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Light force fluctuations in a strongly coupled atom-cavity system

Puppe, T, Maunz, P, Murr, K, Pepijn W. H. Pinkse, Rempe, G, Schuster, I

Published Feb 9, 2007• 2 citations
OpenAlex

Abstract

Between mirrors, the density of electromagnetic modes differs from the one in free space. This changes the radiation properties of an atom as well as the light forces acting on an atom. It has profound consequences in the strong-coupling regime of cavity quantum electrodynamics. For a single atom trapped inside the cavity, we investigate the atom-cavity system by scanning the frequency of a probe laser for various atom-cavity detunings. The avoided crossing between atom and cavity resonance is visible in the transmission of the cavity. It is also visible in the loss rate of the atom from the intracavity dipole trap. On the normal-mode resonances, the dominant contribution to the loss rate originates from dipole-force fluctuations which are dramatically enhanced in the cavity. This conclusion is supported by Monte-Carlo simulations.

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Between mirrors, the density of electromagnetic modes differs from the one in free space. This changes the radiation properties of an atom as well as the light forces acting on an atom. It has profound consequences in the strong-coupling regime of cavity quantum electrodynamics. For a single atom trapped inside the cavity, we investigate the atom-cavity system by scanning the frequency of a probe laser for various atom-cavity detunings. The avoided crossing between atom and cavity resonance is visible in the transmission of the cavity. It is also visible in the loss rate of the atom from the intracavity dipole trap. On the normal-mode resonances, the dominant contribution to the loss rate originates from dipole-force fluctuations which are dramatically enhanced in the cavity. This conclusion is supported by Monte-Carlo simulations.
Between mirrors, the density of electromagnetic modes differs from the one in free space. This changes the radiation properties of an atom as well as the light forces acting on an atom. It has profound consequences in the strong-coupling regime of cavity quantum electrodynamics. For a single atom trapped inside the cavity, we investigate the atom–cavity system by scanning the frequency of a probe laser for various atom–cavity detunings. The avoided crossing between atom and cavity resonance is visible in the transmission of the cavity. It is also visible in the loss rate of the atom from the intracavity dipole trap. On the normal-mode resonances, the dominant contribution to the loss rate originates from dipole-force fluctuations which are dramatically enhanced in the cavity. This conclusion is supported by Monte Carlo simulations.
Two recent experiments have reported the trapping of individual atoms inside optical resonators by the mechanical forces associated with single photons [Hood et al., Science 287, 1447 (2000); Pinkse et al., Nature (London) 404, 365 (2000)]. Here we analyze the trapping dynamics in these settings, focusing on two points of interest. First, we investigate the extent to which light-induced forces in these experiments are distinct from their free-space counterparts, and whether or not there are qualitatively different effects of optical forces at the single-photon level within the setting of cavity QED. Second, we explore the quantitative features of the resulting atomic motion, and how these dynamics are mapped onto experimentally observable variations of the intracavity field. Toward these ends, we present results from extensive numerical simulations of the relevant forces and their fluctuations, as well as a detailed derivation of our numerical simulation method, based on the full quantum-mechanical master equation. Not surprisingly, qualitatively distinct atomic dynamics arise as the coupling and dissipative rates are varied. For the experiment of Hood et al., we show that atomic motion is largely conservative and is predominantly in radial orbits transverse to the cavity axis. A comparison with the free-space theory demonstrates that the fluctuations of the dipole force are suppressed by an order of magnitude. This effect is based upon the Jaynes-Cummings eigenstates of the atom-cavity system and represents distinct physics for optical forces at the single-photon level within the context of cavity QED. By contrast, even in a regime of strong coupling in the experiment of Pinkse et al., there are only small quantitative distinctions between the potentials and heating rates in the free-space theory and the quantum theory, so it is not clear that a description of this experiment as a novel single-quantum trapping effect is necessary. The atomic motion is strongly diffusive, leading to an average localization time comparable to the time for an atom to transit freely through the cavity, and to a reduction in the ability to infer aspects of the atomic motion from the intracavity photon number.
