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On the universality of the fluctuation-dissipation ratio in non-equilibrium critical dynamics

Malte Henkel, Gunter Markus Schutz

Published Jan 1, 2004• 27 citations
OpenAlex

Abstract

The two-time non-equilibrium correlation and response functions in 1D kinetic classical spin systems with non-conserved dynamics and quenched to their zero-temperature critical point are studied. The exact solution of the kinetic Ising model with Glauber dynamics for a wide class of initial states allows for an explicit test of the universality of the non-equilibrium limit fluctuation-dissipation ratio X-infinity. It is shown that the value of X-infinity depends on whether the initial state has finitely many domain walls or not and thus two distinct dynamic universality classes can be identified in this model. Generic ID kinetic spin systems with non-conserved dynamics fall into the same universality classes as the kinetic Glauber-Ising model provided the dynamics is invariant under the C-symmetry of simultaneous spin and magnetic-field reversal. While C-symmetry is satisfied for magnetic systems, it need not be for lattice gases which may therefore display hitherto unexplored types of non-universal kinetics.

Related papers

On the universality of the fluctuation–dissipation ratio in non-equilibrium critical dynamics

Malte Henkel, Gunter Markus Schutz

The two-time nonequilibrium correlation and response functions in 1D kinetic classical spin systems with non-conserved dynamics and quenched to their zero-temperature critical point are studied. The exact solution of the kinetic Ising model with Glauber dynamics for a wide class of initial states allows for an explicit test of the universality of the non-equilibrium limit fluctuation-dissipation ratio X_{\infty}. It is shown that the value of X_{\infty} depends on whether the initial state has finitely many domain walls or not and thus two distinct dynamic universality classes can be identified in this model. Generic 1D kinetic spin systems with non-conserved dynamics fall into the same universality classes as the kinetic Glauber-Ising model provided the dynamics is invariant under the C-symmetry of simultaneous spin and magnetic-field reversal. While C-symmetry is satisfied for magnetic systems, it need not be for lattice gases which may therefore display hitherto unexplored types of non-universal kinetics.

arXiv:cond-mat/0308466•Journal of Physics A Mathematical and General•Jan 6, 2004•36 citations

Ageing and non-equilibrium critical phenomena in Monte Carlo simulations

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It is considered the non-equilibrium critical evolution of statistical systems which displays some features, such as ageing and violation of the fluctuation-dissipation theorem. We review here some theoretical results of computations that have been obtained in recent years for universal quantities, such as the exponents determining the scaling behaviour of dynamic response and correlation functions and the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics, with particular focus on the 3D pure and diluted Ising models with Glauber dynamics. We analyse an influence of critical fluctuations, different non-equilibrium initial states and presence of nonmagnetic impurities in spin systems on two-time dependence of correlation and response functions on characteristic time variables as waiting time t w and time of observation t – t w with t > t w . We discuss the obtained values of non-equilibrium exponents for autocorrelation and response functions and values of the universal long-time limit of the fluctuation-dissipation ratio X ∞ . Analysis of simulation results show that the insertion of disorder leads to new values of X ∞ with X ∞ diluted > X ∞ pure .

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Response of non-equilibrium systems at criticality: ferromagnetic models in dimension two and above

Claude Godrèche, J. M. Luck

We study the dynamics of ferromagnetic spin systems quenched from infinite temperature to their critical point. We perform an exact analysis of the spherical model in any dimension D >2 and numerical simulations on the two-dimensional Ising model. These systems are shown to be ageing in the long-time regime, i.e. their two-time autocorrelation and response functions, and associated fluctuation-dissipation ratio, are non-trivial scaling functions of both time variables. We show in particular that, for 1<< s (waiting time) << t (observation time), the fluctuation-dissipation ratio possesses a non-trivial limit value X ∞ , which appears as a dimensionless amplitude ratio, and is therefore a novel universal characteristic of non-equilibrium critical dynamics. For the spherical model, we obtain X ∞ = 1-2/ D for 2< D <4 and X ∞ = ½ for D >4 (mean-field regime). For the two-dimensional Ising model we measure X ∞ ≈0.26±0.01.

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Non-equilibrium critical dynamics

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We now begin our exposition of universal dynamic scaling behavior that emerges under non-equilibrium conditions. We are mainly concerned with the relaxational models A and B here, but also touch on other dynamic universality classes. First, we consider non-equilibrium critical relaxation from a disordered initial state, and compute the associated universal scaling exponents within the dynamic renormalization group framework. Related phenomena in the early-time regime, prior to reaching temporally translationally invariant asymptotics, are ‘aging’ and a non-equilibrium fluctuation-dissipation ratio, both of which have enjoyed prominence in the literature on ‘glassy’ kinetics. In this context, we derive the critical initial slip exponent for the order parameter, and briefly discuss interesting persistence properties. Second, we explore the long-time scaling laws in phase ordering kinetics and coarsening for the relaxational models, following a fast temperature ‘quench’ into the ordered phase, in systems with either non-conserved or conserved order parameters. Aside from a few explicit computations in the spherical model limit (wherein the number of order parameter components n → ∞), we largely employ phenomenological considerations and scaling theory, stressing the importance of topological defects for energy dissipation during coarsening. Next we address the question how violations of Einstein's relation that links relaxation coefficients and noise correlations might affect the asymptotic dynamic critical scaling behavior. Whereas in systems with non-conserved order parameter typically the equilibrium scaling laws are recovered in the vicinity of the critical point, in contrast genuinely novel universality classes may emerge in the case of a conserved parameter, provided it is driven out of equilibrium in a spatially anisotropic fashion.

