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Physica B+C

Frequency dependence of the polarization of radiation emitted by polarized atoms

Gerard Nienhuis

Published Feb 1, 1976• 1 citation
Publisher
DOI
10.1016/0378-4363(76)90076-0

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Optics and Spectroscopy•Jan 1, 2021•0 citations
Coherent backscattering of pulsed radiation emitted by optically dense atomic ensembles is considered. The diagrammatic technique is used for deriving analytic expressions for correlation functions of scattered light, which make it possible to take into account all main factors affecting the dynamics of the process, including the hyperfine and Zeeman structure of the ground and first excited states of atoms, polarization of probe radiation, the actual shape and size of an atomic cloud, its spatial inhomogeneity, motion of atoms, and angular-momentum polarization of atoms. On the basis of these relations, the time dependence of the total intensity and the dependence of enhancement factor of backscattered light on the pulse duration, type of polarization of the polarization system of observation, optical thickness of the scattering medium, and the carrier frequency of the pulse are investigated. The calculations are performed for an ensemble of rubidium-85 atoms cooled in magnetooptical traps.
In the absence of incoherent relaxation processes, the emission, absorption, and transport of resonant radiation by an extended medium are all cooperative processes in which the medium participates as a whole. Such radiative processes depend sensitively on the geometry of the source, on its size and density, and on the interplay of electric polarization resonances with the ambient electromagnetic field. By making a succession of simple approximations, we reduce the radiative interaction problem to one of solving a linear integral equation for the time-dependent polarization of the radiating medium. For the example of one-dimensional geometry, we show that the polarization possesses a sequence of exponentially decaying eigenmodes that oscillate at frequencies slightly shifted from that of the fundamental resonance. Only a few of these modes, for any radiating medium, are strongly coupled to the electromagnetic field, and thereby radiate efficiently. All of the other modes, infinitely many of them, are found to radiate quite slowly, or not at all. We consider in detail the radiation emitted by an arbitrary initial polarization distribution when the electromagnetic field is initially empty. Analytical and numerical results are presented for the time-dependent fields that follow from a wide variety of initial excitations. A locally oscillatory exchange of energy is found to take place between the electric and polarization fields, which gives rise to a ringing of the radiated intensity. The spectra of the emitted light are shown accordingly to be complex in structure, and to have a frequency gap which becomes independent of the size of the medium and its initial polarization distribution for media that are sufficiently large. The gap is caused by the interference and interaction of oppositely propagating excitations.
Abstract The nonlinear optical effect of free polarization decay (FPD) in an ultrathin gas cell, the inner thickness of which is less than or on the order of the wavelength of the exciting monochromatic laser radiation propagating orthogonally to the plane-parallel walls of this cell, is studied theoretically. The considered coherent FPD signal is emitted immediately after abrupt termination of this comparatively weak stationary radiation. The sub-Doppler resonances appearing at the central frequencies of the studied quantum transitions in the FPD intensity and energy spectra due to the transit-time relaxation of atoms in the gas cell are detected and studied. It is shown that these resonances and the FPD dynamics strongly depend on the ratio between the inner thickness of the gas cell and the wavelength of the exciting monochromatic radiation. The narrow high–contrast sub-Doppler resonances of FPD observed and studied in a linear optical regime can be used in atomic (molecular) high-resolution spectroscopy and as references for compact frequency standards.