The radiative properties of atoms inside an optical cavity can be dramatically changed with respect to those in free space. In the strong-coupling limit, the reversible dipole interaction between an atom and the cavity field dominates the irreversible decay resulting from spontaneous emission and cavity damping. In this limit the atom and field can no longer be regarded as separate quantities but instead form a composite dynamic system. To enhance the dipole coupling constant and increase the photon storage time, our experiments are performed with a small cavity 1 mm long, with a finesse of 8 × 104. On average, 0.4 photons are sufficient to saturate the resonance transition at 852 nm for the cesium atoms used, while the cooperativity parameter for a single atom is 2. Optical bistability is studied in this system over the range 3 < N < 65 atoms inside the cavity, with the semiclassical theory predicting bistability for N > 5. We report observations of manifestly quantum effects in this regime, including photon antibunching and sub-Poissonian photon statistics, with the magnitude of these nonclassical effects observed to be largely independent of the number of intracavity atoms.
Cooling is indispensable for trapping and observing single free atoms.In atomic physics, this can be achieved efficiently by laser cooling.Conventional methods to laser cool atoms are based on repeated optical pumping cycles followed by spontaneous emission of a photon from the atom.Such pumping schemes can only be applied to certain atomic species, which have a closed optical transition.Drawbacks caused by photons spontaneously emitted from the atom can be avoided in the strongly coupled atom-cavity system in which energy and entropy can be removed by photons lost from the cavity.This thesis reports on the first observation of this cooling mechanism which does not rely on spontaneous emission.In the experiment, a single atom is captured in an intracavity dipole trap.Illuminating the system with a weak, slightly blue-detuned light beam extends the storage time of the atom in the trap.The observed cooling force is at least five times larger than the force achieved by free-space cooling methods at comparable excitation of a two-level atom.Utilising cavity cooling, single atoms are prepared strongly-coupled to the mode of a high-finesse cavity.This allows to observe two well-resolved normal-mode peaks in both the cavity transmission as well as in the trap lifetime.The experiment is in agreement with a Monte Carlo simulation, demonstrating the localisation of the atom to within a tenth of a wavelength.The ability to individually excite the normal modes opens new possibilities to use this system for applications in quantum information science, including the realisation of quantum-logic gates.In the future cavity cooling might be applied to systems which cannot be cooled by conventional methods as for instance molecules or an atom carrying a quantum bit.
The process of single-atom transfer in strongly coupled cavity quantum electrodynamics (QED) with free falling atoms is investigated by experiment and Monte Carlo simulation. We conduct the simulation of the whole physical process and give the corresponding experimental results. In experiment, a high finesse optical cavity is used for real-time detection of the single-atom transits from which the interaction information between single atoms and cavity can be extracted, including the transmission spectra of the cavity strongly coupled to single atoms, the interaction duration of the single atoms in the mode, the probability distribution of atom arrival time and the atomic kinetic energy distribution when arriving at the mode. All these can be completely derived from the transmission spectra of the different initial status. An intracavity far-off resonance trap (FORT) has been established and the single-atom trapping time inside the cavity is about 5 ms which is about 30 times longer than that without FORT. This study gives the detailed analysis of the whole procedure of free-falling atom transfer in cavity QED system and is helpful for optimizing the experimental parameters and design.
It is usually considered that the spectrum of an optical cavity coupled to an atomic medium does not exhibit a normal-mode splitting unless the system satisfies the strong coupling condition, meaning the Rabi frequency of the coherent coupling exceeds the decay rates of atom and cavity excitations. Here we show that this need not be the case, but depends on the way in which the coupled system is probed. Measurements of the reflection of a probe laser from the input mirror of an overdamped cavity reveal an avoided crossing in the spectrum that is not observed when driving the atoms directly and measuring the Purcell-enhanced cavity emission. We understand these observations by noting a formal correspondence with electromagnetically induced transparency of a three-level atom in free space, where our cavity acts as the absorbing medium and the coupled atoms play the role of the control field.