Temporal modes (TM) of light are a promising resource for quantum information as they span a discrete infinite dimensional encoding basis [1]. Additionally, TM are compatible with standard fibered communication as they share the same polarization, carrier frequency and transverse spatial mode properties. Single photons in specific TM can be obtained by Spontaneous Parametric Down Conversion (SPDC) and Spontaneous Four-Wave-Mixing (SFWM) sources. The Joint Spectral Amplitude (JSA), derived from energy and momentum conservation constraints describes the two-photon state and the signal and idler spectral distribution. The Schmidt decomposition of the JSA function : F = n √ λ n S n (ω s)I n (ω i) where the ({S n }) and ({I n }) are the TM basis of the signal and idler photons is sometimes reduced to one non zero term [2] where both signal and idler photons are generated in a single TM, giving rise to a fac-torable state of the pair. This can be achieved if a group velocity matching condition is satisfied (either β 1 (ω p) = β 1 (ω s) or β 1 (ω p) = β 1 (ω i) or 2 β 1 (ω p) = β 1 (ω s) + β 1 (ω i) in the case of SFWM with β 1 the inverse group velocity). Such single TM states are very useful for scalable heralded photon sources [3]. On the contrary, having several non-zero terms in the Schmidt decomposition depicts spectral correlations between the signal and idler which can also be required for others applications. Here we show experimentally in a stimulated regime how the shape of the JSA can be changed for photon pairs produced by FWM in a gas-filled inhibited-coupling (IC) fiber. IC fibers exhibit a discontinuous multiband dispersion where the position of the discontinuities are dictated by the strut thickness [4]. Such exotic dispersion opens new possibilities for the FWM phase matching fulfillment, and thus for tailoring the JSA. With the ability to have the pump and the generated signal and idler photons lying in different dispersion band, group-velocity matching can be easily obtained. We use stimulated emission tomography, which consists in seeding the FWM process with a tunable continuous wave laser, to reconstruct the 2D JSI (= |JSA| 2) as a function of signal and idler wavelengths. With a femtosecond pulsed pump at 1030 nm and a seed laser at telecom wavelength, Figure 1: Simulated JSI for different configurations of length, gas pressure and pump wavelength. Starting from the conditions of (a) P =3bar λp =1085 nm L = 1m, (b-d) correspond to the change of one parameter (b) L = 30 cm (c) P = 2.6 bar (d) λp =985 nm we chose two optimized fibers denoted A and B with struts thickness t=600 nm and inner-diameter d=40 µm and t=1250 nm; d=49 µm (Fig 2). These two fiber designs allow a multi-band FWM. Indeed the signal (fiber A), or both the signal and idler (fiber B) are generated in a different band from the pump. Xenon gas has been chosen because i) no Raman-Scattering can take place in a noble gas, which eliminates the usual main source of noise in fibered photon-pair generation and ii) it exhibits high non-linearity (in the order of 10 −21 m 2 /W at 10 bar). For a given fiber design, pump wavelength, gas pressure and fiber length are three adjustable parameters that can be tuned to access various JSA shapes as can be seen on the simulations in Fig.1. Both single TM or, opposingly, multi-TM can be obtained. Changing the gas pressure impacts the medium dispersion, which results in shifting the JSA and modifying its shape (Fig 1). As a first experimental demonstration in such gas-filled IC fibers, we experimentally reconstruct the JSI for two different fibers (Fig 2) with signal and idler wavelength respectively in the 771 nm and 1550 nm ranges. showing that two very different Schmidt decompositions can be obtained: a quasi factorable state and a correlated state. Figure 2: Fiber cross-section, experimental JSI and corresponding Schmidt decomposition for a 8 tubes IC-fiber and a kagome-IC fiber denoted A and B. In JSI of A the red dashed-lines define the measurement range. The pixelated structure of the JSI of B is due to an insufficient number of measures and will be improved. We have made a new proposal of using multi-dispersion band medium in order to engineer photon-pair time-frequency correlations. For the first time to our knowledge, we implement this technique using gas-filled inhibited-coupling fiber. More configurations are currently being investigated in order to demonstrate the real time tuning possibility in such a medium.
