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Annual Meeting Optical Society of America

Bistability and mode-mode competition in a homogeneously broadened CO2 laser

Jorge R. Tredicce, Antonella Poggi, Gian Piero Puccioni, Gian Luca Lippi, F. T. Arecchi, W. Gadomski

Published Jan 1, 1985• 0 citations
Publisher

Abstract

Unstable and bistable behavior has been predicted recently in multimode homogeneously broadened lasers as a function of the detuning between the cavity and the atomic frequencies. As an example of a device for which most required physical conditions for the appearance of this instability are satisfied, we have analyzed the behavior of a low-pressure (10–20 Torr) CO2 laser. The operating parameters (relaxation rates for the population inversion, 104s−1, and for the polarization, 108s−1) restrict the accessible range of theoretically expected phenomena to a stable intensity output without evidence of stable self-pulsing. However, mode–mode competition is responsible for bistability in both the intensity and the operating frequency on varying the detuning parameter. This behavior is confirmed by additional observations of the transient that accompanies the jump between the two stable branches. We have also studied the effect of varying the cavity losses and discovered bistability also in the vicinity of the threshold for laser action. This kind of behavior is not predicted by the plane wave Maxwell-Bloch equations but can be explained in terms of a radial gain profile. Both effects—mode–mode competition and transverse—lead to a variety of bistable behaviors depending on gas pressure and discharge current.

