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Bulletin of the American Physical Society

Quantum Sensing with Fiber-Coupled Diamond Emitters

Sean M. Blakley, Ilya V. Fedotov, Xinghua Liu, Christapher Vincent, Alexey V. Akimov, Philip Hemmer, Aleksei M. Zheltikov

Published Mar 18, 2021• 0 citations
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The interaction of photons with individual quantum systems is a very fundamental process in physics. Thereby, the emission rate as well as the angular emission pattern of a quantum emitter are not only a function of intrinsic properties of the emitter itself, but are also strongly modified by its surrounding. For instance, by restricting the optical modes which are allowed at the position of the dipole, the emission rate can be strongly modified and the emitted photons can be directed into specific optical modes. This effect can be demonstrated by the interaction of a single optically active quantum emitter with the strongly confined optical mode of a single-mode dielectric waveguide. Efficient coupling of the emitter to the dielectric structure can be achieved by placing the quantum emitter inside the evanescent field of the guided mode. This evanescent field coupling mechanism is discussed and demonstrated experimentally. A single nitrogen-vacancy center (NV-center), hosted in a nanodiamond is deterministically coupled to a tapered optical fiber (TOF) via the evanescent field of its guided mode (coupling efficiencies exceeding 30% are predicted). By employing an AFM-based nanomanipulation technique, the diamond nanocrystal is placed on the nanofiber waist of the TOF. Beforehand, the diamond nanocrystal has been characterized to guarantee that it hosts only one fluorescing NV-center. While the diamond nanocrystal is optically exited, single photon fluorescence of the NV-center is detected at both outputs of the tapered optical fiber. This verifies the evanescent coupling of the emitter to the guided mode. In order to quantify the coupling, the comparison of the emission rate into free space with the rate into the fiber yields that 10.0(5) of the emitted photons are coupled into the tapered optical fiber. In the determination of this value, the orientation of the emitting dipoles and the emission pattern, which are modified by the TOF, have been considered. The NV-center features a broad emission spectrum which can be used to investigate the wavelength-dependence of the coupling. Comparing the spectra of the emission into the fiber mode with the emission into free space modes roughly resembles the expected wavelength dependency of the coupling efficiency. The evanescent coupling and the deterministic positioning of preselected fluorescing diamond nanocrystals, which has been demonstrated with the TOF, can be applied to other waveguide structures as well. Dielectric single-mode waveguides made of Ta2O5 on a SiO2 substrate promise similar coupling efficiencies to tapered optical fibers (above 30%). With the design of the on-chip wave-guiding structure being flexible, the combination with other optical on-chip elements is feasible, rendering it a promising platform for on-chip photonic experiments. Test structures of this waveguide design are realized using lithographic processes and are characterized. These waveguides are equipped with inverted taper structures to allow efficient off-chip coupling with butt-coupling to standard single-mode fibers. The evanescent coupling of a single quantum emitter to a singe optical mode can be used to efficiently collect emission of the quantum emitter. This can help building a compact single photon source and is beneficial for the optical read-out of the quantum emitter's internal degree of freedom, which can be either used as probe (sensing) or as information-storage. Utilizing the high coupling efficiency, for instance, the non-linearities of the quantum system can be exploited to build a single photon transistor. The evanescent coupling is very broadband (about hundred nanometers), allowing to efficiently collect emission from broadband emitters like the NV-center, but it can also be used for multi-wavelength manipulation schemes.

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In this work, we present a platform for testing the device performance of a cavity–emitter system, using an ensemble of emitters and a tapered optical fiber. This method provides high-contrast spectra of the cavity modes, selective detection of emitters coupled to the cavity and an estimate of the device performance in the single-emitter case. Using nitrogen-vacancy (NV) centers in diamond and a GaP optical microcavity, we are able to tune the cavity onto the NV resonance at 10 K, couple the cavity-coupled emission to a tapered fiber and measure the fiber-coupled NV spontaneous emission decay. Theoretically, we show that the fiber-coupled average Purcell factor is 2–3 times greater than that of free-space collection, although due to ensemble averaging it is still a factor of 3 less than the Purcell factor of a single, ideally placed center.

