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Coherent propagation effects in multilevel molecular systems

Cyrus D. Cantrell, Frank Rebentrost, W. H. Louisell, F. P. Mattar

Published Jan 1, 1981• 0 citations
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The Journal of Chemical Physics•Sep 15, 1988•30 citations
The Maxwell–Schrödinger equations describing the ultrashort laser pulse propagation in multilevel molecular media are shown to be analytically solvable and to reduce to nonlinear multisine-Gordon equations for certain models of the field–molecule system. Special cases of level schemes are shown to lead to soliton propagation. A numerical study is presented in order to examine the effect of nonresonant (virtual) transitions on pulse propagation and amplification in a three-level molecular system as a function of intensity and detuning.