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Chinese Journal of Physics

Polarization Correlations of Radiation from Electron-Impact Excited Atoms

Wen‐Yu Cheng, Keh‐Ning Huang

Published Feb 1, 1994• 1 citation
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Physical Review Letters•Aug 3, 1992•15 citations
Polarized radiation following electron impact.---If a unidirectional beam of electrons, of velocity slightly in excess of the resonance potential, is projected through a vapor at a very low pressure so that effects due to atomic collision and resonance radiation are negligible, and in the absence of an applied field and resulting Larmor precession, there is reason to suspect that the radiation emitted perpendicular to the electron beam should be partially polarized, especially for lines corresponding to $\ensuremath{\Delta}j=1$.Polarization in mercury and sodium vapor.---Experiment showed a polarization of about 30 percent for $\ensuremath{\lambda}2537$ with the greatest intensity of the electrical vibration having a direction perpendicular to the electron beam. No polarization was detected for the unresolved sodium D-lines, confirming the recent observation of Kossel and Gerthsen.Polarization in mercury with field of 3 gauss.---A field parallel to the electron beam produced no effect. With the field perpendicular to the beam the radiation along the field was unpolarized while that perpendicular to the field was reduced in polarization to 13 percent. These results suggest that the atom radiates with the same distribution of polarization and intensity as in zero field but with the atom rotated through an angle determined by the time of excitation and the precessional velocity.
The coherence analysis technique has been used to determine the state of polarizatitn of 228.8 nm radiation emitted by cadmium atoms excited to 51P1 state by electron impact. Data have been obtained for incident electron energy of 100 eV for scattering angles in the range from 10° to 40°. Reduced Stokes parameters and electron impact coherence parameters (EICP), characterizing the state of the excited atoms immediately after the collision, have been extracted from the measurements and compared with results of relativistic distorted-wave approximation calculations. Theoretical predictions are in good qualitative agreement with experimental values.
The relaxation rates of the monopole, magnetic dipole, and electric quadrupole moments have been determined for the 31{3}^{1}31P state of helium excited by electron impact, The data are determined from atomic lifetimes using linear and circular polarization analyzed radiation with the electron-photon delayed coincidence technique. This has permitted the direct observation of the time dependence of all the off-diagonal elements of the density matrix of the excited state. The implications for atomic state information determined from polarization and angular correlation methods are indicated.