Temporal modes (TM) of light are a promising resource for quantum information as they span a discrete infinite dimensional encoding basis [1]. Additionally, TM are compatible with standard fibered communication as they share the same polarization, carrier frequency and transverse spatial mode properties. Single photons in specific TM can be obtained by Spontaneous Parametric Down Conversion (SPDC) and Spontaneous Four-Wave-Mixing (SFWM) sources. The Joint Spectral Amplitude (JSA), derived from energy and momentum conservation constraints describes the two-photon state and the signal and idler spectral distribution. The Schmidt decomposition of the JSA function : F = n √ λ n S n (ω s)I n (ω i) where the ({S n }) and ({I n }) are the TM basis of the signal and idler photons is sometimes reduced to one non zero term [2] where both signal and idler photons are generated in a single TM, giving rise to a fac-torable state of the pair. This can be achieved if a group velocity matching condition is satisfied (either β 1 (ω p) = β 1 (ω s) or β 1 (ω p) = β 1 (ω i) or 2 β 1 (ω p) = β 1 (ω s) + β 1 (ω i) in the case of SFWM with β 1 the inverse group velocity). Such single TM states are very useful for scalable heralded photon sources [3]. On the contrary, having several non-zero terms in the Schmidt decomposition depicts spectral correlations between the signal and idler which can also be required for others applications. Here we show experimentally in a stimulated regime how the shape of the JSA can be changed for photon pairs produced by FWM in a gas-filled inhibited-coupling (IC) fiber. IC fibers exhibit a discontinuous multiband dispersion where the position of the discontinuities are dictated by the strut thickness [4]. Such exotic dispersion opens new possibilities for the FWM phase matching fulfillment, and thus for tailoring the JSA. With the ability to have the pump and the generated signal and idler photons lying in different dispersion band, group-velocity matching can be easily obtained. We use stimulated emission tomography, which consists in seeding the FWM process with a tunable continuous wave laser, to reconstruct the 2D JSI (= |JSA| 2) as a function of signal and idler wavelengths. With a femtosecond pulsed pump at 1030 nm and a seed laser at telecom wavelength, Figure 1: Simulated JSI for different configurations of length, gas pressure and pump wavelength. Starting from the conditions of (a) P =3bar λp =1085 nm L = 1m, (b-d) correspond to the change of one parameter (b) L = 30 cm (c) P = 2.6 bar (d) λp =985 nm we chose two optimized fibers denoted A and B with struts thickness t=600 nm and inner-diameter d=40 µm and t=1250 nm; d=49 µm (Fig 2). These two fiber designs allow a multi-band FWM. Indeed the signal (fiber A), or both the signal and idler (fiber B) are generated in a different band from the pump. Xenon gas has been chosen because i) no Raman-Scattering can take place in a noble gas, which eliminates the usual main source of noise in fibered photon-pair generation and ii) it exhibits high non-linearity (in the order of 10 −21 m 2 /W at 10 bar). For a given fiber design, pump wavelength, gas pressure and fiber length are three adjustable parameters that can be tuned to access various JSA shapes as can be seen on the simulations in Fig.1. Both single TM or, opposingly, multi-TM can be obtained. Changing the gas pressure impacts the medium dispersion, which results in shifting the JSA and modifying its shape (Fig 1). As a first experimental demonstration in such gas-filled IC fibers, we experimentally reconstruct the JSI for two different fibers (Fig 2) with signal and idler wavelength respectively in the 771 nm and 1550 nm ranges. showing that two very different Schmidt decompositions can be obtained: a quasi factorable state and a correlated state. Figure 2: Fiber cross-section, experimental JSI and corresponding Schmidt decomposition for a 8 tubes IC-fiber and a kagome-IC fiber denoted A and B. In JSI of A the red dashed-lines define the measurement range. The pixelated structure of the JSI of B is due to an insufficient number of measures and will be improved. We have made a new proposal of using multi-dispersion band medium in order to engineer photon-pair time-frequency correlations. For the first time to our knowledge, we implement this technique using gas-filled inhibited-coupling fiber. More configurations are currently being investigated in order to demonstrate the real time tuning possibility in such a medium.
We present a comprehensive numerical investigation of entangled photon pair generation via spontaneous four-wave mixing (SFWM) in hollow-core photonic crystal fibers (HC-PCFs). By analyzing various fiber geometries, dispersion profiles, and anti-resonant characteristics, we identify optimal configurations that enhance photon-pair generation efficiency. Our study highlights the crucial roles of group velocity dispersion engineering, pump parameters, and phase-matching conditions in shaping the joint spectral amplitude (JSA) of the emitted photons. Utilizing gas-filled or evacuated HC-PCFs significantly reduces Raman noise by minimizing field overlap with the glass, while maintaining strong nonlinear interactions. The results reveal practical regimes for improving spectral purity and heralding efficiency. These findings provide practical design guidelines for scalable, low-noise quantum light sources suitable for quantum communication technologies.
