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Springer series in chemical physics

Coherent Pulse Propagation Effects in Multilevel Molecular Systems

Cyrus D. Cantrell, W. H. Louisell, Jenny Lam

Published Jan 1, 1979• 3 citations
Publisher
DOI
10.1007/978-3-642-67254-5_36

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The Maxwell–Schrödinger equations describing the ultrashort laser pulse propagation in multilevel molecular media are shown to be analytically solvable and to reduce to nonlinear multisine-Gordon equations for certain models of the field–molecule system. Special cases of level schemes are shown to lead to soliton propagation. A numerical study is presented in order to examine the effect of nonresonant (virtual) transitions on pulse propagation and amplification in a three-level molecular system as a function of intensity and detuning.