Influence of fifth-order nonlinearities on the statistical fluctuations in emission intensities in a photonic open-cavity complex system
Iván R. R. González, Ernesto P. Raposo, Sandra J. M. Carreño, A. M. S. Macêdo, Melissa E. Maldonado, Leonardo de S. Menezes, Anderson S. L. Gomes, Cid Bartolomeu de Araujo
High-order nonlinear optical effects have become an important feature of photonic systems, both ordered and disordered. In this work, a very large and robust set of experimental data obtained from the emission spectra of a trivalent neodymium ion-based random laser, whose action mechanism relies upon gain and disorder, was characterized in detail. Using an effective model, it was possible to describe how the optical nonlinearities of the disordered gain medium affect the statistical behavior of the intensity fluctuations of the random laser for excitations close to and well above the laser threshold. A theoretical framework is presented and, in particular, in the regime well above threshold a nice fit to the experimental data is obtained with a distribution that incorporates nonlinearities up to fifth order, the Izrailev distribution.
High-order nonlinear optical effects have become an important feature of photonic systems, both ordered and disordered. In this work, a very large and robust set of experimental data obtained from the emission spectra of a trivalent neodymium ion-based random laser, whose action mechanism relies upon gain and disorder, was characterized in detail. Using an effective model, it was possible to describe how the optical nonlinearities of the disordered gain medium affect the statistical behavior of the intensity fluctuations of the random laser for excitations close to and well above the laser threshold. A theoretical framework is presented and, in particular, in the regime well above threshold a nice fit to the experimental data is obtained with a distribution that incorporates nonlinearities up to fifth order, the Izrailev distribution.
The statistical behavior of spectral intensity fluctuations in a Raman gain random fiber laser is investigated for the first time, to the best of our knowledge. Through a fiber Fabry–Perot tunable filter, the intensity of the filtered single wavelength from random laser (RL) spectra is measured at different pump powers. The probability density function (PDF) of spectral intensity values is analyzed. Well below the lasing threshold, the intensity of a single wavelength is stable in the time domain, and the PDF exhibits a typical Gaussian behavior. However, around the threshold, strong fluctuations in intensity emerge. In this case, the statistical distribution is characterized by a power-law-tailed function consistent with a Lévy α-stable distribution. We identify the statistical evolution as the injected pump power increases, from a Gaussian to a Lévy and then back to a Gaussian distribution, which is similar to the case of RLs with a strong disorder due to the presence of photon scatterers and gain related to electronic transitions in the active medium, indicating the universal existence of such statistical properties in random lasing systems.
The peculiar characteristics of random laser emission have been studied in many different media, leading to a classification of the working regimes based on the statistics of spectral fluctuations. Alongside such studies, the possibility to constrain light propagation by L\'evy walks, i.e., with a ``heavy-tailed'' distribution of steps, has opened the opportunity to investigate the behavior of a superdiffusive optical gain medium that can lead to a ``superdiffusive random laser.'' Here, we present a theoretical investigation, based on Monte Carlo simulations, on such a kind of medium, focusing on the widespread presence of fluctuation regimes, that, in contrast to a diffusive random laser, appears very hard to switch off by changing the gain and scattering strength. Hence, the superdiffusion appears as a condition that increases the value of the threshold energy and promotes the presence of fluctuations in the emission spectrum.
We derive the photon number probability distribution of light emitted from a random multiple-light-scattering medium with gain, using a generalized master equation. Our model treats the random laser medium as a collection of low quality-factor cavities, coupled by random photon diffusion. We demonstrate that, with stronger scattering, the pumping threshold for the transition from chaotic to isotropic coherent light emission decreases and the local second order coherence, above threshold, increases.
Radiation from a chaotic cavity filled with gain medium is considered. A set of coupled equations describing the photon density and the population of gain medium is proposed and solved. The spectral distribution and fluctuations of the radiation are found. The full noise is a result of a competition between positive correlations of photons with equal frequencies (due to stimulated emission and chaotic scattering) which increase fluctuations, and a suppression due to interaction with a gain medium which leads to negative correlations between photons. The latter effect is responsible for a pronounced suppression of the photonic noise as compared to the linear theory predictions.
We derive the photon-number probability distribution and the resulting degree of second-order optical coherence for light emission from a uniformly distributed active species within a multiple-light-scattering medium. This is obtained from a master equation describing the probability distribution for photons in the vicinity of position r, traveling with a wave vector k, related, in turn, to a coarse-grained average of the optical Wigner coherence function. Using a simple model for isotropic, spatially uncorrelated scatterers, this reduces to a generalization of the master equation of a conventional laser in which the medium behaves like a random collection of low-quality factor cavities that are coupled by photon diffusion between a given cavity and its neighbors. Laserlike coherence, on average, is obtained in the random laser above a specific pumping threshold. Photon-number statistics above and below the lasing threshold are computed by first assuming that the atomic response to the local electromagnetic fields is nearly instantaneous. Corrections to this simple model, arising from nonadiabatic atomic dynamics, are then estimated. The dependence of the photon statistics on scatterer density, gain concentration, and position within a sample reveal that, on average, increase of the scattering strength (decrease of the photon transport mean free path) in the medium leads to a sharper peak in the local photon-number distribution, characteristic of increased local coherence in the optical field. We also evaluate the coherence of the output field at points outside the random-laser medium. This is a weighted average of radiation emitted at different positions in the sample, exhibiting varying degrees of coherence due to variations in the local pumping intensity.
The interaction of light and matter can be described by a set of coupled nonlinear evolution equations for the material and electromagnetic fields. In order to account for the effects of vacuum fluctuations, noise forces which cause spontaneous transitions have to be included. In these macroscopic systems various sources of noise besides fundamental quantum fluctuations exist which are of macroscopic origin. These cause fluctuations of the cavity dissipation as well as of the external pumping power. In the course of an adiabatic elimination procedure, these fluctuations appear as multiplicative noise in the equations of motion (e.g. for the field intensity, due to the nonlinearity of the interaction). While fluctuations of the cavity damping create noise linear in the field intensity, randomness in the pump strength causes fluctuations that depend nonlinearly on the light intensity. In this respect, the noise terms enter the equations of motion quite differently and have to be distinguished from spontaneous emission noise which is independent of the field strength, and is the basis of all traditional laser models.