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Optical and Quantum Sensing and Precision Metrology

Spin-squeezing by prediction and retrodiction measurements: beyond the Heisenberg uncertainty relation

Han Bao, Shenchao Jin, Junlei Duan, Xingda Lu, Pengxiong Li, Weizhi Qu, Mingfeng Wang, Irina V. Novikova, Eugeniy E. Mikhailov, Kaifeng Zhao, Suotang Jia, Klaus Mølmer, Heng Shen, Yanhong Xiao

Published Mar 4, 2021• 0 citations
Publisher

Abstract

If one has access to information about a quantum system both before and after a measurement, the usual remit of Heisenberg uncertainty relation (HUR) does not apply. Here, we theoretically and experimentally demonstrate that, in such a scenario, one can retrodict position and momentum measurements without being limited by HUR. The experiment uses a large ensemble of 10^11 atoms in a macroscopic vapor cell, and the results may be applicable for quantum state estimation and sensing, especially for sensitive magnetometers equally capable of measuring the amplitude and phase of an RF magnetic field both below the standard quantum limit.

DOI
10.1117/12.2586729

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If one has access to information about a quantum system both before and after a measurement, the usual remit of Heisenberg uncertainty relation (HUR) does not apply. Here, we theoretically and experimentally demonstrate that, in such a scenario, one can retrodict position and momentum measurements without being limited by HUR. The experiment uses a large ensemble of 10^11 atoms in a macroscopic vapor cell, and the results may be applicable for quantum state estimation and sensing, especially for sensitive magnetometers equally capable of measuring the amplitude and phase of an RF magnetic field both below the standard quantum limit.
Abstract In quantum mechanics, the Heisenberg uncertainty relation presents an ultimate limit to the precision by which one can predict the outcome of position and momentum measurements on a particle. Heisenberg explicitly stated this relation for the prediction of “hypothetical future measurements”, and it does not describe the situation where knowledge is available about the system both earlier and later than the time of the measurement. Here, we study what happens under such circumstances with an atomic ensemble containing 1011 rubidium atoms, initiated nearly in the ground state in the presence of a magnetic field. The collective spin observables of the atoms are then well described by canonical position and momentum observables, x^A{\hat{x}}_{\text{A}}x^A​ x ̂ A and p^A{\hat{p}}_{\text{A}}p^​A​ p ̂ A that satisfy [x^A,p^A]=iℏ[{\hat{x}}_{\text{A}}, {\hat{p}}_{\text{A}}]=i\hslash[x^A​,p^​A​]=iℏ [ x ̂ A , p ̂ A ] = i ℏ . Quantum non-demolition measurements of p^A{\hat{p}}_{\text{A}}p^​A​ p ̂ A before and of x^A{\hat{x}}_{\text{A}}x^A​ x ̂ A after time t allow precise estimates of both observables at time t. By means of the past quantum state formalism, we demonstrate that outcomes of measurements of both the x^A{\hat{x}}_{\text{A}}x^A​ x ̂ A and p^A{\hat{p}}_{A}p^​A​ p ̂ A observables can be inferred with errors below the standard quantum limit. The capability of assigning precise values to multiple observables and to observe their variation during physical processes may have implications in quantum state estimation and sensing.
Abstract In quantum mechanics, the Heisenberg uncertainty relation presents an ultimate limit to the precision by which one can predict the outcome of position and momentum measurements on a particle. Heisenberg explicitly stated this relation for the prediction of “hypothetical future measurements”, and it does not describe the situation where knowledge is available about the system both earlier and later than the time of the measurement. Here, we study what happens under such circumstances with an atomic ensemble containing 1011 rubidium atoms, initiated nearly in the ground state in the presence of a magnetic field. The collective spin observables of the atoms are then well described by canonical position and momentum observables, x^A{\hat{x}}_{\text{A}}x^A​ x ̂ A and p^A{\hat{p}}_{\text{A}}p^​A​ p ̂ A that satisfy [x^A,p^A]=iℏ[{\hat{x}}_{\text{A}},{\hat{p}}_{\text{A}}]=i\hslash[x^A​,p^​A​]=iℏ [ x ̂ A , p ̂ A ] = i ℏ . Quantum non-demolition measurements of p^A{\hat{p}}_{\text{A}}p^​A​ p ̂ A before and of x^A{\hat{x}}_{\text{A}}x^A​ x ̂ A after time t allow precise estimates of both observables at time t. By means of the past quantum state formalism, we demonstrate that outcomes of measurements of both the x^A{\hat{x}}_{\text{A}}x^A​ x ̂ A and p^A{\hat{p}}_{A}p^​A​ p ̂ A observables can be inferred with errors below the standard quantum limit. The capability of assigning precise values to multiple observables and to observe their variation during physical processes may have implications in quantum state estimation and sensing.
According to Heisenberg's uncertainty relation, there is an ultimate limit to how precisely we may predict the outcome of position and momentum measurements on a quantum system. We show that this limit may be violated by an arbitrarily large factor if one aims, instead, to guess the unknown value of a past measurement. For experiments on a single quantum system, the precise assignment of past position and momentum measurement outcomes is accompanied by large uncertainty about their linear combinations, while we show that entanglement with an ancillary system permits accurate retrodiction of any such linear combination. Finally, we show that the outcomes of experiments that jointly measure multiple linear combinations of position and momentum observables by means of ancillary probe particles can also be guessed with no formal lower limit. We present quantitative results for projective measurements and for generalized measurements where all components are prepared in Gaussian states.
