Quantum information systems require an interface between photons as a physical system to transport information and atoms which are better suited to store and process it. In this thesis the construction of a novel pulsed, bright and narrow-band light source is presented. It consists of an optical parametric oscillator featuring a periodically poled KTP crystal and a mechanical chopper and produces ?s-pulses of squeezed vacuum. The generated states are resonant to the Rubidium-DI-transition, are almost transform-limited and show more than 3 dB of squeezing. The physical effect of electromagnetically induced transparency (EIT) in hot rubidium vapor can be used to generate ultra-low group velocities and allows for a reversible adiabatic conversion of optical quantum states into collective spin excitations which can be used to stop pulses of light. I report about recent progress in slowing down a pulse of squeezed vacuum by one third of its width while still preserving 0.36 dB of squeezing in the process. I analyze electromagnetically induced transparency and light storage in an ensemble of atoms with multiple excited levels (multi-A configuration) which are coupled to one of the ground states by quantized signal fields and to the other one via classical control fields. A basis transformation of atomic and optical states which reduces the analysis of the system to that of electromagnetically induced transparency in a regular three-level configuration is presented. We demonstrate the existence of dark state polaritons and propose a protocol to transfer quantum information from one optical mode to another by adiabatic control of the control fields and present a proof-of principle experiment to adiabatically transfer light between modes of different frequencies in Rb-87 vapor. To that end a digital phase lock circuit has been designed that allows to electronically phase lock an external-cavity diode laser to a reference laser over a 7 GHz frequency range with sub-Hertz precision.
Quantum information systems require an interface between photons as a physical system to transport information and atoms which are better suited to store and process it. In this thesis the construction of a novel pulsed, bright and narrow-band light source is presented. It consists of an optical parametric oscillator featuring a periodically poled KTP crystal and a mechanical chopper and produces ?s-pulses of squeezed vacuum. The generated states are resonant to the Rubidium-DI-transition, are almost transform-limited and show more than 3 dB of squeezing. The physical effect of electromagnetically induced transparency (EIT) in hot rubidium vapor can be used to generate ultra-low group velocities and allows for a reversible adiabatic conversion of optical quantum states into collective spin excitations which can be used to stop pulses of light. I report about recent progress in slowing down a pulse of squeezed vacuum by one third of its width while still preserving 0.36 dB of squeezing in the process. I analyze electromagnetically induced transparency and light storage in an ensemble of atoms with multiple excited levels (multi-A configuration) which are coupled to one of the ground states by quantized signal fields and to the other one via classical control fields. A basis transformation of atomic and optical states which reduces the analysis of the system to that of electromagnetically induced transparency in a regular three-level configuration is presented. We demonstrate the existence of dark state polaritons and propose a protocol to transfer quantum information from one optical mode to another by adiabatic control of the control fields and present a proof-of principle experiment to adiabatically transfer light between modes of different frequencies in Rb-87 vapor. To that end a digital phase lock circuit has been designed that allows to electronically phase lock an external-cavity diode laser to a reference laser over a 7 GHz frequency range with sub-Hertz precision.
Abstract. We report on the generation of more than 5 dB of vacuum squeezed light at the Rubidium D1 line (795 nm) using periodically poled KTiOPO4 (PPKTP) in an optical parametric oscillator. We demonstrate squeezing at low sideband frequencies, making this source of non-classical light compatible with bandwidth limited atom optics experiments. When PPKTP is operated as a parametric amplifier, we show a noise reduction of 4 dB stably locked within the 150 kHz-500 kHz frequency range. This matches the bandwidth of Electromagnetically Induced Transparency (EIT) in Rubidium hot vapour cells under the condition of large information delay. Squeezed light at the Rubidium D1 line 2 The control of quantum states of light is of great interest for quantum communication purposes. Many quantum information protocols rely on the possibility of coherently delaying and storing the information carried by a laser beam. This can for example be achieved using Electromagnetically Induced Transparency (EIT). Experimental and theoretical studies have shown that information can be delayed within a narrow bandwidth when light interacts with atoms in a lambda configuration [2, 3, 4, 5]. One step further is the delay of quantum information, carried by squeezed
In the last few decades, coherent light-atom interactions have opened unprecedented possibilities for the coherent control of atomic and optical quantum systems, paved the way for the practical realization of quantum information technologies, and allowed for the creation of novel quantum-enhanced sensors. This dissertation investigates the interaction of multiple near-resonant optical fields with hot rubidium atoms under the conditions of electromagnetically induced transparency. The main goal of the presented research is to address some fundamental challenges in using such systems for practical applications. The EIT effect relies on the strong coupling of an optical probe field and a collective long-lived ensemble of atomic spins by the means of a strong classical optical control field in a Lambda configuration. While optically-thick atomic vapor is necessary to achieve such a strong coupling regime, the increasing optical depth of the atomic ensemble also leads to the effective enhancement of other nonlinear light-atom interactions, such as the four-wave mixing effect. Here we discuss the possibility to control four-wave mixing in a three-level system without deteriorating the coherent properties of EIT by introducing an additional absorber resonant exclusively with the Stokes field. The exclusive detection of a weak probe field in the presence of a strong control field is a challenging experimental task, especially at the few-photon level. Many experiments employ polarization and/or frequency filtering to compete the task. We present an alternative filtering technique based on optical vortices for cases when the traditional methods are not sufficient or restrict the experimental arrangements. Finally, we demonstrate the possibility to manipulate the group velocity of a pulsed squeezed vacuum field by using the optical dispersion modification via Zeeman spin coherence in rubidium atoms. By changing the interaction condition, we demonstrate the switch between the ``slow'' and (for the first time) ``fast'' light regime. We also show that increased optical depth simultaneously leads to the enhancement of pulse advancement and the deterioration of squeezing fidelity in the output pulses.