The advancement of quantum technologies [1] heavily relies on the efficient generation and manipulation of the photon-pairs. Among the numerous methods available for photon-pairs generation, spontaneous four-wave mixing (SFWM) in photonic crystal fibers [2] has emerged as a promising technique due to its inherent advantages in scalability and integration within existing telecommunication infrastructures. Inhibited-coupling hollow-core photonic crystal fibers (IC-HCPCFs) filled with inert gases provide a unique platform for SFWM-based photon- pairs generation, offering several features including entanglement control [3], integrability into telecommunication networks and also Raman-free generation [4] which minimizes noise and enhances the purity of the generated photon-pairs resulting in record coincidence-to-accidental ratio (CAR) superior to 104[5]. Building upon these advantages, we have recently focused on enhancing the photon-pairs brightness. In our previous work, we demonstrated significant improvements in brightness through optimization of fiber parameters such length, effective area and dispersion [5]–[6] on one hand and the use of a GHz-repetition rate femtosecond laser [7] on another hand to get closer to the MHz-level. One of the remaining parameters to further improve the generation efficiency(η)of IC-HCPCF based photon-pair source, and thereby conclude our investigation, is the pump pulse duration(τp). Sinceηis inversely proportional to the pump pulse duration [8], shorter pulses are expected to yield larger brightness. In this work, we developed a homemade pulse compressor [9] based on a hybrid IC-HCPCF design [10], which was integrated as the first stage of our photon-pair generation set-up as shown in Fig. 1a. By engineering the fiber dispersion and by controlling the optical nonlinearities through the pressure of the filling gas (argon), we achieved a self-compression of input pulses from an ultrashort pulse laser (~280 fs pulse width,1030 nm wavelength, 2 MHz repetition rate) down to ~35 fs. Fig. 1b shows the pulse duration of the compressor output over an input energy range of0.01μJto0.7μJ. The energy transmission efficiency of the compressor was measured to exceed 80%. This compressor enables tunable pulse durations ranging from 280 fs down to 35 fs. As expected, the compression was accompanied by a spectral broadening from 8 nm to 41 nm (gaussian fit FWHM), primarly driven by self-phase modulation (see Fig. 1c). The compressed pulses were subsequently coupled into the photon-pair generation fiber (1 m of tubular lattice HCPCF with a 40 μm core, filled with xenon at 3.2 bar). As expected, when the pulse duration is reduced, the brightness increase scales as1/τp(see Fig. 1d). For the shortest input duration of 35 fs, the brightness was enhanced by a factor of 7.7, which is in agreement with the expected value. Additionally, we observed a slight improvement in the CAR attributed to the increase in the number of coincidences (see Fig. 1e). Finally, the structuring of the spectral pump has led to a change in the joint spectral intensity (JSI) pattern (see inset of Fig. 1d). The implication of this change on the photon-correlation is under investigation.
