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Charge transport through single molecules, quantum dots and quantum wires

Sabine Andergassen, V. Meden, Splettstößer, Janine, Schoeller, Herbert, M. R. Wegewijs

Published Jan 1, 2010• 55 citations
OpenAlex

Abstract

We review recent progress in the theoretical description of correlation and quantum fluctuation phenomena in charge transport through single molecules, quantum dots and quantum wires. Various physical phenomena are addressed, relating to cotunneling, pair-tunneling, adiabatic quantum pumping, charge and spin fluctuations, and inhomogeneous Luttinger liquids. We review theoretical many-body methods to treat correlation effects, quantum fluctuations, non-equilibrium physics, and the time evolution into the stationary state of complex nanoelectronic systems.

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We review recent progress in the theoretical description of correlation and quantum fluctuation phenomena in charge transport through single molecules, quantum dots and quantum wires. Various physical phenomena are addressed, relating to cotunneling, pair-tunneling, adiabatic quantum pumping, charge and spin fluctuations, and inhomogeneous Luttinger liquids. We review theoretical many-body methods to treat correlation effects, quantum fluctuations, non-equilibrium physics, and the time evolution into the stationary state of complex nanoelectronic systems.
We give a brief introduction to Luttinger liquids and to the phenomena of electronic transport or conductance in quantum wires. We explain why the subject of transport in Luttinger liquids is relevant and fascinating and review some important results on tunneling through barriers in a one-dimensional quantum wire and the phenomena of persistent currents in mesoscopic rings. We give a brief description of our own work on transport through doubly-crossed Luttinger liquids and transport in the Schulz–Shastry exactly solvable Luttinger-like model. With a view to making this article accessible to researchers in diverse fields such as nuclear physics, particle physics, formal field theory and condensed matter physics, we begin by first giving a brief introduction. In Sec. 1, we explain the words such as "Luttinger liquid" and "transport" in the title. We also motivate the study of this subject by showing that field is very important at the current time from the applications point of view and describe why it is theoretically fascinating. We then give a quick review of some of the important results in the field in Sec. 2, before we go on to describe some work that we have recently done and are doing in this field in Sec. 3. Finally, in Sec. 4, we conclude by re-emphasizing the importance of this area and drawing attention towards future possibilities.
Abstract The understanding of out-of-equilibrium fluctuation relations in small open quantum systems has been a focal point of research in recent years. In particular, for systems with adiabatic time-dependent driving, it was shown that the fluctuation relations known from stationary systems do no longer apply due the geometric nature of the pumping current response. However, the precise physical interpretation of the corrected pumping fluctuation relations as well as the role of many-body interactions remained unexplored. Here, we study quantum systems with many-body interactions subject to slow time-dependent driving, and show that fluctuation relations of the charge current can in general not be formulated without taking into account the total energy current put into the system through the pumping process. Moreover, we show that this correction due to the input energy is nonzero only when Coulomb-interactions are present. Thus, fluctuation response relations offer an until now unrevealed opportunity to probe many-body correlations in quantum systems. We demonstrate our general findings at the concrete example of a single-level quantum dot model, and propose a scheme to measure the interaction-induced discrepancies from the stationary case.
In a first part, I study the electronic transport through a one-dimensional, finite-length quantum wire of correlated electrons (Luttinger liquid) coupled at arbitrary position via tunnel barriers to two semi-infinite, one-dimensional as well as stripe-like (two-dimensional) leads, thereby bringing theory closer towards systems resembling setups realized in experiments. In particular, I compute the temperature dependence of the linear conductance of a system without bulk impurities. The appearance of new temperature scales introduced by the lengths of the overhanging parts of the leads and the wire implies a conductance function which is much more complex than the simple power-law behavior obtained in earlier approaches. My results can be used to optimize the experimental setups designed for a verification of Luttinger-liquid scaling. In a second part, I suggest a setup to study Luttinger-liquid behavior in quantum wires which allows to determine the Luttinger-liquid parameter from two independent measurements: transport through a quantum dot embedded in the wire and the charge on the dot. To this end, I identified novel Luttinger-liquid power-laws in the charging of the dot. In a more technical part, I extended an adaption of the functional renormalization group such that it can be used on correlated electrons in complex geometries like the wire-lead structures described above and arbitrary dot structures coupled to Luttinger-liquid leads.
Luttinger-liquid behavior of one-dimensional correlated electron systems is characterized by power-law scaling of a variety of physical observables with exponents determined by a single interaction dependent parameter KKK. We suggest a setup to study Luttinger-liquid behavior in quantum wires which allows us to determine KKK from two independent measurements: transport through a quantum dot embedded in the wire and the charge on the dot. Consistency of the two KKK's for a single probe would provide strong experimental evidence for the Luttinger-liquid paradigm.
We describe microscopic theory for the quantum transport through finite interacting systems connected to noninteracting leads. It can be applied to small systems such as quantum dots, quantum wires, atomic chain, molecule, and so forth. The Keldysh formalism is introduced to study the nonlinear current-voltage characteristics, and general properties of the nonequilibrium Green's functions are provided. We apply the formulated to an out-of-equilibrium Anderson model that has been used widely for the Kondo effect in quantum dots. In the linear-response regime the Kubo formalism still has an advantage, because it relates the transport coefficients directly to the correlation functions defined with respect to the thermal equilibrium, and it has no ambiguities about a profile of the inner electric field. We introduce a many-body transmission coefficient, by which the dc conductance can be expressed in a Landauer-type form, quite generally. We also discuss transport properties of the Tomonaga-Luttinger liquid, which has also been an active field of research in this decade.
This thesis addresses two different topics related to the physics of nanoscale systems. The first topic concerns quantum correlations and entanglement between electrons in solid-state systems, with a focus on how to generate electronic orbital entanglement on a sub-decoherence time scale and how to achieve experimentally more feasible entanglement detection schemes. The second topic concerns heat transport and temperature fluctuations in nanoscale systems, with a focus on how to utilize temperature fluctuations for calorimetric detection of single particles. The thesis comprises five papers.In Paper I, we propose a quantum dot system to generate and detect, using cotunneling processes, orbitally entangled pairs of electrons on a sub-decoherence time scale.In Paper II, we investigate, by applying an entanglement witness, the minimal number of zero-frequency current cross-correlation measurements needed to detect bipartite entanglement between two flying qubits.In Paper III, we consider energy and temperature fluctuations, and the influence of charging effects, in a metallic island tunnel coupled to a normal metallic lead, the so-called single electron box.In Paper IV, we investigate nanoscale quantum calorimetry and propose a setup consisting of a metallic island and a superconducting lead to realize a nanoscale calorimeter that may probe the energies of tunneling electrons.In Paper V, we investigate photon transport statistics of a microwave cavity, including the short-time statistics of single photon emissions and the long-time statistics of heat transport through the cavity.