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Mathematical and Computational Applications

Exact Evaluation of Statistical Moments in Superradiant Emission

Gilberto Medeiros Nakamura, Brenno Caetano Troca Cabella, Alexandre Souto Martinêz

Published Jun 23, 2019• 0 citations
Publisher

Abstract

Superradiance describes the coherent collective radiation caused by the interaction between many emitters, mediated by a shared electromagnetic field. Recent experiments involving Bose–Einstein condensates coupled to high-finesse cavities and interacting quantum dots in condensed-matter have attracted attention to the superradiant regime as a fundamental step to create quantum technologies. Here, we consider a simplified description of superradiance that allows the evaluation of statistical moments. A correspondence with the classical birthday problem recovers the statistical moments for discrete time and an arbitrary number of emitters. In addition, the correspondence provides a way to calculate the degeneracy of the problem.

DOI
10.3390/mca24020066

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Superradiance describes the coherent collective radiation caused by the interaction between many emitters, mediated by a shared electromagnetic field. Recent experiments involving Bose–Einstein condensates coupled to high-finesse cavities and interacting quantum dots in condensed-matter have attracted attention to the superradiant regime as a fundamental step to create quantum technologies. Here, we consider a simplified description of superradiance that allows the evaluation of statistical moments. A correspondence with the classical birthday problem recovers the statistical moments for discrete time and an arbitrary number of emitters. In addition, the correspondence provides a way to calculate the degeneracy of the problem.
In this paper we attempt to unify the theoretical treatment of a variety of cooperative interaction phenomena occurring in resonantly interacting radiation-matter systems. The system consists of a multimode optical field interacting with NNN resonant atoms in a region of large spatial extent. The field and atoms may or may not be coupled to reservoirs. We derive a set of coupled master equations for the reduced matter and radiation density operators of the composite system in the first Born approximation, using a method due to Bogoliubov. These equations describe within a single framework phenomena involving superradiant emission and coherent propagation. In the first place, our theory generalizes existing formulations of the superradiance problem by treating the radiation field as part of the dynamical system rather than as a reservoir. Hence, our equations describe stimulated interaction effects, which are entirely absent in the usual superradiance master equations. Moreover, our equations contain terms describing the self-consistent interaction of an average field with a set of polarizable atoms, as in the coupled Bloch and Maxwell equations of the theory of coherent pulse propagation, and enable us to describe fluctuations, arising from incoherent emission, about the average behavior described by the Bloch-Maxwell theory. We solve formally the dynamical equation for the radiation density operator and obtain a displaced multivariate Gaussian distribution centered on the solution of the Maxwell wave equation, which has as parameters the first and second moments of the matter density operator. Then we derive and discuss the field and atomic-moment equations, both in the wave-number and position representations. The moment equations enable us to show the relationship between descriptions of superradiant damping based on the Bloch equations and those based on the existence of correlated atomic states, including both as special cases. We introduce reduced matter moments, which allow us to separate incoherent- and coherent-emission effects and enable us to discuss the question of the closure of the moment equations. Then we consider cases where the behavior of the atomic system is dominated by a strong coherent pump wave or where the atoms are in a symmetric correlated state and show how the slowly-varying-envelope approximation simplifies the radiation-moment equations in these two cases. In the former case, we obtain an approximate theory which consists, in lowest order, of the Bloch-Maxwell equations with radiative-damping terms, plus an equation describing the time development of the correlation function for field fluctuations. Returning to our general formalism, we relate the usual parameters of the theory of radiative decay and of resonant interactions to the more general quantities appearing in our spatial analysis. Finally, we discuss the importance of the stimulated-emission terms appearing in our theory and describe several extensions, including the introduction of inhomogeneous broadening.
Superradiance is a quantum phenomenon in which coherence between emitters results in enhanced and directional radiative emission. Many quantum optical phenomena can be characterized by the two-time quantum correlation function g(2)(t,τ)g^{(2)}(t,τ)g(2)(t,τ), which describes the photon statistics of emitted radiation. However, the critical task of determining g(2)(t,τ)g^{(2)}(t,τ)g(2)(t,τ) becomes intractable for large emitter ensembles due to the exponential scaling of the Hilbert space dimension with the number of emitters. Here, we analyse and benchmark two approximate numerical sampling methods applicable to emitter arrays embedded within electromagnetic environments, which generally provide upper and lower bounds for g(2)(t,0)g^{(2)}(t,0)g(2)(t,0). We also introduce corrections to these methods (termed offset corrections) that significantly improve the quality of the predictions. The optimal choice of method depends on the total number of emitters, such that taken together, the two approaches provide accurate descriptions across a broad range of important regimes. This work therefore provides new theoretical tools for studying the well-known yet complex phenomenon of superradiance in large ensembles of quantum emitters.
The basic features of coherent spontaneous emission, including its dependence on the square of the number of participating emitters, are reviewed. Analogies with magnetic resonance phenomena are exploited, and we explain the need to go beyond such analogies in order to treat optical emission. Some recent results in the theory of optical superradiance are discussed. The radiative decay process is treated as a quantum-classical interpolation problem, and explicit solutions are given. In addition to its time dependence, we give the angular distribution of radiated power and the expected intensity fluctuations, and we estimate the maximum number of emitters which can cooperate in a superradiant event. Dicke's “coherence brightening” criterion is discussed from the point of view of the present paper. A “failure” of the criterion is exhibited and explained. Two of the purely quantum aspects of superradiance are isolated and discussed briefly.
Motivated by recent experiments with superradiant Bose-Einstein Condensate (BEC) we consider simple microscopic models describing rigorously the interference of the two cooperative phenomena, BEC and radiation, in thermodynamic equilibrium. Our resuts in equilibrium confirm the presence of the observed superradiant light scattering from BEC: (a) the equilibrium superradiance exists only below a certain transition temperature; (b) there is superradiance and matter-wave (BEC) enhancement due to the coherent coupling between light and matter.
A theory of coherent light scattering from an elongated Bose-Einstein condensate exposed to an off-resonant laser beam is presented. The model describes the emission of two superradiant pulses along the sample's major axis simultaneous with the formation of a bidimensional atomic grating inside the sample, as was observed in a recent MIT experiment [Inouye, S. et al., 1999, Science, 285, 571]. We predictions of the semiclassical model, in which the atomic motion is treated classically, are compared with these of the quantum model, obtained including the quantum mechanical description of the atomic motion. In the quantum limit the superradiant regime becomes a sequential process, in which during each collective scattering atoms emit a it hyperbolic secant pulse and populate an adjacent momentum state.
Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled W-states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations in order to explore the photon-photon correlations of the radiation emitted by such states. We present specifically results for the spatially resolved photon-photon correlations of systems prepared in doubly excited W-states and give conditions when the atomic system emits nonclassial light. Equally, we derive the conditions for the occurrence of bunching and even of superbunching, a rare phenomenon otherwise known only from nonclassical states of light like the squeezed vacuum. We finally investigate the photon-photon cross correlations of the spontaneously scattered light and highlight the nonclassicalty of such correlations. The theoretical findings can be implemented with current technology, e.g., using ions in a linear rf-trap, atoms in an optical lattice or quantum dots in a cavity.