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Digest - IEEE Antennas and Propagation Society. International Symposium

Modeling Radiation Reaction Induced Superradiance in Quantum Dot Systems

Elliot Lu, Carlo Piermarocchi, B. Shanker

Published Jul 5, 2020• 1 citation
Publisher

Abstract

We simulate the collective emission effect known as superradiance in quantum dots ensembles by considering interactions with their classical radiation reaction field. We show that this reaction field emerges from the secondary radiated field via an expansion of the associated time domain Green's function. Incorporating this reaction field in a Maxwell-Bloch simulation, we reproduce characteristic superradiant behavior.

DOI
10.1109/ieeeconf35879.2020.9330119

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We simulate the collective emission effect known as superradiance in quantum dots ensembles by considering interactions with their classical radiation reaction field. We show that this reaction field emerges from the secondary radiated field via an expansion of the associated time domain Green's function. Incorporating this reaction field in a Maxwell-Bloch simulation, we reproduce characteristic superradiant behavior.
We introduce a computational Maxwell-Bloch framework for investigating out-of-equilibrium optical emitters in open systems. To do so, we compute the pulse-induced dynamics of each emitter from fundamental light-matter interactions and self-consistently calculate their radiative coupling, including phase inhomogeneity from propagation effects. This semiclassical framework is applied to open quantum dots systems with different densities and dipolar coupling. We observe signatures of superradiant behavior, such as directionality and faster decay, as well as subradiant emission. We compare and discuss the computed light emission obtained with our method and a master equation approach. Our framework enables quantitative investigations of large optical ensembles in the time domain and could be used to design new systems with enhanced superradiant and subradiant properties.
The problem of the evolution in time of a system of two-level atoms that are coupled through their electromagnetic fields, is studied and solved in the framework of semiclassical radiation theory. The atoms may be in any initial states and the radiation reaction is fully taken into account. Both superradiance and time-dependent frequency shift or chirping effects are found. The assumption that all the atoms see the same field is shown to place severe constraints on the evolution of the system, in the form of constants of the motion. These constraints are most easily pictured in terms of the Bloch-vector representation of the atomic system, and they lead to explicit solutions for the time development of each atom. It is shown that the evolution of the complex system is describable by means of a collective super Bloch vector, whose behavior is similar to the behavior of the Bloch vector for a single isolated atom. The constraints on the motion also imply that the system cannot radiate all its energy coherently; some of it remains trapped, to be dissipated ultimately by incoherent processes. Some curves are presented to illustrate the behavior of the system in special cases.
The possibility of realizing the superradiant regime of electromagnetic emission by the assembly of quantum dots is considered. The overall dynamical process is analyzed in detail. It is shown that there can occur several qualitatively different stages of evolution. The process starts with dipolar waves triggering the spontaneous radiation of individual dots. This corresponds to the fluctuation stage, when the dots are not yet noticeably correlated with each other. The second is the quantum stage, when the dot interactions through the common radiation field become more important, but the coherence is not yet developed. The third is the coherent stage, when the dots radiate coherently, emitting a superradiant pulse. After the superradiant pulse, the system of dots relaxes to an incoherent state in the relaxation stage. If there is no external permanent pumping, or the effective dot interactions are weak, the system tends to a stationary state during the last stationary stage, when coherence dies out to a low, practically negligible, level. In the case of permanent pumping, there exists the sixth stage of pulsing superradiance, when the system of dots emits separate coherent pulses.
Superradiance describes the coherent collective radiation caused by the interaction between many emitters, mediated by a shared electromagnetic field. Recent experiments involving Bose–Einstein condensates coupled to high-finesse cavities and interacting quantum dots in condensed-matter have attracted attention to the superradiant regime as a fundamental step to create quantum technologies. Here, we consider a simplified description of superradiance that allows the evaluation of statistical moments. A correspondence with the classical birthday problem recovers the statistical moments for discrete time and an arbitrary number of emitters. In addition, the correspondence provides a way to calculate the degeneracy of the problem.
In this paper we attempt to unify the theoretical treatment of a variety of cooperative interaction phenomena occurring in resonantly interacting radiation-matter systems. The system consists of a multimode optical field interacting with NNN resonant atoms in a region of large spatial extent. The field and atoms may or may not be coupled to reservoirs. We derive a set of coupled master equations for the reduced matter and radiation density operators of the composite system in the first Born approximation, using a method due to Bogoliubov. These equations describe within a single framework phenomena involving superradiant emission and coherent propagation. In the first place, our theory generalizes existing formulations of the superradiance problem by treating the radiation field as part of the dynamical system rather than as a reservoir. Hence, our equations describe stimulated interaction effects, which are entirely absent in the usual superradiance master equations. Moreover, our equations contain terms describing the self-consistent interaction of an average field with a set of polarizable atoms, as in the coupled Bloch and Maxwell equations of the theory of coherent pulse propagation, and enable us to describe fluctuations, arising from incoherent emission, about the average behavior described by the Bloch-Maxwell theory. We solve formally the dynamical equation for the radiation density operator and obtain a displaced multivariate Gaussian distribution centered on the solution of the Maxwell wave equation, which has as parameters the first and second moments of the matter density operator. Then we derive and discuss the field and atomic-moment equations, both in the wave-number and position representations. The moment equations enable us to show the relationship between descriptions of superradiant damping based on the Bloch equations and those based on the existence of correlated atomic states, including both as special cases. We introduce reduced matter moments, which allow us to separate incoherent- and coherent-emission effects and enable us to discuss the question of the closure of the moment equations. Then we consider cases where the behavior of the atomic system is dominated by a strong coherent pump wave or where the atoms are in a symmetric correlated state and show how the slowly-varying-envelope approximation simplifies the radiation-moment equations in these two cases. In the former case, we obtain an approximate theory which consists, in lowest order, of the Bloch-Maxwell equations with radiative-damping terms, plus an equation describing the time development of the correlation function for field fluctuations. Returning to our general formalism, we relate the usual parameters of the theory of radiative decay and of resonant interactions to the more general quantities appearing in our spatial analysis. Finally, we discuss the importance of the stimulated-emission terms appearing in our theory and describe several extensions, including the introduction of inhomogeneous broadening.
We consider sub- and superradiance of quantum emitters in a solid-state environment. This collective emission depends on the electromagnetic interaction between the emitters that can be engineered via the environment and described by the classical electromagnetic Green function. But also phonons may affect the collective emission. Phonons produce dephasing, both non-exponential fast initial dephasing and slower exponential dephasing. We compared several ways to account for both types of phonon interactions into the more standard optical master equation for an arbitrary number of quantum emitters that mutually interact via the electromagnetic field. In particular we present a concatenation method that incorporates phonon effects without adding computational complexity, suitable for arrays of emitters. Here we use it to study the effects of detunings on two-emitter spectra and on the corresponding population and entanglement dynamics.