arXiv:1102.5372•New Journal of Physics•May 31, 2011•28 citations
The interaction of photons with individual quantum systems is a very fundamental process in physics. Thereby, the emission rate as well as the angular emission pattern of a quantum emitter are not only a function of intrinsic properties of the emitter itself, but are also strongly modified by its surrounding. For instance, by restricting the optical modes which are allowed at the position of the dipole, the emission rate can be strongly modified and the emitted photons can be directed into specific optical modes. This effect can be demonstrated by the interaction of a single optically active quantum emitter with the strongly confined optical mode of a single-mode dielectric waveguide. Efficient coupling of the emitter to the dielectric structure can be achieved by placing the quantum emitter inside the evanescent field of the guided mode. This evanescent field coupling mechanism is discussed and demonstrated experimentally. A single nitrogen-vacancy center (NV-center), hosted in a nanodiamond is deterministically coupled to a tapered optical fiber (TOF) via the evanescent field of its guided mode (coupling efficiencies exceeding 30% are predicted). By employing an AFM-based nanomanipulation technique, the diamond nanocrystal is placed on the nanofiber waist of the TOF. Beforehand, the diamond nanocrystal has been characterized to guarantee that it hosts only one fluorescing NV-center. While the diamond nanocrystal is optically exited, single photon fluorescence of the NV-center is detected at both outputs of the tapered optical fiber. This verifies the evanescent coupling of the emitter to the guided mode. In order to quantify the coupling, the comparison of the emission rate into free space with the rate into the fiber yields that 10.0(5) of the emitted photons are coupled into the tapered optical fiber. In the determination of this value, the orientation of the emitting dipoles and the emission pattern, which are modified by the TOF, have been considered. The NV-center features a broad emission spectrum which can be used to investigate the wavelength-dependence of the coupling. Comparing the spectra of the emission into the fiber mode with the emission into free space modes roughly resembles the expected wavelength dependency of the coupling efficiency. The evanescent coupling and the deterministic positioning of preselected fluorescing diamond nanocrystals, which has been demonstrated with the TOF, can be applied to other waveguide structures as well. Dielectric single-mode waveguides made of Ta2O5 on a SiO2 substrate promise similar coupling efficiencies to tapered optical fibers (above 30%). With the design of the on-chip wave-guiding structure being flexible, the combination with other optical on-chip elements is feasible, rendering it a promising platform for on-chip photonic experiments. Test structures of this waveguide design are realized using lithographic processes and are characterized. These waveguides are equipped with inverted taper structures to allow efficient off-chip coupling with butt-coupling to standard single-mode fibers. The evanescent coupling of a single quantum emitter to a singe optical mode can be used to efficiently collect emission of the quantum emitter. This can help building a compact single photon source and is beneficial for the optical read-out of the quantum emitter's internal degree of freedom, which can be either used as probe (sensing) or as information-storage. Utilizing the high coupling efficiency, for instance, the non-linearities of the quantum system can be exploited to build a single photon transistor. The evanescent coupling is very broadband (about hundred nanometers), allowing to efficiently collect emission from broadband emitters like the NV-center, but it can also be used for multi-wavelength manipulation schemes.
Integration of solid-state quantum emitters such as NV center in diamond with tapered optical fiber is demanded by number of applications ranging from sensing and imaging to quantum communications and computations. Nevertheless, utilization of a single NV center coupled with an optical fiber meets significant challenge of fiber fluorescence that can considerably mask emission of the quantum object. In this paper, we analyze main sources of such fluorescence for the case of NV center coupled to tapered single mode optical fiber and discuss possible ways of improving signal to noise ratio in this case.
In this work, we present a platform for testing the device performance of a cavity–emitter system, using an ensemble of emitters and a tapered optical fiber. This method provides high-contrast spectra of the cavity modes, selective detection of emitters coupled to the cavity and an estimate of the device performance in the single-emitter case. Using nitrogen-vacancy (NV) centers in diamond and a GaP optical microcavity, we are able to tune the cavity onto the NV resonance at 10 K, couple the cavity-coupled emission to a tapered fiber and measure the fiber-coupled NV spontaneous emission decay. Theoretically, we show that the fiber-coupled average Purcell factor is 2–3 times greater than that of free-space collection, although due to ensemble averaging it is still a factor of 3 less than the Purcell factor of a single, ideally placed center.