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We investigate the non-equilibrium critical evolution of statistical systems and describe of its some features, such as aging and violation of the fluctuation-dissipation theorem. We consider some theoretical results of computations for universal quantities that have been obtained in recent years, such as the exponents determining the scaling behavior of dynamic response and correlation functions and the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics. We derive our original Monte Carlo simulation results for 3D pure and diluted Ising models with Glauber and Metropolis dynamics. For these models, we analyze the influence of critical fluctuations, different non-equilibrium initial states, and the presence of nonmagnetic impurities on the two-time dependence of correlation and response functions on characteristic time variables, such as waiting time |$t_{\rm w}$| and time of observation |$t - t_{\rm w}$| with |$t>t_{\rm w}$|⁠. We discuss the obtained values of the non-equilibrium exponents for the autocorrelation and response functions and values of the universal long-time limit of the fluctuation-dissipation ratio |$X^{\infty }$|⁠. Our simulation results demonstrate that the insertion of disorder leads to new values of |$X^{\infty }$| with |$X_{\rm diluted}^{\infty }>X_{\rm pure}^{\infty }$|⁠.

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Relaxation phenomena at criticality

Andrea Gambassi

The collective behaviour of statistical systems close to critical points is characterized by an extremely slow dynamics which, in the thermodynamic limit, eventually prevents them from relaxing to an equilibrium state after a change in the thermodynamic control parameters. The non-equilibrium evolution following this change displays some of the features typically observed in glassy materials, such as ageing, and it can be monitored via dynamic susceptibilities and correlation functions of the order parameter, the scaling behaviour of which is characterized by universal exponents, scaling functions, and amplitude ratios. This universality allows one to calculate these quantities in suitable simplified models and field-theoretical methods are a natural and viable approach for this analysis. In addition, if a statistical system is spatially confined, universal Casimir-like forces acting on the confining surfaces emerge and they build up in time when the temperature of the system is tuned to its critical value. We review here some of the theoretical results that have been obtained in recent years for universal quantities, such as the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics, with particular focus on the Ising model with Glauber dynamics in the bulk. The non-equilibrium dynamics of the Casimir force acting in a film is discussed within the Gaussian model.

