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Tunable optical parametric generator based on the pump spatial walk-off

Cavanna, A., Just, F., Sharapova, P., Taheri, M., Gerd Leuchs, Chekhova, M.

Published Jan 1, 2016• 7 citations
OpenAlex

Abstract

We suggest a novel optical parametric generator (OPG) in which one of the downconverted beams is spontaneously generated along the Poynting vector of the pump beam. In this configuration, the generation takes advantage of the walk-off of the extraordinary pump, rather than being degraded by it. As a result, the generated signal and idler beams are bright due to a high conversion efficiency, spatially nearly single mode due to the preferred direction of the Poynting vector, tunable over a wide range of wavelengths and broadband. The two beams are also correlated in frequency and in the photon number per pulse. Furthermore, due to their thermal statistics, these beams can be used as a pump to efficiently generate other nonlinear processes. (C) 2016 Optical Society of America

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Aug 1, 2008•3 citations
We suggest a novel optical parametric generator (OPG) in which one of the downconverted beams is spontaneously generated along the Poynting vector of the pump beam. In this configuration, the generation takes advantage of the walk-off of the extraordinary pump, rather than being degraded by it. As a result, the generated signal and idler beams are bright due to a high conversion efficiency, spatially nearly single mode due to the preferred direction of the Poynting vector, tunable over a wide range of wavelengths and broadband. The two beams are also correlated in frequency and in the photon number per pulse. Furthermore, due to their thermal statistics, these beams can be used as a pump to efficiently generate other nonlinear processes. (C) 2016 Optical Society of America
We suggest a novel optical parametric generator (OPG) in which one of the downconverted beams is spontaneously generated along the Poynting vector of the pump beam. In this configuration, the generation takes advantage of the walk-off of the extraordinary pump, rather than being degraded by it. As a result, the generated signal and idler beams are bright due to a high conversion efficiency, spatially nearly single mode due to the preferred direction of the Poynting vector, tunable over a wide range of wavelengths and broadband. The two beams are also correlated in frequency and in the photon number per pulse. Furthermore, due to their thermal statistics, these beams can be used as a pump to efficiently generate other nonlinear processes.
Walk-off effects, originating from the difference between the group and phase velocities, limit the efficiency of nonlinear optical interactions. While transverse walk-off can be eliminated by proper medium engineering, longitudinal walk-off is harder to avoid. In particular, ultrafast twin-beam generation via pulsed parametric down-conversion and four-wave mixing is only possible in short crystals or fibres. Here we show that in high-gain parametric down-conversion, one can overcome the destructive role of both effects and even turn them into useful tools for shaping the emission. In our experiment, one of the twin beams is emitted along the pump Poynting vector or its group velocity matches that of the pump. The result is markedly enhanced generation of both twin beams, with the simultaneous narrowing of angular and frequency spectrum. The effect will enable efficient generation of ultrafast twin photons and beams in cavities, waveguides and whispering-gallery mode resonators.
Summary form only given. The efficiency and engineering capabilities afforded by parametric processes in second-order [χ(2)] nonlinear media have tremendously benefitted from periodic poling technologies in ferroelectric materials such as LiNbO3, nowadays routinely exploited in optical parametric generators, amplifiers and oscillators, as well as high brightness sources of entangled photons [1, 2]. Nonlinear photonic crystals (NPCs) implemented by periodic poling, have also attracted a great deal of attention, since they provide additional degrees of freedom to coherently shape the angular and spectral response of parametric devices [3-4]. Following the first demonstration of coherently coupled twin-beam optical parametric generation (OPG) in a χ(2)NPC [4], a number of studies investigated their potential for classical and quantum applications [5-6].Here we demonstrate twin beam OPG in a hexagonally poled LiTaO3 NPC pumped at 527 nm and generating signal and idlers in the near-infrared (λS~800 nm) and telecom (λI~1550nm) ranges. We perform a complete spectral and angular mapping of its OPG response for different pump pulse energies (10 - 100μJ) and incidence angles (-2.5 to 2.5°), finding very good agreement between predictions (Fig. 1b-c) and experiments
Spontaneous parametric down-conversion (SPDC) is one of the most important sources for entangled or correlated photon pairs, which are the foundation of the emerging fields of quantum-optical imaging and spectroscopy. Using periodically poled materials as an SPDC-source allows broad emission spectra in widely tunable wavelength ranges in an efficient and walk-off-free process. For applications that employ nonlinear interference setups, maximum interferometric contrast is only achieved when signal and idler modes are overlapped precisely in the second crystal. Thus, accurate knowledge of the spectral-angular characteristic of SPDC is crucial for designing such devices.
The OAM of light provides a new resource to explore quantum physics in a d-dimensional Hilbert space, beyond the two dimensional Hilbert space generated by the polarization state of the photons. The implementation of such a ddimensional quantum channel requires the generation of arbitrary engineered entangled states, thus controlling the OAM of the entangled photons is of paramount importance for many applications. Here we address the orbital angular momentum, i.e. the spatial shape, of photons generated in SPDC in non collinear geometries, when the interacting waves can exhibit Poynting vector walk off. The spatial shape depends on the interplay between the state ellipticity caused by the nonlinear geometry, and the Poynting vector walk off. The importance of both effects is dictated by the relationship between three characteristics lengths: the length of the nonlinear crystal, the walk off length and the non collinear length. The effects described here are relevant to current experiments, especially for the implementation of quantum information protocols based on spatially encoded information. Finally, the consideration of new geometries for SPDC, more specifically, highly non collinear configurations, will lead us to the discussion of the relationship between the OAM of the classical beam that pumps the nonlinear crystal, and the quantum OAM of the down converted photons. Regarding experimental measurements related to this issue, it is of great importance to make a clear distinction between the measurement of locally paraxial light beams in a suitable transverse frame, and the description of the global down conversion process, which is not necessarily paraxial.
Photons produced in the process of spontaneous parametric down-conversion (SPDC) are typically entangled in multiple degrees of freedom. Although polarization is often the parameter of interest, the presence of spectral or spatial entanglement can complicate experiments, either by reducing the visibility of certain interference effects or by reducing collection efficiency. Several recent works have shown that the collection efficiency can be improved by focusing the pump beam. This approach has the added benefit of increasing the bandwidths of the emitted photons. We show that, in the case of type II SPDC, a focused pump can result in different spatial profiles for the signal and idler. If the crystal is configured for emission of polarization-entangled photon pairs, this effect will reduce the fidelity of that entanglement. Moreover, this spatial asymmetry leads to different spectral profiles for the two photons, even when the pump is monochromatic. The spectral and spatial asymmetries can be attributed to the difference in the angular dispersion (walk-off) of the two polarizations, along with a strong correlation between wavelength and emission direction. We also examine the link between spatial entanglement and single-mode coupling efficiency. We find that efficiency is maximized when spatial entanglement can be eliminated. For the case in which walk-off does not play a role, this can be accomplished by properly focusing the pump.