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Heisenberg-scaling measurement of the single-photon Kerr non-linearity using mixed states

Geng Chen, N. Aharon, Yong-Nan Sun, Zi-Huai Zhang, Wen-Hao Zhang, De‐Yong He, Jian‐Shun Tang, Xiao-Ye Xu, Yaron Kedem, Chuan‐Feng Li, Guang‐Can Guo

Published Jan 1, 2018• 43 citations
OpenAlex

Abstract

Abstract Improving the precision of measurements is a significant scientific challenge. Previous works suggest that in a photon-coupling scenario the quantum fisher information shows a quantum-enhanced scaling of N2, which in theory allows a better-than-classical scaling in practical measurements. In this work, utilizing mixed states with a large uncertainty and a post-selection of an additional pure system, we present a scheme to extract this amount of quantum fisher information and experimentally attain a practical Heisenberg scaling. We performed a measurement of a single-photon’s Kerr non-linearity with a Heisenberg scaling, where an ultra-small Kerr phase of ≃6 × 10−8 rad was observed with a precision of ≃3.6 × 10−10 rad. From the use of mixed states, the upper bound of quantum fisher information is improved to 2N2. Moreover, by using an imaginary weak-value the scheme is robust to noise originating from the self-phase modulation.

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Abstract Improving the precision of measurements is a significant scientific challenge. Previous works suggest that in a photon-coupling scenario the quantum fisher information shows a quantum-enhanced scaling of N2, which in theory allows a better-than-classical scaling in practical measurements. In this work, utilizing mixed states with a large uncertainty and a post-selection of an additional pure system, we present a scheme to extract this amount of quantum fisher information and experimentally attain a practical Heisenberg scaling. We performed a measurement of a single-photon’s Kerr non-linearity with a Heisenberg scaling, where an ultra-small Kerr phase of ≃6 × 10−8 rad was observed with a precision of ≃3.6 × 10−10 rad. From the use of mixed states, the upper bound of quantum fisher information is improved to 2N2. Moreover, by using an imaginary weak-value the scheme is robust to noise originating from the self-phase modulation.
Abstract Improving the precision of measurements is a significant scientific challenge. Previous works suggest that in a photon-coupling scenario the quantum fisher information shows a quantum-enhanced scaling of N 2 , which in theory allows a better-than-classical scaling in practical measurements. In this work, utilizing mixed states with a large uncertainty and a post-selection of an additional pure system, we present a scheme to extract this amount of quantum fisher information and experimentally attain a practical Heisenberg scaling. We performed a measurement of a single-photon’s Kerr non-linearity with a Heisenberg scaling, where an ultra-small Kerr phase of ≃6 × 10 −8 rad was observed with a precision of ≃3.6 × 10 −10 rad. From the use of mixed states, the upper bound of quantum fisher information is improved to 2 N 2 . Moreover, by using an imaginary weak-value the scheme is robust to noise originating from the self-phase modulation.
Improving the precision of measurements is a prime challenge to the scientific community. Quantum metrology provides methods to overcome the standard quantum limit (SQL) of 1/sqrt{N} and to reach the fundamental Heisenberg-limit (HL) of 1/N. While a lot of theoretical and experimenta works have been dedicated to this task, most of the attempts focused on utilizing NOON and squeezed states, which exhibit unique quantum correlations. Here we present, and experimentally implement, a new scheme for precision measurements that enables reaching the HL. Our scheme is based on a probe in a mixed state with a large uncertainty, combined with a post-selection, such that the Fisher information is maximized, and the Carmer-Rao bound is saturated. We performed a Heisenberg limited measurement of the Kerr non-linearity of a single photon, where an ultra-small Kerr phase of 6 *10^{-8}$ was observed with an unprecedented precision of 10^{-9}. Our method paves the way to Heisenberg-limited metrology with only mixed state.
