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Acta Physica Sinica

Degenerate four-wave mixing-based double-channel optical gain spectrum with two frequency bands

Dan Wang, Rui-Xiang Guo, Yu-Peng Dai, Haitao Zhou

Published Jan 1, 2021• 0 citations
Publisher

Abstract

Focusing on the frequency division multiplexing technology in the applications of large scale optical communication, the double-channel optical gain spectrum with two frequency bands is studied in this paper. The double-channel gain spectrum, named probe channel and four wave mixing channel, comes from a co-propagating degenerate four wave mixing in a hot atomic ensemble. The intention is to divide the gain spectrum into several sub frequency bands through dressed four wave mixing. When a dressed field is exerted on one transition that shares the common excited state with the degenerate four wave mixing, the excited state can experience dressed splitting. It opens two transition paths for the degenerate four wave mixing simultaneously. Because of quantum interference between the two paths, the degenerate four wave mixing are suppressed at two-photon resonance. Consequently, Autler-Townes splitting appears in the gain spectrum, i.e. spectrum is changed from single frequency band into two “M”-type bands. In this paper, the nonlinear density matrix element describing the degenerate (dressed) four wave mixing is solved through perturbation theory, and then the gain spectrum in Doppler broadening atomic medium is plotted, and its Autler-Townes splitting is analyzed by using the dressed-state theory. It shows that the Autler-Townes splitting depends on both the Rabi frequency and single photon detuning of the dressed field. Relevant experiment is performed in cesium vapor at 60 ℃, a pair of high-gain optical spectra with two frequency bands for both double channels is successfully obtained. Moreover, the Autler-Townes splitting as a function of the dressed field intensity and single photon detuning are studied quantitatively. The experimental results accord well with the theoretical predictions. Compared with the degenerate four wave mixing, the atom-field coupled system is changed from an original open two-level into a closed Λ three-level due to the external dressed field, which greatly improves the atomic population on the coherent ground state via optical pumping, and therefore enhancing the gain significantly. This work is important for the field of atom-based optical communication. It provides an optional way of conveying multi-frequency information to the two parallel channels as well as improving the gain of four wave mixing.