•Jan 1, 2008•24 citations
The two-time non-equilibrium correlation and response functions in 1D kinetic classical spin systems with non-conserved dynamics and quenched to their zero-temperature critical point are studied. The exact solution of the kinetic Ising model with Glauber dynamics for a wide class of initial states allows for an explicit test of the universality of the non-equilibrium limit fluctuation-dissipation ratio X-infinity. It is shown that the value of X-infinity depends on whether the initial state has finitely many domain walls or not and thus two distinct dynamic universality classes can be identified in this model. Generic ID kinetic spin systems with non-conserved dynamics fall into the same universality classes as the kinetic Glauber-Ising model provided the dynamics is invariant under the C-symmetry of simultaneous spin and magnetic-field reversal. While C-symmetry is satisfied for magnetic systems, it need not be for lattice gases which may therefore display hitherto unexplored types of non-universal kinetics.
The two-time nonequilibrium correlation and response functions in 1D kinetic classical spin systems with non-conserved dynamics and quenched to their zero-temperature critical point are studied. The exact solution of the kinetic Ising model with Glauber dynamics for a wide class of initial states allows for an explicit test of the universality of the non-equilibrium limit fluctuation-dissipation ratio X_{\infty}. It is shown that the value of X_{\infty} depends on whether the initial state has finitely many domain walls or not and thus two distinct dynamic universality classes can be identified in this model. Generic 1D kinetic spin systems with non-conserved dynamics fall into the same universality classes as the kinetic Glauber-Ising model provided the dynamics is invariant under the C-symmetry of simultaneous spin and magnetic-field reversal. While C-symmetry is satisfied for magnetic systems, it need not be for lattice gases which may therefore display hitherto unexplored types of non-universal kinetics.
It is considered the non-equilibrium critical evolution of statistical systems which displays some features, such as ageing and violation of the fluctuation-dissipation theorem. We review here some theoretical results of computations that have been obtained in recent years for universal quantities, such as the exponents determining the scaling behaviour of dynamic response and correlation functions and the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics, with particular focus on the 3D pure and diluted Ising models with Glauber dynamics. We analyse an influence of critical fluctuations, different non-equilibrium initial states and presence of nonmagnetic impurities in spin systems on two-time dependence of correlation and response functions on characteristic time variables as waiting time t w and time of observation t – t w with t > t w . We discuss the obtained values of non-equilibrium exponents for autocorrelation and response functions and values of the universal long-time limit of the fluctuation-dissipation ratio X ∞ . Analysis of simulation results show that the insertion of disorder leads to new values of X ∞ with X ∞ diluted > X ∞ pure .
We study the dynamics of ferromagnetic spin systems quenched from infinite temperature to their critical point. We perform an exact analysis of the spherical model in any dimension D >2 and numerical simulations on the two-dimensional Ising model. These systems are shown to be ageing in the long-time regime, i.e. their two-time autocorrelation and response functions, and associated fluctuation-dissipation ratio, are non-trivial scaling functions of both time variables. We show in particular that, for 1<< s (waiting time) << t (observation time), the fluctuation-dissipation ratio possesses a non-trivial limit value X ∞ , which appears as a dimensionless amplitude ratio, and is therefore a novel universal characteristic of non-equilibrium critical dynamics. For the spherical model, we obtain X ∞ = 1-2/ D for 2< D <4 and X ∞ = ½ for D >4 (mean-field regime). For the two-dimensional Ising model we measure X ∞ ≈0.26±0.01.
We now begin our exposition of universal dynamic scaling behavior that emerges under non-equilibrium conditions. We are mainly concerned with the relaxational models A and B here, but also touch on other dynamic universality classes. First, we consider non-equilibrium critical relaxation from a disordered initial state, and compute the associated universal scaling exponents within the dynamic renormalization group framework. Related phenomena in the early-time regime, prior to reaching temporally translationally invariant asymptotics, are ‘aging’ and a non-equilibrium fluctuation-dissipation ratio, both of which have enjoyed prominence in the literature on ‘glassy’ kinetics. In this context, we derive the critical initial slip exponent for the order parameter, and briefly discuss interesting persistence properties. Second, we explore the long-time scaling laws in phase ordering kinetics and coarsening for the relaxational models, following a fast temperature ‘quench’ into the ordered phase, in systems with either non-conserved or conserved order parameters. Aside from a few explicit computations in the spherical model limit (wherein the number of order parameter components n → ∞), we largely employ phenomenological considerations and scaling theory, stressing the importance of topological defects for energy dissipation during coarsening. Next we address the question how violations of Einstein's relation that links relaxation coefficients and noise correlations might affect the asymptotic dynamic critical scaling behavior. Whereas in systems with non-conserved order parameter typically the equilibrium scaling laws are recovered in the vicinity of the critical point, in contrast genuinely novel universality classes may emerge in the case of a conserved parameter, provided it is driven out of equilibrium in a spatially anisotropic fashion.
We investigate the non-equilibrium critical evolution of statistical systems and describe of its some features, such as aging and violation of the fluctuation-dissipation theorem. We consider some theoretical results of computations for universal quantities that have been obtained in recent years, such as the exponents determining the scaling behavior of dynamic response and correlation functions and the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics. We derive our original Monte Carlo simulation results for 3D pure and diluted Ising models with Glauber and Metropolis dynamics. For these models, we analyze the influence of critical fluctuations, different non-equilibrium initial states, and the presence of nonmagnetic impurities on the two-time dependence of correlation and response functions on characteristic time variables, such as waiting time |twt_{\rm w}tw​| and time of observation |t−twt - t_{\rm w}t−tw​| with |t>twt>t_{\rm w}t>tw​|⁠. We discuss the obtained values of the non-equilibrium exponents for the autocorrelation and response functions and values of the universal long-time limit of the fluctuation-dissipation ratio |X∞X^{\infty }X∞|⁠. Our simulation results demonstrate that the insertion of disorder leads to new values of |X∞X^{\infty }X∞| with |Xdiluted∞>Xpure∞X_{\rm diluted}^{\infty }>X_{\rm pure}^{\infty }Xdiluted∞​>Xpure∞​|⁠.
The collective behaviour of statistical systems close to critical points is characterized by an extremely slow dynamics which, in the thermodynamic limit, eventually prevents them from relaxing to an equilibrium state after a change in the thermodynamic control parameters. The non-equilibrium evolution following this change displays some of the features typically observed in glassy materials, such as ageing, and it can be monitored via dynamic susceptibilities and correlation functions of the order parameter, the scaling behaviour of which is characterized by universal exponents, scaling functions, and amplitude ratios. This universality allows one to calculate these quantities in suitable simplified models and field-theoretical methods are a natural and viable approach for this analysis. In addition, if a statistical system is spatially confined, universal Casimir-like forces acting on the confining surfaces emerge and they build up in time when the temperature of the system is tuned to its critical value. We review here some of the theoretical results that have been obtained in recent years for universal quantities, such as the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics, with particular focus on the Ising model with Glauber dynamics in the bulk. The non-equilibrium dynamics of the Casimir force acting in a film is discussed within the Gaussian model.