DOI
10.1364/oam.1985.fg2

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Physical Review A•Sep 1, 1985•84 citations
Unstable and bistable behavior has been predicted recently in multimode homogeneously broadened lasers as a function of the detuning between the cavity and the atomic frequencies. As an example of a device for which most required physical conditions for the appearance of this instability are satisfied, we have analyzed the behavior of a low-pressure (10–20 Torr) CO2 laser. The operating parameters (relaxation rates for the population inversion, 104s−1, and for the polarization, 108s−1) restrict the accessible range of theoretically expected phenomena to a stable intensity output without evidence of stable self-pulsing. However, mode–mode competition is responsible for bistability in both the intensity and the operating frequency on varying the detuning parameter. This behavior is confirmed by additional observations of the transient that accompanies the jump between the two stable branches. We have also studied the effect of varying the cavity losses and discovered bistability also in the vicinity of the threshold for laser action. This kind of behavior is not predicted by the plane wave Maxwell-Bloch equations but can be explained in terms of a radial gain profile. Both effects—mode–mode competition and transverse—lead to a variety of bistable behaviors depending on gas pressure and discharge current.
Homogeneously broadened lasers are considered as intrinsically single mode monostable devices [1] where intensity and frequency are defined by the cavity mode that lies nearest to the center of the atomic line. Here we show theoretically and experimentally that this heuristic picture falls when the interaction between different cavity modes becomes relevant. In fact, for sufficiently high detuning between cavity and atomic resonance frequencies (δAC), self pulsing of the laser arise from the simultaneous operation in two modes (phase instability) even if it is operating near threshold (C ⪯ 1) and in the so-called good cavity limit (k ≪ γ⊥, γ‖). Using parameter values which are typical of many solid state and molecular gas lasers (γ‖, k ≪ γ⊥), the theory predicts a bistable behavior in both the output intensity and frequency, as δAC is varied (Fig. 1). These theoretical results have been confirmed by experiments carried out on a CO2 laser where the distance between modes was controlled by changing the losses inside the cavity and the detuning δAC was varied by a fine tuning of the distance between mirrors. The output intensity versus δAC is shown in Fig. 2 for two different values of losses and gas pressure. Direct comparison between Fig. 2b) and Fig. 1 shows a good qualitative agreement. Measurements of the transients during the jump of Fig.2b) confirmed the mode-mode competition interpretation.
Detailed analysis of the steady-state and dynamical unstable behavior of single-mode, homogeneously broadened Raman lasers is presented. Bistable features of the Raman emission and its operating conditions are determined from steady-state analysis. Parametrization of the dynamical behavior shows instabilities to exist over a broad range of operation conditions and for broad cavity detuning to the low-frequency side of the gain center where the bistable emission also prevails. Notably, period-doubling routes to chaos and sustained oscillatory behavior in both intensity and phase are found to occur for both good and bad cavity conditions, the dynamics of the phase revealing additional temporal features to that of intensity.
We provide a comprehensive analysis of the standard model of the bidirectional ring laser in which only one mode can be supported in each direction and in the limit that the polarization can be eliminated adiabatically. The interaction between the two counterpropagating modes can be derived and it is most naturally viewed as a coupling between them via scattering from a spatial grating formed in the population inversion. If the grating is a sufficiently small modulation of the spatial average of the population inversion, it can be approximated by a sinusoidal function. A systematic derivation of the model with only a sinusoidal grating for the homogeneously broadened case is presented that reveals and corrects errors in several previously published analyses. The stability of the steady-state solution is analyzed. The bidirectional steady-state solution is unstable and the unidirectional steady-state solutions may be stable or unstable depending on the parameters. The well-established result of bistability between the two modes when the cavity is tuned to resonance is recovered, a result that persists, in part, even when the losses between the two modes are different.With detuning, the unidirectional steady-state solutions can be destabilized, creating regions in the parameter space where only time-dependent solutions are found. For parameters characteristic of solid-state or molecular gas lasers, the instability can occur for very small detunings and even very close to the lasing threshold. Asymptotic limits of the instability boundaries for these parameters are presented. Additional results are derived formally for inhomogeneous broadening with a Lorentzian line shape and for arbitrary inhomogeneous linewidths. Explicit analytic results are presented in the limits of very small and very large inhomogeneous linewidths compared with the homogeneous linewidth. Time-dependent solutions in the homogeneously broadened case for relaxation rates appropriate to CO2{\mathrm{CO}}_{2}CO2​ lasers show that there are broad regions in the parameter space of gain and detuning for which the behavior is dynamically chaotic in the form of nearly ``square-wave'' alternation between the counterpropagating modes of the laser with irregular switching times. In other regions of that parameter space we find more irregular pulsations and pulse alternations. Regions of periodic pulsations also have been found.
We review and extend the theory of instabilities in absorptive optical bistability for ring cavities containing homogeneously broadened two-level media. The instabilities occur in the high-transmission branch and result in either a precipitation to the low-transmission branch or in pulsed multimode operation. Two numerical approaches are used to predict operation away from the simple mean-field limit. First, an iterative method is used to solve the general field eigenvalue equation for cavity modes with frequencies displaced from the input frequency. This work shows that the instability region decreases in size as the mirror transmission increases. These calculations are confirmed by the second numerical technique, consisting of direct integrations of the coupled Maxwell-Bloch equations. This second approach also provides time histories of the instability evolutions, and divides the instability range into a precipitation regime and a self-pulsing regime. The results are discussed in terms of first- and second-order phase transitions, and agree with the analytical results obtained within the dressed-mode description of optical bistability. They show that when the incident field is adiabatically decreased along the high-transmission branch, the spiking behavior always appears abruptly. By further decreasing the incident intensity, the self-pulsing disappears either continuously if the system remains in the high-transmission branch, or discontinuously if the system precipitates to the low-transmission branch. Connection is made with induced probe gain known in the saturation spectroscopy of absorbers (uninverted media), in which population pulsations transfer energy from a saturating wave to the probe waves. The very close relationship with multimode operation in homogeneously broadened unidirectional ring lasers is also established.
We compare theoretical predictions and experimental data for the multimode instability of optical bistability, which arises from the coherent dynamics of a system of two-level molecules contained in an optical cavity and driven by an external stationary laser field. Considerable insight into this phenomenon is provided by two ``rules of thumb'' that govern the behavior of the self-pulsing frequency, and establish its relation with the Rabi frequency of the intracavity field. We describe in detail the experimental apparatus and the main features of the experimental findings. The theoretical results are based on the Maxwell-Bloch equations for a ring cavity in the plane-wave approximation. Despite the crudeness of this model, the numerical data display a satisfactory qualitative agreement with the experimental results. Additional period-doubling and chaotic phenomena, predicted by the theory and not observed in the experiment, are presumably washed out by the longitudinal and radial variation of the electric field in the cavity.
This paper contains a description of the behavior of a multimode unidirectional ring laser with a homogeneously broadened active medium. Our formulation is based on the conventional Maxwell-Bloch (MB) equations, but is distinguished from other treatments by the inclusion of a finite mirror reflectivity and an arbitrary value of the gain parameter. We review the steady-state behavior of the system and analyze the longitudinal profile of the field and of the atomic variables. With an appropriate transformation of variables, we transform the boundary conditions of the ring cavity into standard periodicity type, even in the presence of a finite reflectivity, and derive an infinite hierarchy of coupled mode equations. We analyze exactly the linear stability of the system, and investigate the dependence of the instability domain on the reflectivity and gain parameters. A numerical study of the full MB equations for a parameter range of the type explored in the recent experiments by Hillman et al. [Phys. Rev. Lett. 52, 1605 (1984)] reveals similarities, but also considerable differences between the results of the theory and the main experimental signatures of their instability. However, the injection of numerical noise shows the presence of numerous coexisting basins of attraction which are likely to play a significant role in the dynamics of a noisy laser.