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Moiré heterostructures as a condensed-matter quantum simulator

Kennes, Dante Marvin, Martin Claassen, Xian, Lede, Georges, Antoine, Andrew J. Millis, Hone, James, Dean, Cory R., D. N. Basov, Pasupathy, Abhay N., Ángel Rubio

Published Jan 1, 2021• 468 citations
OpenAlex

Abstract

Twisted van der Waals heterostructures have latterly received prominent attention for their many remarkable experimental properties and the promise that they hold for realizing elusive states of matter in the laboratory. We propose that these systems can, in fact, be used as a robust quantum simulation platform that enables the study of strongly correlated physics and topology in quantum materials. Among the features that make these materials a versatile toolbox are the tunability of their properties through readily accessible external parameters such as gating, straining, packing and twist angle; the feasibility to realize and control a large number of fundamental many-body quantum models relevant in the field of condensed-matter physics; and finally, the availability of experimental readout protocols that directly map their rich phase diagrams in and out of equilibrium. This general framework makes it possible to robustly realize and functionalize new phases of matter in a modular fashion, thus broadening the landscape of accessible physics and holding promise for future technological applications.

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Twisted van der Waals heterostructures have latterly received prominent attention for their many remarkable experimental properties and the promise that they hold for realizing elusive states of matter in the laboratory. We propose that these systems can, in fact, be used as a robust quantum simulation platform that enables the study of strongly correlated physics and topology in quantum materials. Among the features that make these materials a versatile toolbox are the tunability of their properties through readily accessible external parameters such as gating, straining, packing and twist angle; the feasibility to realize and control a large number of fundamental many-body quantum models relevant in the field of condensed-matter physics; and finally, the availability of experimental readout protocols that directly map their rich phase diagrams in and out of equilibrium. This general framework makes it possible to robustly realize and functionalize new phases of matter in a modular fashion, thus broadening the landscape of accessible physics and holding promise for future technological applications.
Abstract Moiré superlattice designed in stacked van der Waals material provides a dynamic platform for hosting exotic and emergent condensed matter phenomena. However, the relevance of strong correlation effects and the large size of moiré unit cells pose significant challenges for traditional computational techniques. To overcome these challenges, we develop an unsupervised deep learning approach to uncover electronic phases emerging from moiré systems based on variational optimization of neural network many-body wavefunction. Our approach has identified diverse quantum states, including novel phases such as generalized Wigner crystals, Wigner molecular crystals, and previously unreported Wigner covalent crystals. These discoveries provide insights into recent experimental studies and suggest new phases for future exploration. They also highlight the crucial role of spin polarization in determining Wigner phases. More importantly, our proposed deep learning approach is proven general and efficient, offering a powerful framework for studying moiré physics.
Moiré related physics in twisted bilayer two-dimensional (2D) materials has attracted widespread interest in condensed matter physics. Simulation of moiré related physics in cold atom platform is expected to outperform the 2D materials thanks to its advantage of higher tunablility. Here, we demonstrate that, the cold atom platform enables a new mechanism of moiré lattice formation, induced by interlayer interaction with intrinsic "dynamical" character, in contrast to conventional moiré lattice induced by "static" ways such as single-particle interlayer tunneling. Specifically, we consider a twisted bilayer Bose-Hubbard model with vanishing interlayer tunneling, and the bilayer is solely coupled through interlayer interaction that originates from contact interaction of atoms. We find that this system hosts a plethora of novel phases unique to this dynamical lattice, including a variety of Mott insulator (MI) and superfluid (SF) phases either preserving or breaking moiré lattice symmetry, phases with one layer in SF and the other in MI, "interlocked" MI, and self-localized phases at commensurate twist angles, which exhibits the characteristics of Bose glass and quasi-many-body localization in the absence of (quasi)disorder or quasicrystalline lattices. Our prediction can be readily observed in current experimental setup of twisted bilayer optical lattices, opening up new avenues for exploring the rich physics of interaction induced moiré systems in cold atoms.
We propose multilayer moiré structures in strong external magnetic fields as a novel platform for realizing highly tunable, frustrated Hubbard physics with topological order. Identifying the layer degree of freedom as a pseudospin allows us to retain SU(2) symmetry while controlling ring-exchange processes and concurrently quenching the kinetic energy by large external magnetic fields. This way, a broad class of interacting Hubbard-Hofstadter states and their transitions can be studied. Remarkably, in the limit of strong interactions the system becomes Mott insulating and we find chiral pseudospin-liquid phases which are induced by the magnetic field. We find that this topologically ordered state remains exceptionally stable toward relevant perturbations. We discuss how layer pseudospin can be probed in near-term experiments. As the magnetic flux can be easily tuned in moiré systems, our approach provides a promising route toward the experimental realization and control of topologically ordered phases of matter. Published by the American Physical Society 2024
Twisted transition metal dichalcogenides offer an exceptionally tunable moiré platform for studying correlation physics beyond conventional condensed matter systems. In particular, the intriguing interplay between the displacement field and the twist angle remains to be fully resolved. In this paper, we use large-scale density matrix renormalization group simulations to study the minimal moiré Hubbard model on a triangular lattice at half-filling, where the displacement field effect is captured by a spin-dependent staggered flux. We find that the displacement field significantly enriches the triangular Hubbard phase diagram in several qualitative ways. It rapidly destabilizes the chiral spin liquid phase beyond a narrow weak-field regime, induces pronounced chiral correlations in the strong-coupling 120∘120^\circ120∘-antiferromagnetic phase, and stabilizes incommensurate spin-density wave phases at weaker coupling. We further find signatures of a continuous transition between the chiral spin liquid and chiral antiferromagnetic phases at a finite displacement field, potentially driven by spinon condensation. Our results uncover rich displacement-field-driven many-body physics and provide useful guidance for future experiments in moiré superlattice systems.
Quantum hardware platforms are getting increasingly sophisticated in their ability to simulate condensed matter, including but not limited to strongly-correlated, topological, and non-equilibrium phenomena. This review surveys recent progress in quantum-hardware-based simulations of condensed matter, primarily emphasizing gate-based digital quantum computer simulation, with analog experiments discussed as complementary benchmarks. We first review major hardware platforms, including superconducting qubits, trapped-ions, ultracold atoms, Rydberg arrays, photonic systems, and moire quantum materials. We then introduce the basic ingredients of digital quantum simulation. Building on this foundation, we discuss representative applications to condensed-matter physics, spanning ground-state problems, strongly correlated matter, topological phases, non-equilibrium dynamics, open-system physics, and high-energy-physics-inspired simulations. Finally, we summarize key methodological tools used in state-of-the-art quantum-simulation workflows. We emphasize that present noisy quantum simulations serve not only as near-term demonstrations, but also as prototypes for the encodings, diagnostic protocols and error-control strategies required for future fault-tolerant quantum simulation.