Photon correlations for colloidal nanocrystals and their clusters
O. A. Shcherbina, G. A. Shcherbina, Mathieu Manceau, Stefano Vezzoli, Luigi Carbone, Massimo De Vittorio, Alberto Bramati, E. Giacobino, Maria V. Chekhova, Gerd Leuchs
Images of semiconductor "dot-in-rods" and their small clusters are studied by measuring the second-order correlation function with a spatially resolving intensified CCD camera. This measurement allows one to distinguish between a single dot and a cluster and, to a certain extent, to estimate the number of dots in a cluster. A more advanced measurement is proposed, based on higher-order correlations, enabling more accurate determination of the number of dots in a small cluster. Nonclassical features of the light emitted by such a cluster are analyzed.
Images of semiconductor "dot-in-rods" and their small clusters are studied by measuring the second-order correlation function with a spatially resolving intensified CCD camera. This measurement allows one to distinguish between a single dot and a cluster and, to a certain extent, to estimate the number of dots in a cluster. A more advanced measurement is proposed, based on higher-order correlations, enabling more accurate determination of the number of dots in a small cluster. Nonclassical features of the light emitted by such a cluster are analyzed.
Images of semiconductor "dot-in-rods" and their small clusters are studied by measuring the second-order correlation function with a spatially resolving intensified CCD camera. This measurement allows one to distinguish between a single dot and a cluster and, to a certain extent, to estimate the number of dots in a cluster. A more advanced measurement is proposed, based on higher-order correlations, enabling more accurate determination of the number of dots in a small cluster. Nonclassical features of the light emitted by such a cluster are analyzed.
We consider nonclassical features of light emitted by clusters of room-temperature single-photon emitters. As signatures of nonclassicality, we discuss violation of inequalities for normalized correlation functions of orders higher than two. These conditions are stronger than higher-order antibunching, i.e., higher-order normalized correlation functions being less than unity. In experiment, we observe third-order nonclassicality as well as second-, third-, and fourth-order antibunching for clusters of 1 to 20 colloidal CdSe/CdS dot-in-rods.
We study nonclassical features of multiphoton light emitted by clusters of single-photon emitters. As signatures of nonclassicality, we use violation of inequalities for normalized correlation functions of different orders or the probabilities of multiphoton detection. In particular, for clusters of 2–14 colloidal CdSe/CdS dot-in-rods we observe antibunching and nonclassicality of up to the fourth-order. Surprisingly, violation of certain classical inequalities gets even more pronounced for larger clusters.
We investigate the intensity correlation properties of single photons emitted from an optically excited single semiconductor quantum dot. The second order temporal coherence function of the photons emitted at various wavelengths is measured as a function of the excitation power. We show experimentally and theoretically that a quantum dot is not only a source of nonclassically correlated monochromatic photons but is also a source of multicolor photons with tunable correlation properties. We found that the emitted photon statistics can be varied by the excitation rate from a sub-Poissonian one, where the photons are temporally antibunched, to super-Poissonian, where they are temporally bunched.
Cameras with single-photon sensitivities can be used to measure the spatial correlations between the photon-pairs that are produced by parametric down-conversion. Even when pumped by a single-mode laser, the signal and idler photons are typically distributed over several thousand spatial modes yet strongly correlated with each other in their position and anti-correlated in their transverse momentum. These spatial correlations enable applications in imaging, sensing, communication, and optical processing. Here we show that, using a photon-number resolving camera, spatial correlations can be observed after only a few 10s of seconds of measurement time, thereby demonstrating comparable performance with previous single photon sensitive camera technologies but with the additional capability to resolve photon-number. Consequently, these photon-number resolving technologies are likely to find wide use in quantum, low-light, imaging systems.
Imaging is the estimation of the spatial distribution of a physical object by measuring the optical radiation it emits, or by making use of an optical wave that interacts with the object, via reflection or transmission, for example, before being measured by a detector. The resolution of an imaging system is limited by the inability to localize the optical field at points of the object. Under otherwise ideal conditions, resolution is limited by diffraction. The sensitivity of an imaging system is limited by the uncertainty in the measurement. Under ideal conditions, this is determined by photon noise, which depends on the statistical fluctuations of the light. In conventional imaging systems, an extended detector, such as a CCD camera or an array detector, measures the spatial distribution of the optical intensity, which is proportional to the photon flux density. In interferometric systems, the spatial distribution of the optical field is inferred from measurements of the optical intensity. With the emergence of coherence theory, imaging systems based on measurements of the second-order coherence function at pairs of points in the detection plane were developed. An example is the imaging of an incoherent object based on the van Cittert-Zernike theorem. Imaging systems based on measurement of intensity correlation, or the photon coincidence rate, at pairs of points, were developed in the 1960s. A classic example of the photon-correlation imaging of an object emitting thermal light is stellar imaging using a Hanbury-Brown-Twiss intensity-correlation interferometer. More recently, two-photon light, which may be generated via spontaneous parametric downconversion in a second-order nonlinear optical crystal, has been used for imaging. This type of two-photon (or biphoton) imaging, which has come to be called quantum imaging, is also based on the measurement of photon coincidence by the use of photon-counting array detectors or by scanning two photon-counting detectors at pairs of points. To compare the resolution and sensitivity of imaging systems based on the aforementioned types of measurements, it is necessary to derive expressions for the measured quantities in terms of the object distribution. The point-spread functions based on such expressions can be used to assess the resolution. One measure of the sensitivity of the imaging process is the signal-to-noise ratio (SNR) of the measured variables. The statistical nature of the light source must be known in order to determine the SNR. The purpose of this chapter is to compare the resolution and sensitivity of photon-correlation imaging systems that make use of thermal light and two-photon light. We will henceforth refer to these two imaging modalities as classical and quantum photon-correlation imaging, or simply classical and quantum imaging, respectively. Clearly, light in other quantum states can also be used for imaging.