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The Effect of Pump Coherence Length on Stimulated Light Scattering

J. Frank Harmon, Michel Bergeron, P.A. Chernek, Mark E. Rogers, T. Kim, C.L. Stauffer

Published May 21, 1990• 0 citations
OpenAlex

Abstract

We are experimentally investigating Stimulated Brillouin Scattering (SBS) and Stimulated Raman Scattering (SRS) in the transient regime in acetone. While measuring the scattered light as a function of the input energy, we noticed an unexpected “roll-off” in the scattered light as pump energy was increased. Theory predicts as input energy increases scattered energy increases until saturation is reached. We think that the observed roll-off is related to the coherence length of the pump, and we are investigating that relationship.

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Molecular cooperation in the transient regime of stimulated Raman scattering

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The nonlinear regime of stimulated Raman scattering (SRS) may be reached in two ways. The best known is that of depletion of the pump laser as a large number of photons are scattered into the Stokes field. There is, however, another way in which gain saturation can occur, that is, by depletion of the atomic population while the laser remains undepleted. The equations which describe SRS, including damping and population inversion,1 are remarkably similar to those of well-known theories of two-level superfluorescence, and it is possible by analogy to define a delay time τ D for cooperative Raman scattering (CRS). This delay time is inversely proportional to the spontaneous scattering rate, which depends on the pump laser intensity. A sufficient condition for CRS is that the spontaneous Stokes linewidth Γ is very much greater than τ D − 1 . The only other requirement is that there be more laser photons than scatterers, so that τ D is independent of the number of scatterers. The S(1) transition in molecular hydrogen, when excited by a short (≅ 100-ps) laser pulse, provides a possible system for observing pure CRS. Similar studies have been carried out previously2 for Γ ≅ τ D − 1 .

Annual Meeting Optical Society of America•Jan 1, 1985•0 citations

Influence of group-velocity mismatch and inertia of optical nonlinearity on slow-light effects in stimulated inelastic scattering of light

Aleksei M. Zheltikov

Group-velocity mismatch between the pump and Stokes pulses and the inertia of optical nonlinearity are shown to modify scenarios of slow-light evolution of laser pulses accompanying stimulated Raman and Brillouin scattering (SRS and SBS) of light. In the transient regime of SRS and SBS, the inertia of nonlinear polarization of a medium shifts the peak of an amplified Stokes field envelope relative to the input Stokes pulse. This shift is sensitive to the shape of input laser pulses and is controlled by the SRS and/or SBS gain, the damping time of the optical phonon wave, and the delay time between the input pump and Stokes pulses. In the regime where both the inertia of nonlinear polarization of an SRS medium and group-delay effects are significant, stationary modes of the Stokes field may exist in the frame of reference propagating with the group velocity of the pump field. The maximum group delay attainable for such modes of the Stokes field is limited, similar to the steady-state regime, by the ratio of the steady-state SRS gain to the Raman gain bandwidth.

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We have measured the spatial coherence of an initially fully spatially coherent pump laser beam following stimulated Brillouin scattering (SBS) in SF6 gas at 15 atm. Using a simple interferometric technique, we find that the fraction of the diameter of the scattered beam which is spatially coherent decreases with increasing f/No. of the incident 308-nm pump beam. Surprisingly, we also find that the spatial coherence of the scattered beam increases with decreasing pump energy. To our knowledge, these measurements are the first to address the issue of spatial coherence in SBS and point toward an important measure of the fidelity of phase conjugation produced by SBS. The influence of a weak seed beam on the coherence of the phase conjugate beam is also discussed.

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The polarization-related properties of stimulated Brillouin scattering (SBS) processes in long, randomly birefringent, standard optical fibers are examined. Evolution equations for the pump and signal waves, in the presence of both birefringence and SBS, are provided in Jones and Stokes spaces. It is shown that in the undepleted pump regime, the amplification of the SBS signal wave is equivalent to that of a linear medium with polarization-dependent gain. The process is associated with a pair of orthogonal states of polarizations (SOPs) of the signal wave, which undergo maximum and minimum amplification. In long, standard fibers, the Jones vector of the probe SOP which corresponds to maximum amplification is aligned with the complex conjugate of the pump wave Jones vector. The maximum and minimum SBS gain coefficients in such fibers equal two-thirds and one-third of the gain coefficient that is predicted by scalar theory, respectively. The large differential gain of the SBS process gives rise to an effective pulling of the amplified Stokes probe wave SOP, towards that of maximum amplification. Lastly, Stokes wave pulses that are aligned for maximum and minimum amplification experience different group delays, which manifest as polarization-related distortions in SBS slow light setups.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Feb 10, 2011•4 citations

