power of this criterion is illustrated on two models which show very different behaviors. Historical and Conceptual Introduction The first introduction of concepts of nonequilibrium statistical mechanics into the realm of optics dates back to the early 1970s with pioneering works by Graham and Haken [1] and by DeGiorgio and Scully [2], who proposed a very insightful interpretation of the laser threshold in terms of a spontaneous breaking of the U( 1 ) symmetry associated with the phase of the emitted light. Similar to what happens to the order parameter at a second-order phase transition, such an optical phase is randomly chosen every time the device is switched on and remains constant for macroscopic times. Moreover, a long-range spatial order is established, as light emitted by a laser device above threshold is phase-coherent on macroscopic distances. While textbooks typically discuss this interpretation of laser operation in terms of a phase transition for the simplest case of a single-mode laser cavity, rigorously speaking this is valid only in spatially infinite systems. In fact, only in this case one can observe nonanalytic behaviors of the physical quantities at the transition point. In particular, the long-range order is typically assessed by looking at the long-distance behavior of the correlation function of the order parameter, which, for a laser, corresponds to the first-order spatial coherence of the emitted electric field, the spontaneous symmetry breaking is signaled by this quantity becoming nonzero (see Chapter 5). The average is taken on the stationary density matrix of the system. In order to be able to probe this long-distance behavior, experimental studies need devices with a spatially extended active region.
We present an exact solution of the quantum laser master equation using generating functions and confluent Heun equations. By reformulating the evolution of both diagonal and off-diagonal elements of the reduced density matrix, we derive closed-form expressions for the generating functions and identify the full spectrum of decay rates from a two-point connection problem for the confluent Heun equation. This method captures both transient dynamics and steady-state properties without truncation. In the thermodynamic limit of vanishing saturation, the spectrum separates into two analytically tractable eigenvalue families; their intersections mark exceptional points, reflecting nontrivial structure in the system's Liouvillian dynamics. At the lasing threshold, we observe a Liouvillian spectral collapse, signaling a nonequilibrium phase transition. Our results provide a unified, nonperturbative description of laser dynamics across different regimes.