DOI
10.7498/aps.70.20201778

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Focusing on the frequency division multiplexing technology in the applications of large scale optical communication, the double-channel optical gain spectrum with two frequency bands is studied in this paper. The double-channel gain spectrum, named probe channel and four wave mixing channel, comes from a co-propagating degenerate four wave mixing in a hot atomic ensemble. The intention is to divide the gain spectrum into several sub frequency bands through dressed four wave mixing. When a dressed field is exerted on one transition that shares the common excited state with the degenerate four wave mixing, the excited state can experience dressed splitting. It opens two transition paths for the degenerate four wave mixing simultaneously. Because of quantum interference between the two paths, the degenerate four wave mixing are suppressed at two-photon resonance. Consequently, Autler-Townes splitting appears in the gain spectrum, i.e. spectrum is changed from single frequency band into two “M”-type bands. In this paper, the nonlinear density matrix element describing the degenerate (dressed) four wave mixing is solved through perturbation theory, and then the gain spectrum in Doppler broadening atomic medium is plotted, and its Autler-Townes splitting is analyzed by using the dressed-state theory. It shows that the Autler-Townes splitting depends on both the Rabi frequency and single photon detuning of the dressed field. Relevant experiment is performed in cesium vapor at 60 ℃, a pair of high-gain optical spectra with two frequency bands for both double channels is successfully obtained. Moreover, the Autler-Townes splitting as a function of the dressed field intensity and single photon detuning are studied quantitatively. The experimental results accord well with the theoretical predictions. Compared with the degenerate four wave mixing, the atom-field coupled system is changed from an original open two-level into a closed Λ three-level due to the external dressed field, which greatly improves the atomic population on the coherent ground state via optical pumping, and therefore enhancing the gain significantly. This work is important for the field of atom-based optical communication. It provides an optional way of conveying multi-frequency information to the two parallel channels as well as improving the gain of four wave mixing.
With a forward cone emitting from the strong pump laser in a thermal rubidium atomic vapor, we investigate the non-degenerate parametrically amplified four-wave mixing (PA-FWM) process with dressing effects in a three-level "double-Λ" configuration both theoretically and experimentally. By seeding a weak probe field into the Stokes or anti-Stokes channel of the FWM, the gain processes are generated in the bright twin beams which are called conjugate and probe beams, respectively. However, the strong dressing effect of the pump beam will dramatically affect the gain factors both in the probe and conjugate channels, and can inevitably impose an influence on the quantum effects such as entangled degree and the quantum noise reduction between the two channels. We systematically investigate the intensity evolution of the dressed gain processes by manipulating the atomic density, the Rabi frequency and the frequency detuning. Such dressing effects are also visually evidenced by the observation of Autler-Townes splitting of the gain peaks. The investigation can contribute to the development of quantum information processing and quantum communications.
We study two-photon resonant nondegenerate four-wave mixing (NFWM) in a dressed cascade four-level system. In the presence of a strong coupling field, the two-photon resonant NFWM spectrum exhibits Autler-Townes splitting, accompanied by either suppression or enhancement of the NFWM signal. Such phenomena are demonstrated in Ba through inducing of atomic coherence between the ground state 6s26{s}^{2}6s2 and the doubly excited autoionizing Rydberg state 6pnd6pnd6pnd. This technique provides a spectroscopic tool for measuring not only the resonant frequency and dephasing rate but also the transition dipole moment between two highly excited atomic states.
Abstract We demonstrate the influence of dressed states on two-mode optical entanglement in a double Λ-type energy level atomic ensemble of parametric amplification four-wave mixing (PA-FWM) processes. By injecting a coherent or Einstein–Podolsky–Rosen field into PA-FWM channels, we investigate the corresponding entanglement. The quantum entanglement may be enhanced or suppressed via a bright state or a dark state. In free space, the two-mode entanglement is determined by nonlinear gain, which can be manipulated by field dressing in an atomic ensemble (i.e. Autler–Towns splitting, dressed enhancement/suppression of entanglement). However, in a ring cavity, the cavity dressing brings about the AT-like splitting of entanglement. Such an entanglement profile may be modified by field dressing through vacuum Rabi splitting, vacuum-induced enhancement and suppression of entanglement.
Abstract A higher degree of entanglement of entangled sources in quantum communications is always desired and can be achieved with high nonlinear gains. The dressing of atomic coherence and optical pumping can be considered as effective parameters to obtain such entangled sources. In this regard, we have experimentally studied doubly dressed effects in a small range of frequency, and optical pumping and de-pumping effects over a wide frequency range in multi-level atomic system in order to enhance the nonlinear gain. The multi-mode phenomenon that results from the multi-peak of Autler–Townes splitting can be observed at the large beam size of the pinhole of the pump field. Theoretical calculations fit well with the experimentally measured results. The dressing of atomic coherence and optical pumping lead to the enhancement of nonlinear gain up to 8.2 when the original nonlinear gain is 4.7.
In this work, we present a set of experiments involving four-wave mixing processes in rubidium atoms. We employ several experimental configurations exploring two- and three-level systems in cascade or Λ configurations, all of which are in a copropagating geometry, to investigate different physical phenomena present in each scenario. In the first experiment, we combine a cw diode laser and a 1 GHz femtosecond pulse train to generate coherent blue light through the four-wave mixing process in hot rubidium vapor. The generated coherent signal is analyzed by scanning either the diode frequency or the repetition rate of the frequency comb. In both cases, the cw laser induces an Autler- Townes splitting with a wide separation in the doublet structure due to the configuration of copropagating fields. To model these results, we employ the density matrix formalism to write the Bloch equations and solve them numerically. The solutions allow us to explore other cases beyond those involving our experimental setup, comparing the response of the upper-level population and the generated signal coherence for homogeneously and non-homogeneously broadened systems. Moreover, in this same experiment, we also observed an unexpected interference effect between excitation routes of the four-wave mixing process when the repetition rate of the pulse train is scanned. The theoretical model demonstrates that the interfering effect appears only when the repetition rate is carefully chosen to produce a pair of modes of the frequency comb resonant with both one- and two-photon transitions for the same atomic velocity group. In the second experiment, still with a hot rubidium vapor, we explore two symmetrical degenerate four- wave mixing signals induced by two almost copropagating laser beams, with~ka and~kb wave-vectors, and detected simultaneously in the 2~ka −~kb and 2~kb −~ka directions. Each spectrum has a single peak with a short frequency separation between them, which our model indicates is due to the nonlinear behavior of the refractive indexes, a consequence of the high intensity of both input fields. Finally, we use the same experimental setup for the two symmetrical signals to study the field intensity fluctuations of the degenerate four-wave mixing signals and the transmission signals. In this case, the sample is an ensemble of cold rubidium atoms in a magneto-optical trap. There is an intensity- intensity cross-correlation between the signals due to the resonant phase-noise to amplitude-noise conversion. In this type of cold system, we can neglect the Doppler- broadening, allowing a straightforward study of the dependency of the correlations on the laser detuning. In these measurements, we observe a type of oscillation in the correlation curves that the theoretical model indicates to be connected with Rabi oscillations, revealed by the fluctuations long after the transient period.
Abstract We investigate the coherent control of dressing interaction in four-wave mixing (FWM) in a Y-type four-level atomic system based on the dressed states theory. We study the density matrix equation acted by two dressing fields simultaneously governing FWM signal intensity and the eigenvalues under the dressed state formalism. It is shown that the peak position and intensity of Autler–Townes splitting both originate from the dressing interaction as the detuning of the probe field is scanned. Moreover, it is observed that the interaction could be controlled by the dressing fields. Such flexibly controlled nonlinear signal has potential applications in optical communication and quantum information processing.