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The equations describing the transfer of intensity from a pump beam simultaneously to forward and backward stimulated scattered beams in an infinite medium are shown to lead to pulsations similar to relaxation oscillations in the scattered intensities. The period of the pulsations is simply related to the gain length for the forward-scattered beam, and may be much longer than the ordinary transient time (related to the damping of material excitations) usually associated with stimulated scattering. Similar oscillations occur for backward scattering alone (stimulated Brillouin scattering) if the scattering medium is finite. In this case the period equals the photon round-trip time in the medium if the latter exceeds the backward gain length. Both phenomena should be observable in scattering from gases such as ${\mathrm{N}}_{2}$ and ${\mathrm{H}}_{2}$ at high pressure, and may also play a role in determining the temporal structure of light scattered from the region of a self-focus in liquids.

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Stimulated Raman scattering spectra: quantum fluctuations and time evolution of linewidth

Владимир Григорьевич Беспалов

Manifestations of quantum fluctuations in stimulated Raman scattering ( SRS ) have been intensively studied lately1. Quantum noise present in spontaneous scattering stimulates fluctuations both in phase and in amplitude characteristics of output Stokes emission. At present statistical properties of amplitude fluctuations are studied in detail and it is shown that in linear transient regime of SRS without pump depletion statistical scatter of Stokes energy Es has negative exponential distribution2. In saturation regime of SRS the amplitude fluctuations are almost suppressed simultaneously with pump depletion. The phase fluctuations manifest both in linear and in nonlinear SRS and produce beam pointing fluctuations3, a change in Stokes emission spectra from pulse to pulse4 and cause soliton appearance in Rayleigh component of SRS5. Phase noise is observed in saturation regime due to relation between phases of Stokes and phonon waves which is preserved in processes of stationary and quasistationary SRS amplification. Spectrum phase fluctuations manifest as fine structure of SRS spectrum4, fluctuations of average Stokes frequency and Stokes linewidth fluctuations. The evolution of phase fluctuations in time is determined by the nature of spontaneous scattering and polarization of Raman media and is of great interest as one can follow its development from vacuum modes level to saturation regime. However up to now this problem has not been studied yet.