We propose a high-precision phase estimation scheme in a hybrid interferometer by synergistically combining a Kerr nonlinear phase shifter and multi-photon subtraction operations. Using a coherent state and a vacuum state as input resources, we systematically evaluate the phase sensitivity via homodyne detection and analyze the quantum Fisher information as well as the quantum Cramér-Rao bound under both ideal and lossy conditions. Our results show that the joint integration of Kerr nonlinearity and multi-photon subtraction yields remarkable advantages over either technique used alone. The proposed scheme enables the phase sensitivity to surpass the standard quantum limit, exceed the conventional Heisenberg scaling (1/N1/N1/N), and approach the super-Heisenberg scaling (1/N21/N^{2}1/N2)-a direct consequence of Kerr nonlinearity. More precisely, the super-Heisenberg scaling $\propto $ 1/N21/N^{2}1/N2 is the ultimate precision limit permitted by the k=2k=2k=2 Kerr nonlinearity and does not violate the fundamental Heisenberg limit for linear phase accumulation. Even under moderate internal photon loss, the system maintains high precision and exhibits enhanced robustness to decoherence. The Kerr nonlinearity introduces an intensity-dependent phase shift proportional to the squared photon number, while multi-photon subtraction tailors non-Gaussian states to strengthen phase information extraction. Compared with existing schemes based on hybrid interferometers or SU(1,1) interferometers, our architecture achieves superior precision and stronger loss resilience. All components are experimentally accessible with current quantum optical technologies. This work provides a promising route for practical high-precision quantum metrology and quantum sensing.
Abstract The precision of quantum measurements can be effectively improved by using both photon-added non-Gaussian operations and Kerr nonlinear phase shift. Here, we employ a coherent state mixed with a photon-added squeezed vacuum state as the input to a Mach–Zehnder interferometer with parity detection, thereby achieving a significant enhancement in phase measurement precision. Our research focuses on the phase sensitivity of linear phase shift under both ideal conditions and photon loss, as well as quantum Fisher information (QFI). The results demonstrate that employing the photon addition operations can markedly enhance phase sensitivity and QFI, and under optimal conditions, the measurement precision can approach the Heisenberg limit for the linear phase shift case. In addition, we delve deeper into the scenario of replacing the linear phase shift with a Kerr nonlinear one and systematically analyze the QFI under both ideal and photon loss conditions. By comparison, it is evident that employing both the photon addition operations and the Kerr nonlinear phase shift can further significantly enhance phase measurement precision while effectively improving the system’s robustness against photon loss. These findings are instrumental in facilitating the development and practical application of quantum metrology.
It has been suggested that both quantum superpositions and nonlinear interactions are important resources for quantum metrology. However, to date the different roles that these two resources play in the precision enhancement are not well understood. Here, we experimentally demonstrate a Heisenberg-scaling metrology to measure the parameter governing the nonlinear coupling between two different optical modes. The intense mode with n (more than 10^{6} in our work) photons manifests its effect through the nonlinear interaction strength which is proportional to its average photon number. The superposition state of the weak mode, which contains only a single photon, is responsible for both the linear Hamiltonian and the scaling of the measurement precision. By properly preparing the initial state of single photon and making projective photon-counting measurements, the extracted classical Fisher information (FI) can saturate the quantum FI embedded in the combined state after coupling, which is ∼n^{2} and leads to a practical precision ≃1.2/n. Free from the utilization of entanglement, our work paves a way to realize Heisenberg-scaling precision when only a linear Hamiltonian is involved.
Quantum metrology employs quantum resources to achieve measurement precision beyond classical limits. This work investigates a Mach--Zehnder interferometer incorporating a Kerr nonlinear phase shifter, with photon-added two-mode squeezed coherent states generated via four-wave mixing as input. We demonstrate that increasing both the photon-addition order and the input resource strength systematically enhances phase sensitivity, quantum Fisher information, and the corresponding quantum Cramér--Rao bound. The proposed system not only surpasses the standard quantum limit but also approaches or exceeds the Heisenberg limit for linear phase shifts, while Kerr nonlinearity enables surpassing the super-Heisenberg limit. Furthermore, the scheme exhibits enhanced robustness against photon loss, providing a promising pathway toward practical high-precision quantum metrology applications.