A fiber-based photon-pair source in the telecom C-band is suitable for quantum information science including quantum communications.Spontaneous four-wave mixing effects are known to create photon pairs that are slightly detuned from the pump wavelength only in the anomalous groupvelocity-dispersion (GVD) regime.Here, we achieve high-quality photon-pair generation slightly detuned from the pump wavelength in the normal GVD regime through a dispersion shifted fiber, for the first time.The photon pairs in C-band exhibit strong temporal correlation with each other and excellent heralded anti-bunching property.This photon-pair generation scheme can be exploited as telecom-band quantum light sources for quantum information applications.A non-classical light source is one of the key elements of quantum information processing systems, and several types of these sources have been investigated, including molecules [1], trapped atoms [2], quantum dots [3], diamond vacancy centers [4], spontaneous parametric down-conversion (SPDC) [5], and spontaneous fourwave mixing (SFWM) [6]. Among these processes, the SPDC and the SFWM processes create quantumcorrelated photon pairs from one and two pump photons, respectively, and both processes require satisfying the energy conservation as well as phase matching [7].Typically, the nonlinear coefficient of SPDC in second-order nonlinear crystals is larger than that of SFWM in amorphous single mode optical fibers as SFWM is a third-order nonlinear process.In the case of several hundred meters long single-mode fibers, however, the SFWM conversion efficiency from pump beam to photon pairs can be similar with that of the SPDC process in nonlinear crystals.In addition, the fiber based photon-pair sources are able to be directly coupled to fiber systems with negligible coupling loss, but waveguide-to-fiber coupling efficiency of a periodically poled SPDC crystal is reported about 50% [8].The SFWM process has been studied intensively for the fiber-based photon generation [6, 9-20] for quantum information applications including quantum key distribution.Photon-pair generation via SFWM is active near the zero group-velocity-dispersion (GVD) wavelength, λ ZGVD , in the anomalous GVD regime [6, 9-15] or normal GVD regime [16][17][18][19][20].In the normal GVD regime, the wavelength of the generated photon pairs is significantly detuned from the pump wavelength.In this case, Raman noise can be avoided, but the generated photon pair do not exhibit telecom-band wavelength together.On the other hand, in the anomalous GVD regime, the wavelength of the generated photon pair is slightly detuned from the pump in the telecom C-band and is strongly power dependent [16].Since the wavelength of the generated pair is sensitive to the λ ZGVD of the generation medium, several types of commercial fibers which have λ ZGVD in the telecom C-band have been investigated as the telecom C-band pair sources.Even if commercial optical fibers have small tolerances in their physical properties, it is common to have sizeable λ ZGVD variance along an optical fiber [21,22].Therefore, the precise measurement of the GVD spectrum is required, but it is often tricky with short length optical fibers.One way to overcome this problem is engineering the dispersion of a commercial fiber by heating and pulling the fiber, but this method is an ambitious research field [19,20,23].On the other hand, if a slightly detuned pair can be generated in the normal GVD regime, the constraint for the λ ZGVD of medium can be weakened, but it has not been reported to the best of our knowledge because phases are mis-matched in this regime due to the Kerr effects of the media.
We present a comprehensive numerical investigation of entangled photon pair generation via spontaneous four-wave mixing (SFWM) in hollow-core photonic crystal fibers (HC-PCFs). By analyzing various fiber geometries, dispersion profiles, and anti-resonant characteristics, we identify optimal configurations that enhance photon-pair generation efficiency. Our study highlights the crucial roles of group velocity dispersion engineering, pump parameters, and phase-matching conditions in shaping the joint spectral amplitude (JSA) of the emitted photons. Utilizing gas-filled or evacuated HC-PCFs significantly reduces Raman noise by minimizing field overlap with the glass, while maintaining strong nonlinear interactions. The results reveal practical regimes for improving spectral purity and heralding efficiency. These findings provide practical design guidelines for scalable, low-noise quantum light sources suitable for quantum communication technologies.
We present a comprehensive numerical investigation of entangled photon pair generation via spontaneous four-wave mixing (SFWM) in hollow-core photonic crystal fibers (HC-PCFs). By analyzing various fiber geometries, dispersion profiles, and anti-resonant characteristics, we identify optimal configurations that enhance photon-pair generation efficiency. Our study highlights the crucial roles of group velocity dispersion engineering, pump parameters, and phase-matching conditions in shaping the joint spectral amplitude (JSA) of the emitted photons. Utilizing gas-filled or evacuated HC-PCFs significantly reduces Raman noise by minimizing field overlap with the glass, while maintaining strong nonlinear interactions. The results reveal practical regimes for improving spectral purity and heralding efficiency. These findings provide practical design guidelines for scalable, low-noise quantum light sources suitable for quantum communication technologies. We bridge fiber design and nonlinear optics to create a predictive model and practical design charts for application-specific quantum light sources.
We demonstrate theoretically and experimentally a high level of control of the four-wave mixing process in an inert gas-filled inhibited-coupling guiding hollow-core photonic crystal fiber. The specific multiple-branch dispersion profile in such fibers allows both correlated and separable bi-photon states to be produced. By controlling the choice of gas and its pressure and the fiber length, we experimentally generate various joint spectral intensity profiles in a stimulated regime that is transferable to the spontaneous regime. The generated profiles may cover both spectrally separable and correlated bi-photon states and feature frequency tuning over tens of THz, demonstrating a large dynamic control that will be very useful when implemented in the spontaneous regime as a photon pair source.