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Physical Review A

Multimode instability in optical bistability

Bernard Ségard, B. Macke, L. A. Lugiato, Franco Prati, Massimo Brambilla

Published Jan 1, 1989• 49 citations
Publisher

Abstract

We compare theoretical predictions and experimental data for the multimode instability of optical bistability, which arises from the coherent dynamics of a system of two-level molecules contained in an optical cavity and driven by an external stationary laser field. Considerable insight into this phenomenon is provided by two ``rules of thumb'' that govern the behavior of the self-pulsing frequency, and establish its relation with the Rabi frequency of the intracavity field. We describe in detail the experimental apparatus and the main features of the experimental findings. The theoretical results are based on the Maxwell-Bloch equations for a ring cavity in the plane-wave approximation. Despite the crudeness of this model, the numerical data display a satisfactory qualitative agreement with the experimental results. Additional period-doubling and chaotic phenomena, predicted by the theory and not observed in the experiment, are presumably washed out by the longitudinal and radial variation of the electric field in the cavity.

DOI
10.1103/physreva.39.703

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We compare theoretical predictions and experimental data for the multimode instability of optical bistability, which arises from the coherent dynamics of a system of two-level molecules contained in an optical cavity and driven by an external stationary laser field. Considerable insight into this phenomenon is provided by two ``rules of thumb'' that govern the behavior of the self-pulsing frequency, and establish its relation with the Rabi frequency of the intracavity field. We describe in detail the experimental apparatus and the main features of the experimental findings. The theoretical results are based on the Maxwell-Bloch equations for a ring cavity in the plane-wave approximation. Despite the crudeness of this model, the numerical data display a satisfactory qualitative agreement with the experimental results. Additional period-doubling and chaotic phenomena, predicted by the theory and not observed in the experiment, are presumably washed out by the longitudinal and radial variation of the electric field in the cavity.
We have recently observed a sinewave self-pulsing in the beam transmitted by a passive cavity containing 2-level molecules, driven by a continuous wave. In this experiment made at a wavelength λ ≅ 3.5 mm, the intracavity Rabi frequency is comparable to the free spectral range ( 830 kHz ) of the very long cavity used (l =182 m) {1} and much larger than the collisional linewidth (≅ 25 kHz) .The medium is then strongly saturated by the driving field ( saturation parameter > 1000) so that its absorption , heavy in the linear regime (αl > 100), is in fact quite moderate. We claim that the self-pulsing observed in these conditions is the first experimental evidence of the multimode instability, predicted a long time ago by Bonifacio and Lugiato {2} but not yet observed. This instability is the multimode counterpart of the single mode instability, recently observed by Orozco et al {3}.
This paper gives a detailed description of the plane-wave Gaussian models of optical bistability and of the experimental investigations of the single-mode instability induced on a beam of sodium atoms in a cavity by an external driving field. Our goal is to provide a careful comparison of the theoretical and experimental results. We focus on the shape of the instability domain, the nature and behavior of the spontaneous output oscillations produced by the instability, and their frequency dependence on the control parameters. We carry out this comparison using both the plane-wave and Gaussian models. Our analysis shows that the latter is in good quantitative agreement with the experimental results. We investigate in detail the main assumption of the Gaussian model, namely, that the internal cavity field retains the same radial profile as the input field.
We review and extend the theory of instabilities in absorptive optical bistability for ring cavities containing homogeneously broadened two-level media. The instabilities occur in the high-transmission branch and result in either a precipitation to the low-transmission branch or in pulsed multimode operation. Two numerical approaches are used to predict operation away from the simple mean-field limit. First, an iterative method is used to solve the general field eigenvalue equation for cavity modes with frequencies displaced from the input frequency. This work shows that the instability region decreases in size as the mirror transmission increases. These calculations are confirmed by the second numerical technique, consisting of direct integrations of the coupled Maxwell-Bloch equations. This second approach also provides time histories of the instability evolutions, and divides the instability range into a precipitation regime and a self-pulsing regime. The results are discussed in terms of first- and second-order phase transitions, and agree with the analytical results obtained within the dressed-mode description of optical bistability. They show that when the incident field is adiabatically decreased along the high-transmission branch, the spiking behavior always appears abruptly. By further decreasing the incident intensity, the self-pulsing disappears either continuously if the system remains in the high-transmission branch, or discontinuously if the system precipitates to the low-transmission branch. Connection is made with induced probe gain known in the saturation spectroscopy of absorbers (uninverted media), in which population pulsations transfer energy from a saturating wave to the probe waves. The very close relationship with multimode operation in homogeneously broadened unidirectional ring lasers is also established.
Although the discovery of oscillatory instabilities (both single-mode and multimode) in free-running lasers was achieved in the 1960s, investigations on oscillatory instabilities in optical bistability did not take place until the 1970s and 1980s. The first section of this chapter does not deal with oscillatory instabilities, but instead concerns an interesting dynamical phenomenon in optical bistability that arises when the input field approaches a boundary of the bistable domain, and is called critical slowing down . This has been investigated both theoretically and experimentally. The remainder of this chapter is entirely devoted to oscillatory instabilities, following a historical order. With an inverse approach with respect to the laser case, we discuss multimode instabilities first. In Section 24.2.1 we start with the description of the instability which arises under exactly resonant conditions. While this is the counterpart in optical bistability of the resonant multimode laser instability discussed in Section 22.5, a striking difference from the laser case is that in the passive configuration there is no corresponding single-mode instability. This difference disappears, however, when we consider the generalization of the multimode instability of optical bistability to the detuned configuration. Finally we show that in the detuned case it has been possible to achieve a convincing experimental observation of the multimode instability in a long microwave cavity. After some relevant miscellaneous considerations in Section 24.2.2, in Section 24.2.3 we address the subject of the multimode Ikeda instability which leads to period doubling and chaos and aroused a lot of interest in optical chaos. We emphasize also the intrinsic connections with the standard multimode instability discussed in Section 24.2.1, showing, in particular, that the Ikeda instability requires conditions far from the low-transmission limit, i.e. that ∝L is not small. In Section 24.3 we discuss single-mode instabilities in optical bistability. In Section 24.3.1 we illustrate a configuration for the single-mode instability that includes also the Gaussian shape of the electric field in the beam section, and leads to periodic, close-to-sinusoidal self-pulsations.