17th Congress of the International Commission for Optics: Optics for Science and New Technology•Sep 1, 1996•0 citations
We are experimentally investigating Stimulated Brillouin Scattering (SBS) and Stimulated Raman Scattering (SRS) in the transient regime in acetone. While measuring the scattered light as a function of the input energy, we noticed an unexpected “roll-off” in the scattered light as pump energy was increased. Theory predicts as input energy increases scattered energy increases until saturation is reached. We think that the observed roll-off is related to the coherence length of the pump, and we are investigating that relationship.
The nonlinear regime of stimulated Raman scattering (SRS) may be reached in two ways. The best known is that of depletion of the pump laser as a large number of photons are scattered into the Stokes field. There is, however, another way in which gain saturation can occur, that is, by depletion of the atomic population while the laser remains undepleted. The equations which describe SRS, including damping and population inversion,1 are remarkably similar to those of well-known theories of two-level superfluorescence, and it is possible by analogy to define a delay time τ D for cooperative Raman scattering (CRS). This delay time is inversely proportional to the spontaneous scattering rate, which depends on the pump laser intensity. A sufficient condition for CRS is that the spontaneous Stokes linewidth Γ is very much greater than τ D − 1 . The only other requirement is that there be more laser photons than scatterers, so that τ D is independent of the number of scatterers. The S(1) transition in molecular hydrogen, when excited by a short (≅ 100-ps) laser pulse, provides a possible system for observing pure CRS. Similar studies have been carried out previously2 for Γ ≅ τ D − 1 .
Group-velocity mismatch between the pump and Stokes pulses and the inertia of optical nonlinearity are shown to modify scenarios of slow-light evolution of laser pulses accompanying stimulated Raman and Brillouin scattering (SRS and SBS) of light. In the transient regime of SRS and SBS, the inertia of nonlinear polarization of a medium shifts the peak of an amplified Stokes field envelope relative to the input Stokes pulse. This shift is sensitive to the shape of input laser pulses and is controlled by the SRS and/or SBS gain, the damping time of the optical phonon wave, and the delay time between the input pump and Stokes pulses. In the regime where both the inertia of nonlinear polarization of an SRS medium and group-delay effects are significant, stationary modes of the Stokes field may exist in the frame of reference propagating with the group velocity of the pump field. The maximum group delay attainable for such modes of the Stokes field is limited, similar to the steady-state regime, by the ratio of the steady-state SRS gain to the Raman gain bandwidth.
We have measured the spatial coherence of an initially fully spatially coherent pump laser beam following stimulated Brillouin scattering (SBS) in SF6 gas at 15 atm. Using a simple interferometric technique, we find that the fraction of the diameter of the scattered beam which is spatially coherent decreases with increasing f/No. of the incident 308-nm pump beam. Surprisingly, we also find that the spatial coherence of the scattered beam increases with decreasing pump energy. To our knowledge, these measurements are the first to address the issue of spatial coherence in SBS and point toward an important measure of the fidelity of phase conjugation produced by SBS. The influence of a weak seed beam on the coherence of the phase conjugate beam is also discussed.
The polarization-related properties of stimulated Brillouin scattering (SBS) processes in long, randomly birefringent, standard optical fibers are examined. Evolution equations for the pump and signal waves, in the presence of both birefringence and SBS, are provided in Jones and Stokes spaces. It is shown that in the undepleted pump regime, the amplification of the SBS signal wave is equivalent to that of a linear medium with polarization-dependent gain. The process is associated with a pair of orthogonal states of polarizations (SOPs) of the signal wave, which undergo maximum and minimum amplification. In long, standard fibers, the Jones vector of the probe SOP which corresponds to maximum amplification is aligned with the complex conjugate of the pump wave Jones vector. The maximum and minimum SBS gain coefficients in such fibers equal two-thirds and one-third of the gain coefficient that is predicted by scalar theory, respectively. The large differential gain of the SBS process gives rise to an effective pulling of the amplified Stokes probe wave SOP, towards that of maximum amplification. Lastly, Stokes wave pulses that are aligned for maximum and minimum amplification experience different group delays, which manifest as polarization-related distortions in SBS slow light setups.
The equations describing the transfer of intensity from a pump beam simultaneously to forward and backward stimulated scattered beams in an infinite medium are shown to lead to pulsations similar to relaxation oscillations in the scattered intensities. The period of the pulsations is simply related to the gain length for the forward-scattered beam, and may be much longer than the ordinary transient time (related to the damping of material excitations) usually associated with stimulated scattering. Similar oscillations occur for backward scattering alone (stimulated Brillouin scattering) if the scattering medium is finite. In this case the period equals the photon round-trip time in the medium if the latter exceeds the backward gain length. Both phenomena should be observable in scattering from gases such as N2{\mathrm{N}}_{2}N2​ and H2{\mathrm{H}}_{2}H2​ at high pressure, and may also play a role in determining the temporal structure of light scattered from the region of a self-focus in liquids.
Manifestations of quantum fluctuations in stimulated Raman scattering ( SRS ) have been intensively studied lately1. Quantum noise present in spontaneous scattering stimulates fluctuations both in phase and in amplitude characteristics of output Stokes emission. At present statistical properties of amplitude fluctuations are studied in detail and it is shown that in linear transient regime of SRS without pump depletion statistical scatter of Stokes energy Es has negative exponential distribution2. In saturation regime of SRS the amplitude fluctuations are almost suppressed simultaneously with pump depletion. The phase fluctuations manifest both in linear and in nonlinear SRS and produce beam pointing fluctuations3, a change in Stokes emission spectra from pulse to pulse4 and cause soliton appearance in Rayleigh component of SRS5. Phase noise is observed in saturation regime due to relation between phases of Stokes and phonon waves which is preserved in processes of stationary and quasistationary SRS amplification. Spectrum phase fluctuations manifest as fine structure of SRS spectrum4, fluctuations of average Stokes frequency and Stokes linewidth fluctuations. The evolution of phase fluctuations in time is determined by the nature of spontaneous scattering and polarization of Raman media and is of great interest as one can follow its development from vacuum modes level to saturation regime. However up to now this problem has not been studied yet.