Measurements with quantum limited resolution have important applications in metrology and sensing, including atomic clocks, atom interferometry, and magnetometry. We perform a quantum-non-demolition measurement on a collective angular momentum of a million spin-4 Cs atoms with high optical depth in our work. Quantum mechanics limits the measurement's resolution to what is known as the standard quantum limit (SQL) when there is no entanglement between the individual atoms. We can generate entanglement between atoms to create spin squeezed states through quantum backaction, improving the measurement sensitivity by 5.5 dB relative to the SQL. We have recently rebuilt the entire experiment inside a state-of-the-art magnetic shield of mu-metal and aluminum. This upgrade has drastically mitigated classical control errors in the spin squeezing experiment. Furthermore, the ensemble's sensitivity to magnetic fields allows us to make precise measurements of the magnetic field environment. Using closed-loop feedback, we use our atomic magnetometer to measure magnetic fields 4.3 dB below the SQL. The shielded environment will allow us to optimize the magnetometer and sets the stage for future experiments to use the closed-loop control to explore more complicated quantum dynamics.
Quantum Sensors, like atom interferometers (AI), can be employed for high-precision measurements of inertial forces, including their application as gravimeters, gradiometers, accelerometers, and gyroscopes. Their measurement principle relies on ultracold atoms that are prepared in quantum-mechanical superposition states in external degrees of freedom. These states can be prepared by a momentum transfer of a Raman laser. Then the superposition state senses the effect of an inertial force, which induce a corresponding relative phase. The phase is read out by a final coupling which converts the interferometric phase into a atom number difference between the two states. The difference provides an estimate of the interferometric phase and the corresponding quantity of interest. The quantum mechanical noise of the atomic ensemble cause a fundamental uncertainty of this estimation, which I analyze for generic AIs. For small atomic densities, the quantum phase noise of the ensemble limits the interferometric sensitivity. For large densities, quantum number fluctuations generate density fluctuations, which generates phase noise. I show that these two competing effects result in an optimal atom number with a maximal interferometer resolution. Squeezed atomic samples allow for a reduction of the quantum noise of one quantity at the expense of an increased noise along of a conjugate quantity. Phase and number are such quantities which obey to a variant of Heisenberg’s uncertainty principle. Neither phase nor number squeezing can improve the maximal interferometer resolution. As one main result of this thesis, I show how an optimal squeezing in between number and phase squeezing, allows for a fundamental improvement. I evaluate possible experimental paths to implement the proposed protocol. Concepts for a squeezing-enhanced operation of external-degree AIs have not yet been demonstrated. I propose and implement an atomic gravimeter, which is designed to accept spin-squeezed atomic states as input states. The interferometer is designed such that the interferometer couplings are performed in spin space, while the phase accumulation is performed in momentum states. For this interferometer, the squeezed input can be directly obtained from spin dynamics in spinor Bose-Einstein condensates. The main noise contributions in the experiment are analyzed, which results in a factor of 84 above the relevant quantum limit, preventing a squeezing enhancement so far. I outline a suppression of the main noise source, uncontrolled AC Stark shift on the squeezed mode and propose future important applications, including test of spontaneous collapse theories and an improvement of large-scale, high-precision gradiometers.
Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is beneficial to consider macroscopic spin ensembles, such as nuclear spins in solids and liquids. Coupling a macroscopic spin ensemble to a parametrically-modulated resonant circuit can create collective spin squeezing by generating spin correlations mediated by the circuit. We analyze the squeezing dynamics in the presence of decoherence and finite spin polarization, showing that achieving 7 dB spin squeezing is feasible in several nuclear spin systems. The metrological benefit of squeezing a macroscopic spin ensemble lies in the suppression of technical noise sources in the spin detection system relative to the spin projection noise. This expands the experimental sensitivity bandwidth when searching for signals of unknown frequency and can improve the resonant signal-to-noise ratio. Squeezing macroscopic spin ensembles may prove to be a useful technique for fundamental physics experiments aimed at detecting spin interactions with oscillating background fields, such as ultralight dark matter.