In this thesis we study light-matter coherence phenomena related to the interaction of a coherent laser field and the so-called Λ-system, a three-level quantum system (e.g., an atom). We observe electromagnetically induced transparency (EIT), slow and stored light in hot rubidium vapor. For example, a 6 μs Gaussian pulse propagate at a velocity of ~1 km/s (to be compared with the normal velocity of 300 000 km/s). Dynamic changes of the control parameter allows us to slow down a pulse to a complete stop, store it for ~100 μs, and then release it. During the storage time, and also during the release process, some properties of the light pulse can be changed, e.g., frequency chirping of the pulse is obtained by means of Zeeman shifting the energy levels of the Λ-system. If, bichromatic continuous light fields are applied we observe overtone generation in the beating signal, and a narrow `dip' in overtone generation efficiency on two-photon resonance, narrower than the `coherent population trapping' transparency. The observed light-matter coherence phenomena are explained theoretically from first principles, using the Lindblad master equation, in conjunction with the Maxwell's equations. Furthermore, we analyze an optical delay-line based on EIT and show that there is in principle (besides decoherence) no fundamental limitation, but the usefulness today is scant. The combination of EIT and a photonic crystal cavity is inquired into, and we show that the quality value of a small resonator (area of 2.5λ×2.5λ with a missing central rod) can be enhanced by a factor of 500 due to the increased modal density close to two-photon resonance. Open system effects (decoherence effects) are thoroughly investigated using a coherence vector formalism, furthermore, a vector form of the Lindblad equation is derived. Specifically we find an open system channel that lead to slow light and gain.
Recent years have observed fast developments in neutral atomic vapor based quantum information storage technology. The technique utilizes light fields in the optical wavelength region as signal carrier and retriever and neutral atomic systems (e.g. single atoms, ensembles of atoms, atom-like defects in solids) as storage media. Photons are robust carriers of information due to their high velocity (c = 2.998 x 108 m/s) and ease of transportation (they propagate rectilinearly with low loss). Their high mobility, however, makes it a challenging task to spatially localize and therefore store them. Atoms (or atom-like systems), on the other hand, can be easily localized in space while providing quantum states accessible to photons and therefore are ideal candidates for storage media. Electromagnetically-induced transparency (EIT) is a light-induced atomic coherence phenomenon that dramatically modifies the optical properties of an atomic medium to a weak probe field by the application of a strong coupling field. As a probe pulse propagates in an EIT medium it experiences ultraslow group velocity and generates a copropagating spin wave. These consequences of EIT can be exploited for light pulse storage and retrieval in an atomic medium.
We analyze electromagnetically induced transparency and light storage in an ensemble of atoms with multiple excited levels (multi-$\ensuremath{\Lambda}$ configuration) which are coupled to one of the ground states by quantized signal fields and to the other one via classical control fields. We present a basis transformation of atomic and optical states which reduces the analysis of the system to that of electromagnetically induced transparency in a regular three-level configuration. We demonstrate the existence of dark state polaritons and propose a protocol to transfer quantum information from one optical mode to another by an adiabatic control of the control fields.
This thesis set out to investigate light storage based on dynamic electromagnetically induced transparency (EIT) in a room-temperature atomic ensemble of rubidium as a means to provide a quantum memory for single-photons created by a single rubidium atom coupled to a high-finesse optical resonator. Setting up the light storage medium presented a new addition to the research group's portfolio of experimental techniques and led to investigations of EIT, slow light and stored light in warm rubidium-87 vapour. Lambda level schemes connecting Zeeman or hyperfine substates on the D1 and D2 lines were addressed in rubidium vapour cells containing different buffer gases and different isotopic fractions of rubidium-87 and rubidium-85. Single beam spectroscopy with a weak probe was used to characterise the vapour cells. A numerical method to fit the D line spectrum to a theoretical model to include isotopic fractions and collisional broadening of a buffer gas has been implemented. Temperature and isotopic fractions could be reliably extracted from the fit parameters. For an offset-stabilisation of two lasers to address a lambda level scheme connecting the two different hyperfine groundstates in rubidium a phase locked loop including a frequency divider has been designed and implemented. Light storage and retrieval has been demonstrated using a Zeeman scheme on the D1 line. Two microsecond long classical light pulses containing one million photons on average were stored and retrieved with an efficiency of 15% after a delay of one microsecond. Several methods of attenuating the strong co-propagating control laser beam to allow for lowering the signal pulse intensity in future experiments are discussed.